Numerical simulation of radionuclides migration in the far field of a geological repository

Safety conditions associated with geological repositories must be guaranteed also in the case of radionuclides migrating from the near field to the far field of a geological repository and to the external environment. For this reason the migration process of radionuclides and the factors affecting the process patterns have a crucial importance. In the present article, in order to simulate the migration process of radionuclides in the far-field of a geological repository, the groundwater simulation code PMWIN (Processing Modflow) is used, following a methodology applied by the same authors in a previous work. The present case study refers to a non-uniform groundwater flow field and shows the influence of two important parameters, the distribution coefficient and the hydraulic gradient. The results are compared with the ones previously obtained for the uniform flow case and the different scenarios are discussed

Risk Estimation and Expert Judgment: The Case of Yucca Mountain

Professor Shrader-Frechette discusses factors responsible for acute disagreement between the federal government and Nevada citizens over potential Risks at Yucca Mountain and focuses on the use of expert judgment, concluding that some of them appear to exemplify bad science. That aside, she argues that 1,000 year predictions cannot be made from current knowledge of geology or, e.g., institutional behavior and concludes that permanent disposal of radioactive waste is currently impossible

Microbial Effects on Repository Performance

This report presents a critical review of the international literature on microbial effects in and around a deep geological repository for higher activity wastes. It is aimed at those who are familiar with the nuclear industry and radioactive waste disposal, but who are not experts in microbiology; they may have a limited knowledge of how microbiology may be integrated into and impact upon radioactive waste disposal safety cases and associated performance assessments (PA)

Understanding radionuclide migration from the D1225 Shaft, Dounreay, Caithness, UK

A 65 m vertical shaft was sunk at Dounreay in the 1950s to build a tunnel for the offshore discharge of radioactive effluent from the various nuclear facilities then under construction. In 1959, the Shaft was licensed as a disposal facility for radioactive wastes and was routinely used for the disposal of ILW until 1970. Despite the operation of a hydraulic containment scheme, some radioactivity is known to have leaked into the surrounding rocks. Detailed logging, together with mineralogical and radiochemical analysis of drillcore has revealed four distinct bedding-parallel zones of contamination. The data show that Sr-90 dominates the bulk beta/gamma contamination signal, whereas Cs-137 and Pu-248/249 are found only to be weakly mobile, leading to very low activities and distinct clustering around the Shaft. The data also suggest that all uranium seen in the geosphere is natural in origin. At the smaller scale, contamination adjacent to fracture surfaces is present within a zone of enhanced porosity created by the dissolution of carbonate cements from the Caithness flagstones during long-term rockwater interactions. Quantitative modelling of radionuclide migration, using the multiphysics computer code QPAC shows the importance of different sorption mechanisms and different mineralogical substrates in the Caithnesss flagstones in controlling radionuclide migration

Detailed plan for the COMET WP3 initial research activity - list of research projects and goals, participants and timing

Detailed plan for the COMET Work Package (WP) 3

Modelling of radionuclide migration through the geosphere with radial basis function method and geostatistics

The modelling of radionuclide transport through the geosphere is necessary in the safety assessment of repositories for radioactive waste. A number of key geosphere processes need to be considered when predicting the movement of radionuclides through the geosphere. The most important input data are obtained from field measurements, which are not available for all regions of interest. For example, the hydraulic conductivity, as input parameter, varies from place to place. In such cases geostatistical science offers a variety of spatial estimation procedures. To assess the a long term safety of a radioactive waste disposal system, mathematical models are used to describe the complicated groundwater flow, chemistry and potential radionuclide migration through geological formations. The numerical solution of partial differential equations (PDEs) has usually been obtained by finite difference methods (FDM), finite element methods (FEM), or finite volume methods (FVM). Kansa introduced the concept of solving PDEs using radial basis functions (RBFs) for hyperbolic, parabolic and elliptic PDEs. The aim of this study was to present a relatively new approach to the modelling of radionuclide migration through the geosphere using radial basis functions methods and to determine the average and sample variance of radionuclide concentration with regard to spatial variability of hydraulic conductivity modelled by a geostatistical approach. We will also explore residual errors and their influence on optimal shape parameters

Integrating nuclide specific and dose rate based methods for airborne and ground based gamma spectrometry

Results of joint airborne survey work conducted by SUERC and JAEA are presented, for areas to the north and south of Fukushima Daiichi using four different airborne survey systems, cross calibrated at reference sites in Scotland and near Namie. Airborne measurements were made at a series of different survey heights using three high volume NaI based spectrometers, and for the first time using a high resolution system based on the Ortec IDM HPGe spectrometer. The JAEA data sets were analysed using the same methods applied to national scale mapping in Japan since the accident. The SUERC data sets were analysed using nuclide specific approaches validated in the European ECCOMAGS project. The data presented on a digital terrain model show marked correspondence with landscape features, which both suggest the initial deposition processes, and indicate trajectories for future re-deposition by natural processes. All data sets are traceable to each other, and to the ground based calibration sites. Nuclide specific inventories have been defined, which can serve as a future reference to evaluate environmental change

Natural attenuation of Fukushima-derived radiocesium in soils due to its vertical and lateral migration

Processes of vertical and lateral migration lead to gradual reduction in contamination of catchment soil, particularly its top layer. The reduction can be considered as natural attenuation. This, in turn, results in a gradual decrease of radiocesium activity concentrations in the surface runoff and river water, in both dissolved and particulate forms. The purpose of this research is to study the dynamics of Fukushima-derived radiocesium in undisturbed soils and floodplain deposits exposed to erosion and sedimentation during floods. Combined observations of radiocesium vertical distribution in soil and sediment deposition on artificial lawn-grass mats on the Niida River floodplain allowed us to estimate both annual mean sediment accumulation rates and maximum sedimentation rates corresponding to an extreme flood event during Tropical Storm Etau, 6-11 September 2015. Dose rates were reduced considerably for floodplain sections with high sedimentation because the top soil layer with high radionuclide contamination was eroded and/or buried under cleaner fresh sediments produced mostly due to bank erosion and sediments movements. Rate constants of natural attenuation on the sites of the Takase River and floodplain of Niida River was found to be in range 0.2-0.4 year-1. For the site in the lower reach of the Niida River, collimated shield dose readings from soil surfaces slightly increased during the period of observation from February to July 2016. Generally, due to more precipitation, steeper slopes, higher temperatures and increased biological activities in soils, self-purification of radioactive contamination in Fukushima associated with vertical and lateral radionuclide migration is faster than in Chernobyl. In many cases, monitored natural attenuation along with appropriate restrictions seems to be optimal option for water remediation in Fukushima contaminated areas