Nonlocal study of ultimate plasmon hybridization

Within our recently proposed generalized nonlocal optical response (GNOR) model, we revisit the fundamental problem of an optically excited plasmonic dimer. The dimer consists of two identical cylinders separated by a nanometre-sized gap. We consider the transition from separated dimers via touching dimers to finally overlapping dimers. In particular, we focus on the touching case, showing a fundamental limit on the hybridization of the bonding plasmon modes due to nonlocality. Using transformation optics we determine a simple analytical equation for the resonance energies of the bonding plasmon modes of the touching dimer

Generalized nonlocal optical response in nanoplasmonics

Metallic nanostructures exhibit a multitude of optical resonances associated with localized surface plasmon excitations. Recent observations of plasmonic phenomena at the sub-nanometer to atomic scale have stimulated the development of various sophisticated theoretical approaches for their description. Here instead we present a comparatively simple semiclassical generalized nonlocal optical response (GNOR) theory that unifies quantum-pressure convection effects and induced-charge diffusion kinetics, with a concomitant complex-valued GNOR parameter. Our theory explains surprisingly well both the frequency shifts and size-dependent damping in individual metallic nanoparticles (MNPs) as well as the observed broadening of the cross-over regime from bonding-dipole plasmons to charge-transfer plasmons in MNP dimers, thus unraveling a classical broadening mechanism that even dominates the widely anticipated short-circuiting by quantum tunneling. We anticipate that the GNOR theory can be successfully applied in plasmonics to a wide class of conducting media, including doped semiconductors and low-dimensional materials such as graphene.Comment: 7 pages, including 3 figures. Supplementary information is available upon request to author

Nanoplasmonics beyond Ohm's law

In tiny metallic nanostructures, quantum confinement and nonlocal response change the collective plasmonic behavior with important consequences for e.g. field-enhancement and extinction cross sections. We report on our most recent developments of a real-space formulation of an equation-of-motion that goes beyond the common local-response approximation and use of Ohm's law as the central constitutive equation. The electron gas is treated within a semi-classical hydrodynamic model with the emergence of a new intrinsic length scale. We briefly review the new governing wave equations and give examples of applying the nonlocal framework to calculation of extinction cross sections and field enhancement in isolated particles, dimers, and corrugated surfaces.Comment: Invited paper for TaCoNa-Photonics 2012 (www.tacona-photonics.org), to appear in AIP Conf. Pro

What does a primary care annual review for RA include? A national GP survey

Letter to the edito