1,287 research outputs found

    Observation of Parity-Unfavored Transitions in the Nonresonant Photoionization of Argon

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    Single-photon ionization of an atom or molecule can be subdivided into parity-favored and -unfavored transitions, the latter characterized by electron emission, preferentially perpendicular to the electric vector. The nonresonant existence of these transitions is shown experimentally and studied over an extended energy range for a variety of satellite transitions in atomic argon. The spectra exhibit several clearly resolved satellite lines with strongly negative β values close to -1, independent of the photon energy. The results confirm the corresponding predictions of angular-momentum transfer theory

    Electron-Energy and –Angular Distributions in the Double Photoionization of Helium

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    Photoelectron spectra of helium have been measured at different angles and at various energies above the double-ionization threshold up to 120 eV to investigate the behavior of the energy and angular distributions, of shake-off electrons. Both energy and angular distributions clearly show a U-shaped profile which turns to a flat curve near threshold pointing to a uniform intensity distribution over the kinetic energy for all angles in this excitation energy regime. Our results for the angular-distribution asymmetry parameter indicate qualitative agreement with theoretical predictions but fail to provide them quantitatively

    High-Resolution Photoelectron Spectrometry Study of Conjugate Shakeup Processes in the Li 1s Threshold Region

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    Partial cross sections and angular-distribution asymmetry parameters of diagram and satellite lines associated with Li 1s photoionization were measured using synchrotron-radiation excitation. Special emphasis was given to a high-resolution study of the 1P and 3P conjugate shakeup satellite lines testing qualitative predictions of the conjugate shakeup model: increasing σ and decreasing β values towards threshold, both being verified. Comparison with recent relaxed Hartree-Fock calculations shows good agreement for the 1P satellite, but demonstrates also that the present theory does not seem to be able to describe the cross-section behavior of the 3P satellite correctly

    Natural widths in open-shell atoms: The K absorption spectrum of atomic oxygen

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    Total-ion-yield measurements and Hartree-Fock calculations are presented for the 1s→np, n=2 to 5 photoexcitations in atomic oxygen. Energies and relative intensities of the [1s]2s22p4(4P)np and [1s]2s22p4(2P)np series members are determined, and the apparent linewidths are measured. It is shown that natural widths in an open-shell atom can be deduced from an absorption spectrum only with the aid of theoretical input. The linewidth for the six individual components contained in the 1s→2p transition is determined to be 140(9) meV

    Dual-path state reconstruction scheme for propagating quantum microwaves and detector noise tomography

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    Quantum state reconstruction involves measurement devices that are usually described by idealized models, but not known in full detail in experiments. For weak propagating microwaves, the detection process requires linear amplifiers which obscure the signal with random noise. Here, we introduce a theory which nevertheless allows one to use these devices for measuring all quadrature moments of propagating quantum microwaves based on cross-correlations from a dual-path amplification setup. Simultaneously, the detector noise properties are determined, allowing for tomography. We demonstrate the feasibility of our novel concept by proof-of-principle experiments with classical mixtures of weak coherent microwaves.Comment: 11 pages, 3 figure

    Evidence for Atomic Processes in Molecular Valence Double Ionization

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    Complete molecular valence-electron spectra were measured for CO. Unexpectedly, discrete lines at low kinetic energies were found, superimposed on a continuous energy spectrum representing direct double-ionization processes. The appearance of these lines is discussed in the context of the formation of the C++O+ ion pair near its associated threshold at 38.4 eV. It is ascribed to valence-excited repulsive (CO+)* states, which dissociate to a large part rapidly into atomic fragments before electronic relaxation takes place. From our spectra, partial cross sections for the different processes leading to dissociative valence double ionization are derived

    Comparing extractions of Sivers functions

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    A comparison is given of the various recently published extractions of the Sivers functions from the HERMES and COMPASS data on single-transverse spin asymmetries in semi-inclusive deeply inelastic scattering.Comment: Contribution to the proceedings of "The International Workshop on Transverse Polarisation Phenomena in Hard Processes" (Transversity 2005), Villa Olmo (Como), 7-10th. September 200

    Natural Widths In Open-Shell Atoms: The K Absorption Spectrum Of Atomic Oxygen

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    Total-ion-yield measurements and Hartree-Fock calculations are presented for the 1s-- \u3enp, n=2 to 5 photoexcitations in atomic oxygen. Energies and relative intensities of the [1s]2s(2)2p(4)(P-4)np and [1s]2s(2)2p(4)(P-2)np series members are determined, and the apparent linewidths are measured. It is shown that natural widths in an open-shell atom can be deduced from an absorption spectrum only with the aid of theoretical input. The linewidth for the six individual components contained in the 1s--\u3e2p transition is determined to be 140(9) meV

    Multiplet-Changing Auger Transitions in Valence Double Photoionization

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    The decay of valence satellite states in neon above the first double-ionization threshold has been studied experimentally and theoretically. Special emphasis was given to differentiate between two decay modes: valence Auger and valence-multiplet Auger decay. It is shown that the latter process is predominant in the low kinetic energy part of the spectrum. The main structures of this low-energy Auger spectrum could be designated by help of calculated transition energies and decay rates
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