Effect of Core Size on Performance of Fused-Ring Electron Acceptors

We report 4 fused-ring electron acceptors (FREAs) with the same end-groups and side-chains but different cores, whose sizes range from 5 to 11 fused rings. The core size has considerable effects on the electronic, optical, charge transport, morphological, and photovoltaic properties of the FREAs. Extending the core size leads to red-shift of absorption spectra, upshift of the energy levels, and enhancement of molecular packing and electron mobility. From 5 to 9 fused rings, the core size extension can simultaneously enhance open-circuit voltage (<i>V</i>_OC), short-circuit current density (<i>J</i>_SC), and fill factor (FF) of organic solar cells (OSCs). The best efficiency of the binary-blend devices increases from 5.6 to 11.7%, while the best efficiency of the ternary-blend devices increases from 6.3 to 12.6% as the acceptor core size extends

Synthesis of Ultrathin High-Entropy Oxides with Phase Controllability

High-entropy oxides (HEOs) with an ultrathin geometric structure are especially expected to exhibit extraordinary performance in different fields. The phase structure is deemed as a key factor in determining the properties of HEOs, rendering their phase control synthesis tempting. However, the disparity in intrinsic phase structures and physicochemical properties of multiple components makes it challenging to form single-phase HEOs with the target phase. Herein, we proposed a self-lattice framework-guided strategy to realize the synthesis of ultrathin HEOs with desired phase structures, including rock-salt, spinel, perovskite, and fluorite phases. The participation of the Ga assistor was conducive to the formation of the high-entropy mixing state by decreasing the formation energy. The as-prepared ultrathin spinel HEOs were demonstrated to be an excellent catalyst with high activity and stability for the oxygen evolution reaction in water electrolysis. Our work injects new vitality into the synthesis of HEOs for advanced applications and undoubtedly expedites their phase engineering

Additional file 3 of Transcriptome sequencing and metabolome analysis reveal the metabolic reprogramming of partial hepatectomy and extended hepatectomy

Additional file 3: Table S2. Expression patterns of all 14,505 reserved genes in eHx vs. pHx

Additional file 6 of Transcriptome sequencing and metabolome analysis reveal the metabolic reprogramming of partial hepatectomy and extended hepatectomy

Additional file 6: Figure S3. Metabolomic cluster dendrogram of different samples

Additional file 1 of Transcriptome sequencing and metabolome analysis reveal the metabolic reprogramming of partial hepatectomy and extended hepatectomy

Additional file 1: Table S1. All the reserved genes for differential analysis, the genes in all groups with a mean expression of < 3 read counts were filtered out

Additional file 5 of Transcriptome sequencing and metabolome analysis reveal the metabolic reprogramming of partial hepatectomy and extended hepatectomy

Additional file 5: Table S3. 1383 metabolites were filtered (variable coefficient ≥ 0.3) in all groups

Additional file 9 of Transcriptome sequencing and metabolome analysis reveal the metabolic reprogramming of partial hepatectomy and extended hepatectomy

Additional file 9: Figure S6. The pearson correlation analysis between qRT-PCR and RNA-seq

Additional file 10 of Transcriptome sequencing and metabolome analysis reveal the metabolic reprogramming of partial hepatectomy and extended hepatectomy

Additional file 10: Figure S7. The experimental workflow chart of this study

Additional file 4 of Transcriptome sequencing and metabolome analysis reveal the metabolic reprogramming of partial hepatectomy and extended hepatectomy

Additional file 4: Figure S2. The expression pattern of TOP10 DEGs of 5 clusters of pHx and eHx