11,804 research outputs found
Anomalous electronic Raman scattering in Na_xCoO_2 H_2O
Raman scattering experiments on Na_{x}CoO_2 yH_2O single crystals show a
broad electronic continuum with a pronounced peak around 100 cm-1 and a cutoff
at approximately 560 cm-1over a wide range of doping levels. The electronic
Raman spectra in superconducting and non-superconducting samples are similar at
room temperature, but evolve in markedly different ways with decreasing
temperature. For superconducting samples, the low-energy spectral weight is
depleted upon cooling below T* sim 150K, indicating a opening of a pseudogap
that is not present in non-superconducting materials. Weak additional phonon
modes observed below T* suggest that the pseudogap is associated with charge
ordering.Comment: 5 pages, 4 figures, for further information see www.peter-lemmens.d
Resonance peak in underdoped cuprates
The magnetic susceptibility measured in neutron scattering experiments in
underdoped YBaCuO is interpreted based on the self-consistent
solution of the t-J model of a Cu-O plane. The calculations reproduce correctly
the frequency and momentum dependencies of the susceptibility and its variation
with doping and temperature in the normal and superconducting states. This
allows us to interpret the maximum in the frequency dependence -- the resonance
peak -- as a manifestation of the excitation branch of localized Cu spins and
to relate the frequency of the maximum to the size of the spin gap. The
low-frequency shoulder well resolved in the susceptibility of superconducting
crystals is connected with a pronounced maximum in the damping of the spin
excitations. This maximum is caused by intense quasiparticle peaks in the hole
spectral function for momenta near the Fermi surface and by the nesting.Comment: 9 pages, 6 figure
Pressure-induced hole doping of the Hg-based cuprate superconductors
We investigate the electronic structure and the hole content in the
copper-oxygen planes of Hg based high Tc cuprates for one to four CuO2 layers
and hydrostatic pressures up to 15 GPa. We find that with the pressure-induced
additional number of holes of the order of 0.05e the density of states at the
Fermi level changes approximately by a factor of 2. At the same time the saddle
point is moved to the Fermi level accompanied by an enhanced k_z dispersion.
This finding explains the pressure behavior of Tc and leads to the conclusion
that the applicability of the van Hove scenario is restricted. By comparison
with experiment, we estimate the coupling constant to be of the order of 1,
ruling out the weak coupling limit.Comment: 4 pages, 4 figure
Optical properties, electron-phonon coupling, and Raman scattering of vanadium ladder compounds
The electronic structure of two V-based ladder compounds, the quarter-filled
NaVO in the symmetric phase and the iso-structural half-filled
CaVO is investigated by ab initio calculations. Based on the
bandstructure we determine the dielectric tensor of these
systems in a wide energy range. The frequencies and eigenvectors of the fully
symmetric A phonon modes and the corresponding electron-phonon and
spin-phonon coupling parameters are also calculated from first-principles. We
determine the Raman scattering intensities of the A phonon modes as a
function of polarization and frequency of the exciting light.
All results, i.e. shape and magnitude of the dielectric function, phonon
frequencies and Raman intensities show very good agreement with available
experimental data.Comment: 11 pages, 10 figure
Electron-phonon and spin-phonon coupling in NaVO: charge fluctuations effect
We show that the asymmetric crystal environment of the V site in the ladder
compound NaVO leads to a strong coupling of vanadium 3d electrons
to phonons. This coupling causes fluctuations of the charge on the V ions, and
favors a transition to a charge-ordered state at low temperatures. In the low
temperature phase the charge fluctuations modulate the spin-spin superexchange
interaction, resulting in a strong spin-phonon coupling.Comment: Europhysics Letters, to be publishe
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