593 research outputs found
Evaporation of buffer gas-thermalized anions out of a multipole rf ion trap
We identify plain evaporation of ions as the fundamental loss mechanism out
of a multipole ion trap. Using thermalized negative Cl- ions we find that the
evaporative loss rate is proportional to a Boltzmann factor. This thermodynamic
description sheds new light on the dynamics of particles in time-varying
confining potentials. It specifically allows us to extract the effective depth
of the ion trap as the activation energy for evaporation. As a function of the
rf amplitude we find two distinct regimes related to the stability of motion of
the trapped ions. For low amplitudes the entire trap allows for stable motion
and the trap depth increases with the rf field. For larger rf amplitudes,
however, rapid energy transfer from the field to the ion motion can occur at
large trap radii, which leads to a reduction of the effective trapping volume.
In this regime the trap depth decreases again with increasing rf amplitude. We
give an analytical parameterization of the trap depth for various multipole
traps that allows predictions of the most favorable trapping conditions.Comment: Phys. Rev. Lett., in pres
Potential and limitations of nucleon transfer experiments with radioactive beams at REX-ISOLDE
As a tool for studying the structure of nuclei far off stability the
technique of gamma-ray spectroscopy after low-energy single-nucleon transfer
reactions with radioactive nuclear beams in inverse kinematics was
investigated. Modules of the MINIBALL germanium array and a thin
position-sensitive parallel plate avalanche counter (PPAC) to be employed in
future experiments at REX-ISOLDE were used in a test experiment performed with
a stable 36S beam on deuteron and 9Be targets. It is demonstrated that the
Doppler broadening of gamma lines detected by the MINIBALL modules is
considerably reduced by exploiting their segmentation, and that for beam
intensities up to 10^6 particles/s the PPAC positioned around zero degrees with
respect to the beam axis allows not only to significantly reduce the gamma
background by requiring coincidences with the transfer products but also to
control the beam and its intensity by single particle counting. The predicted
large neutron pickup cross sections of neutron-rich light nuclei on 2H and 9Be
targets at REX-ISOLDE energies of 2.2 MeV A are confirmed.Comment: 11 pages, 8 figure
A renormalisation approach to excitable reaction-diffusion waves in fractal media
Of fundamental importance to wave propagation in a wide range of physical phenomena is the structural geometry of the supporting medium. Recently, there have been several investigations on wave propagation in fractal media. We present here a renormalization approach to the study of reaction-diffusion (RD) wave propagation on finitely ramified fractal structures. In particular we will study a Rinzel-Keller (RK) type model, supporting travelling waves on a Sierpinski gasket (SG), lattice
Energy-sensitive imaging detector applied to the dissociative recombination of D2H+
We report on an energy-sensitive imaging detector for studying the
fragmentation of polyatomic molecules in the dissociative recombination of fast
molecular ions with electrons. The system is based on a large area (10 cm x 10
cm) position-sensitive, double-sided Si-strip detector with 128 horizontal and
128 vertical strips, whose pulse height information is read out individually.
The setup allows to uniquely identify fragment masses and is thus capable of
measuring branching ratios between different fragmentation channels, kinetic
energy releases, as well as breakup geometries, as a function of the relative
ion-electron energy. The properties of the detection system, which has been
installed at the TSR storage ring facility of the Max-Planck Institute for
Nuclear Physics in Heidelberg, is illustrated by an investigation of the
dissociative recombination of the deuterated triatomic hydrogen cation D2H+. A
huge isotope effect is observed when comparing the relative branching ratio
between the D2+H and the HD+D channel; the ratio 2B(D2+H)/B(HD+D), which is
measured to be 1.27 +/- 0.05 at relative electron-ion energies around 0 eV, is
found to increase to 3.7 +/- 0.5 at ~5 eV.Comment: 11 pages, 12 figures, submitted to Physical Review
Dissociative recombination measurements of HCl+ using an ion storage ring
We have measured dissociative recombination of HCl+ with electrons using a
merged beams configuration at the heavy-ion storage ring TSR located at the Max
Planck Institute for Nuclear Physics in Heidelberg, Germany. We present the
measured absolute merged beams recombination rate coefficient for collision
energies from 0 to 4.5 eV. We have also developed a new method for deriving the
cross section from the measurements. Our approach does not suffer from
approximations made by previously used methods. The cross section was
transformed to a plasma rate coefficient for the electron temperature range
from T=10 to 5000 K. We show that the previously used HCl+ DR data
underestimate the plasma rate coefficient by a factor of 1.5 at T=10 K and
overestimate it by a factor of 3.0 at T=300 K. We also find that the new data
may partly explain existing discrepancies between observed abundances of
chlorine-bearing molecules and their astrochemical models.Comment: Accepted for publication in ApJ (July 7, 2013
Enhanced dielectronic recombination of lithium-like Ti19+ ions in external ExB fields
Dielectronic recombination(DR) of lithium-like Ti19+(1s2 2s) ions via 2s->2p
core excitations has been measured at the Heidelberg heavy ion storage ring
TSR. We find that not only external electric fields (0 <= Ey <= 280 V/cm) but
also crossed magnetic fields (30 mT <= Bz <= 80 mT) influence the DR via high-n
(2p_j nl)-Rydberg resonances. This result confirms our previous finding for
isoelectronic Cl14+ ions [Bartsch T et al, PRL 82, 3779 (1999)] that
experimentally established the sensitivity of DR to ExB fields. In the present
investigation the larger 2p_{1/2}-2p_{3/2} fine structure splitting of Ti19+
allowed us to study separately the influence of external fields via the two
series of Rydberg DR resonances attached to the 2s -> 2p_{1/2} and 2s ->
2p_{3/2} excitations of the Li-like core, extracting initial slopes and
saturation fields of the enhancement. We find that for Ey > 80 V/cm the field
induced enhancement is about 1.8 times stronger for the 2p_{3/2} series than
for the 2p_{1/2} series.Comment: 10 pages, 3 figures, to be published in Journal of Physics B, see
also http://www.strz.uni-giessen.de/~k
Dielectronic Recombination in Photoionized Gas. II. Laboratory Measurements for Fe XVIII and Fe XIX
In photoionized gases with cosmic abundances, dielectronic recombination (DR)
proceeds primarily via nlj --> nl'j' core excitations (Dn=0 DR). We have
measured the resonance strengths and energies for Fe XVIII to Fe XVII and Fe
XIX to Fe XVIII Dn=0 DR. Using our measurements, we have calculated the Fe
XVIII and Fe XIX Dn=0 DR DR rate coefficients. Significant discrepancies exist
between our inferred rates and those of published calculations. These
calculations overestimate the DR rates by factors of ~2 or underestimate it by
factors of ~2 to orders of magnitude, but none are in good agreement with our
results. Almost all published DR rates for modeling cosmic plasmas are computed
using the same theoretical techniques as the above-mentioned calculations.
Hence, our measurements call into question all theoretical Dn=0 DR rates used
for ionization balance calculations of cosmic plasmas. At temperatures where
the Fe XVIII and Fe XIX fractional abundances are predicted to peak in
photoionized gases of cosmic abundances, the theoretical rates underestimate
the Fe XVIII DR rate by a factor of ~2 and overestimate the Fe XIX DR rate by a
factor of ~1.6. We have carried out new multiconfiguration Dirac-Fock and
multiconfiguration Breit-Pauli calculations which agree with our measured
resonance strengths and rate coefficients to within typically better than
<~30%. We provide a fit to our inferred rate coefficients for use in plasma
modeling. Using our DR measurements, we infer a factor of ~2 error in the Fe XX
through Fe XXIV Dn=0 DR rates. We investigate the effects of this estimated
error for the well-known thermal instability of photoionized gas. We find that
errors in these rates cannot remove the instability, but they do dramatically
affect the range in parameter space over which it forms.Comment: To appear in ApJS, 44 pages with 13 figures, AASTeX with postsript
figure
A Global Potential Analysis of the O+Si Reaction Using a New Type of Coupling Potential
A new approach has been used to explain the experimental data for the
O+Si system over a wide energy range in the laboratory system
from 29.0 to 142.5 MeV. A number of serious problems has continued to plague
the study of this system for a couple of decades. The explanation of anomalous
large angle scattering data; the reproduction of the oscillatory structure near
the Coulomb barrier; the out-of-phase problem between theoretical predictions
and experimental data; the consistent description of angular distributions
together with excitation functions data are just some of these problems. These
are long standing problems that have persisted over the years and do represent
a challenge calling for a consistent framework to resolve these difficulties
within a unified approach. Traditional frameworks have failed to describe these
phenomena within a single model and have so far only offered different
approaches where these difficulties are investigated separately from one
another. The present work offers a plausible framework where all these
difficulties are investigated and answered. Not only it improves the
simultaneous fits to the data of these diverse observables, achieving this
within a unified approach over a wide energy range, but it departs for its
coupling potential from the standard formulation. This new feature is shown to
improve consistently the agreement with the experimental data and has made
major improvement on all the previous coupled-channels calculations for this
system.Comment: 21 pages with 12 figure
Anisotropic fragmentation in low-energy dissociative recombination
On a dense energy grid reaching up to 75 meV electron collision energy the
fragmentation angle and the kinetic energy release of neutral dissociative
recombination fragments have been studied in a twin merged beam experiment. The
anisotropy described by Legendre polynomials and the extracted rotational state
contributions were found to vary on a likewise narrow energy scale as the
rotationally averaged rate coefficient. For the first time angular dependences
higher than 2 order could be deduced. Moreover, a slight anisotropy at
zero collision energy was observed which is caused by the flattened velocity
distribution of the electron beam.Comment: 8 pages, 4 figures; The Article will be published in the proceedings
of DR 2007, a symposium on Dissociative Recombination held in Ameland, The
Netherlands (18.-23. July 2008); Reference 19 has been published meanwhile in
S. Novotny, PRL 100, 193201 (2008
One Dimensional Oxygen Ordering in YBa2Cu3O(7-delta)
A model consisting of oxygen-occupied and -vacant chains is considered, with
repulsive first and second nearest-neighbor interactions V1 and V2,
respectively. The statistical mechanics and the diffraction spectrum of the
model is solved exactly and analytically with the only assumption V1 >> V2. At
temperatures T ~ V1 only a broad maximum at (1/2,0,0) is present, while for
ABS(delta - 1/2) > 1/14 at low enough T, the peak splits into two. The simple
expression for the diffraction intensity obtained for T << V1 represents in a
more compact form previous results of Khachaturyan and Morris[1],extends them
to all delta and T/V2 and leads to a good agreement with experiment. [1]
A.G.Khachaturyan and J.W.Morris, Jr., Phys.Rev.Lett. 64,76(1990)Comment: 13 pages,Revtex,3 figures available upon request but can be plotted
using simple analytical functions,CNEA-CAB 92/04
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