Modelling of a Two-Signal SFQ Detection Scheme for the Readout of Superconducting Nanowire Single Photon Detectors

We present a two-signal single flux quantum (SFQ) detection scheme for the purpose of reading out two pixels of a superconducting nanowire single photon detector (SNSPD). The circuit is based on a coincidence buffer element which is able to output a signal when both of its input lines are triggered. The circuit model for the SNSPD element is simulated in SPICE and optimized to match the experimental SNSPD response data. The two-signal detection scheme is simulated using JSIM which allows for the simulation of Josephson junction elements in a circuit. We demonstrate a model of the two-signal circuit operating with two simulated SNSPD pixel inputs and investigate the response of the scheme when a phase shift is applied to one of the inputs. The scheme shows potential as a useful coincidence detector of single photons. We also present preliminary experimental results of nanobridge-based Josephson junctions to be used in the realization of the coincidence detector circuit. Evidence of the nanobridges exhibiting Josephson behavior (SQUID modulation) are presented

Readout and Control Beyond a Few Qubits: Scaling-up Solid State Quantum Systems

Quantum entanglement and superposition, in addition to revealing interesting physics in their own right, can be harnessed as computational resources in a machine, enabling a range of algorithms for classically intractable problems. In recent years, experiments with small numbers of qubits have been demonstrated in a range of solid-state systems, but this is far from the numbers required to realise a useful quantum computer. In addition to the qubits themselves, quantum operation requires a host of classical electronics for control and readout, and current techniques used in few-qubit systems are not scalable. This thesis presents a series of techniques for control and readout of solid-state qubits, working towards scalability by integrating classical control with the quantum technology. Two techniques for reducing the footprint associated with readout of gallium arsenide spin qubits are demonstrated. Gate electrodes, used to define the quantum dot, are also shown to be sensitive state detectors. These gate-sensors, and the more conventional Quantum Point Contacts, are then multiplexed in the frequency domain, where three-channel qubit readout and ten-channel QPC readout are demonstrated. Two types of superconducting devices are also explored. The loss in superconducting coplanar waveguide resonators is measured, and a suppression of coupling to the parasitic electromagnetic environment is demonstrated. The thesis also details software for the simulation of Josephson-junction based circuits including features beyond what is available in commercial products. Finally, an architecture for managing control of a scalable machine is proposed where classical components are distributed throughout a cryostat and cryogenic switches route control pulses to the appropriate qubits. A simple implementation of the architecture is demonstrated that incorporates a double quantum dot, a gallium arsenide switch matrix, frequency multiplexed readout, and cryogenic classical computation

Superconducting single photon detectors for quantum information processing

Single photon detectors are a vital part of many emerging technologies which harness the quantum properties of light to benefit the fields of communication, computation and sensing. Superconducting nanowire single photon detectors (SNSPDs) offer high detection efficiency, low dark count rates, low timing jitter, and infrared sensitivity that are required by the most demanding single photon counting applications. This thesis presents SNSPDs fabricated and tested at the University of Glasgow that are integrated with optical structures which enable enhanced detection efficiency and integration with waveguide circuit technology. The monolithic integration of waveguide circuit components presents a route towards realisation of an optical quantum information processor that has the stability and scalability to perform the demanding tasks of quantum computation. A novel process is introduced for incorporating superconducting detectors with single mode gallium arsenide waveguides and quantum dot single photon sources. Together these elements would enable the generation of quantum states of light which could be manipulated and detected on a single chip. Detectors are patterned in NbTiN thin superconducting films on to suspended nanobeam waveguides with better than 50 nm alignment accuracy. Low temperature electrical and optical testing confirms the detectors’ single photon sensitivity under direct illumination as well as to waveguide coupled light. Measured detectors were found to have internal registering efficiencies of 6.8 ± 2.4%. Enhancing absorption of photons into thin superconducting films is vital to the creation of high efficiency superconducting single photon detectors. Fabricating an SNSPD on a dielectric mirror creates a partial cavity that can be tailored to enhance detection of light at specific wavelengths. Devices have been fabricated and tested in this thesis with enhanced detection efficiency at infrared and visible wavelengths for quantum cryptography, remote sensing and life science applications. Detectors fabricated in NbTiN on GaAs/AlGaAs Bragg mirrors exhibited a system detection efficiency of 1.5% at 1500 nm wavelength for the best device measured. SNSPDs were also fabricated in NbN on aperiodic dielectric mirrors with a range of different bandwidths. A peak system detection efficiency of 82.7% at 808 nm wavelength was recorded

Nano-optical studies of superconducting nanowire devices for single-photon detection

Superconducting nanowire single photon detectors (SNSPDs) are a rapidly maturing detector technology that offer superior performance relative to competing infrared photon counting technologies. The original experimental work presented here explores three novel methods of improving and analysing detector characteristics, employing low-temperature piezoelectric motors at temperatures below 4 K in a closed-cycle cryostat. Utilizing the low-temperature piezoelectric nanopositioners in tandem with a miniature confocal microscope, this work specifically shows a spatially-separable parallel-wire SNSPD demonstrating one- and two-pixel photon discrimination, with the detector responding more quickly when triggering two pixels. The work demonstrates nanoantenna-coupled SNSPDs, which are simulated, designed, and tested using the same nano-optical setup. In these an increased local absorption into the nanowire is seen at the antennas' resonant wavelengths, enhancing the efficiency of the detector by up to 130 %. Finally, a modified optical setup using a distributed Bragg reflector fibre in place of the microscope to form a tunable cavity around two configurations of SNSPD is demonstrated, improving absorption of the incident light into the nanowire across the whole active area. For these, enhancement in the system detection efficiency of up to 40 % is seen

Singlet oxygen luminescence detection

The detection of a single photon at 1270 nm wavelength allows the direct monitoring of Singlet Oxygen (1O2), making Singlet Oxygen Luminescence Detection (SOLD) a powerful dosimetry technique for photodynamic therapy in the treatment of cancer. However, the direct detection of 1O2 emission at 1270 nm wavelength is extremely challenging as the 1O2 → 3O2 transition in biological media has very low probability and short lifetime due to the high reactivity of singlet oxygen with biomolecules. Recent advances in single photon detection providing high detection efficiency, low noise single-photon detectors are an important innovation in the development of a practical SOLD system for eventual clinical use. In this thesis I present a compact fibre coupled SOLD system, using a supercontinuum pump source to precisely target exact photosensitizer absorption peak wavelengths and single-photon detectors for near-infrared detection by benchmarking a superconducting and a semiconductor photon counting detector. Both pump laser and detector are intrinsically fibre-coupled making them ideally suited for the development of practical singlet oxygen sensor head. The SOLD system was used to carry out a series of singlet oxygen time-resolved measurements in solution and in live cells. These measurements offer information on the photosensitized generation and deactivation of singlet oxygen generated by different photosensitizers and microenvironments at the 1270 nm wavelength and a first investigation of the 1590 nm singlet oxygen luminescence signal is presented

Experimental study of the quantum phase-slip effect in NbN nanowires

Coherent quantum phase-slip (QPS) in a superconducting nanowire is the dual phenomenon to the well-known Josephson effect. Josephson junctions form the basis of superconducting electronic circuits with a wide range of applications, and each of those circuits has a corresponding dual quantum phase-slip device with a dual purpose. Examples that draw particular attention are a new quantum standard of electric current, and a quantum phase-slip qubit. The aim of this project is to develop methods of design, fabrication, and measurement of quantum phase-slip nanowires, and to demonstrate the potential of these devices for technological application. In our experiments we incorporate NbN nanowires into a superconducting loop and bias the loop with a magnetic flux. The state of the nanowire-embedded loop is then read out by coupling to a high quality coplanar waveguide resonator. In this thesis we present the results of two such experiments. First, we fabricated NbN nanowires using a neon focused-ion-beam, and measured their properties at T=300 mK. Periodic tuning of the resonant frequency of the readout resonator revealed that magnetic flux is transferred to the interior of the loop with flux-quantum-periodicity. Our measurements confirm that the flux-quantum transfer is mediated by incoherent quantum phase-slips occurring in the nanowires, and that these incoherent QPS can be fully controlled with an external bias. In the second experiment, nanowire-embedded NbN loops were fabricated by electron-beam lithography and cooled to T=10 mK. The resonant frequency tuning exhibited avoided crossings, which is evidence of coherent coupling between the resonator and a coherent quantum two-level system. We numerically fit these avoided crossings to the Jaynes-Cummings model to extract the properties of the two-level system, and find a good fit with the design parameters of our nanowire qubit. Finally we discuss whether the observation of coherent dynamics is evidence of coherent QPS in the EBL-fabricated nanowire

Superinductance and fluctuating two-level systems: Loss and noise in disordered and non-disordered superconducting quantum devices

In this thesis, we first demonstrate that a disordered superconductor with high kinetic inductance can realise a microwave low-loss, non-dissipative circuit element with impedance greater than the quantum resistance. This element, known as a superinductor, can suppress the fluctuations of charge in a quantum circuit.For this purpose, we fabricated and characterised 20 nm thick, 40 nm wide niobium-nitride nanowires and determined the impedance to 6.795 kΩ. We demonstrate internal quality factors Qi = 2.5e4 in nanowire resonators at single photon excitation, which is significantly higher than values reported in devices with similar materials and geometries. Moreover, we show that the dominant dissipation in our nanowires is not an intrinsic property of the disordered films, but can instead be fully understood within the framework of two-level systems.To further characterise these losses, we then explore the geometrical scaling, toward nanowire dimensions, of dielectric losses in superconducting microwave resonators fabricated with the same techniques and from the same NbN thin-film as the nanowire superinductors. For this purpose, we perform an experimental and numerical study of dielectric loss at low temperatures. Using 3D finite-element simulation of the Maxwell--London equations, we compute the geometric filling factors of the lossy regions in our resonator structures and fit the experimental data to determine the intrinsic loss tangents of its interfaces and dielectrics. Finally, we study the effect of two-level systems on the performance of various superconducting quantum circuits. For this purpose, we measure coherence-time fluctuations in qubits and frequency fluctuations in resonators. In all devices, through statistical analysis, we identify the signature of individual Lorentzian fluctuators in the noise. We find that fluctuations in qubit relaxation are local to the qubit and are caused by instabilities of near-resonant two-level-systems. Furthermore, when examining the low-frequency noise of three different types of superconducting resonator - one NbN nanowire, one Al coplanar waveguide, and one Al 3D cavity - we observe a similar power-law dependence of the Lorentzian switching time and amplitude on the circulating power in the resonators, suggesting a common noise mechanism in the three different types of devices