Reduced transition probabilities for the gamma decay of the 7.8 eV isomer in 229^{229}Th

The reduced magnetic dipole and electric quadrupole transition probabilities for the radiative decay of the $^{229}$Th 7.8 eV isomer to the ground state are predicted within a detailed nuclear-structure model approach. We show that the presence and decay of this isomer can only be accounted for by the Coriolis mixing emerging from a remarkably fine interplay between the coherent quadrupole-octupole motion of the nuclear core and the single-nucleon motion within a reflection-asymmetric deformed potential. We find that the magnetic dipole transition probability which determines the radiative lifetime of the isomer is considerably smaller than presently estimated. The so-far disregarded electric quadrupole component may have non-negligible contributions to the internal conversion channel. These findings support new directions in the experimental search of the $^{229}$Th transition frequency for the development of a future nuclear frequency standard.Comment: 5 pages, 1 figure, supplementary material is available as pdf with the source files, v3 includes small corrections to match the published version, results unchange

Stopping narrow-band x-ray pulses in nuclear media

A control mechanism for stopping x-ray pulses in resonant nuclear media is investigated theoretically. We show that narrow-band x-ray pulses can be mapped and stored as nuclear coherence in a thin-film planar x-ray cavity with an embedded $^{57}\mathrm{Fe}$ nuclear layer. The pulse is nearly resonant to the 14.4 keV M\"ossbauer transition in the $^{57}\mathrm{Fe}$ nuclei. The role of the control field is played here by a hyperfine magnetic field which induces interference effects reminding of electromagnetically induced transparency. We show that by switching off the control magnetic field, a narrow-band x-ray pulse can be completely stored in the cavity for approximately 100 ns. Additional manipulation of the external magnetic field can lead to both group velocity and phase control of the pulse in the x-ray cavity sample.Comment: 5 pages, 3 figures; v2 slight modifications in title, abstract, marketing, to match the final published version; added a supplementary material; results unchange

Determination of plasma screening effects for thermonuclear reactions in laser-generated plasmas

Due to screening effects, nuclear reactions in astrophysical plasmas may behave differently than in the laboratory. The possibility to determine the magnitude of these screening effects in colliding laser-generated plasmas is investigated theoretically, having as a starting point a proposed experimental setup with two laser beams at the Extreme Light Infrastructure facility. A laser pulse interacting with a solid target produces a plasma through the Target Normal Sheath Acceleration scheme, and this rapidly streaming plasma (ion flow) impacts on a secondary plasma created by the interaction of a second laser pulse on a gas jet target. We model this scenario here and calculate the reaction events for the astrophysically relevant reaction $^{13}$C($^4$He, $n$)$^{16}$O. We find that it should be experimentally possible to determine the plasma screening enhancement factor for fusion reactions by detecting the difference in reaction events between two scenarios of ion flow interacting with the plasma target and a simple gas target. This provides a way to evaluate nuclear reaction cross-sections in stellar environments and can significantly advance the field of nuclear astrophysics.Comment: 9 pages, 4 figures, 4 tables; minor changes made, accepted by The Astrophysical Journa

Coherent control of nuclear forward scattering

The possibility to control the coherent decay of resonant excitations in nuclear forward scattering is investigated. By changing abruptly the direction of the nuclear hyperfine magnetic field, the coherent scattering of photons can be manipulated and even completely suppressed via quantum interference effects between the nuclear transition currents. The efficiency of the coherent decay suppression and the dependence of the scattered light polarization on the specific switching parameters is analyzed in detail. Using a sophisticated magnetic switching sequence involving four rotations of the hyperfine magnetic field, two correlated coherent decay pulses with different polarizations can be generated out of one excitation, providing single-photon entanglement in the keV regime. The verification of the generated entanglement by testing a single-particle version of Bell's inequality in an x-ray optics experimental setup is put forward.Comment: 22 pages, 6 figures; revised to match the published version: added one figure, small modifications in tex

Optomechanically induced transparency of x-rays via optical control

The search for new control methods over light-matter interactions is one of the engines that advances fundamental physics and applied science alike. A specific class of light-matter interaction interfaces are setups coupling photons of distinct frequencies via matter. Such devices, nontrivial in design, could be endowed with multifunctional tasking. Here we envisage for the first time an optomechanical system that bridges optical and robust, high-frequency x-ray photons, which are otherwise notoriously difficult to control. The x-ray-optical system comprises of an optomechanical cavity and a movable microlever interacting with an optical laser and with x-rays via resonant nuclear scattering. We show that optomechanically induced transparency of a broad range of photons (10 eV-100 keV) is achievable in this setup, allowing to tune nuclear x-ray absorption spectra via optomechanical control. This paves ways for metrology applications, e.g., the detection of the $^{229}$Thorium clock transition, and an unprecedentedly precise control of x-rays using optical photons.Comment: 2 figures, supplementary material available with the file

Quantum interference between nuclear excitation by electron capture and radiative recombination

We investigate the quantum interference between the resonant process of nuclear excitation by electron capture (NEEC) followed by the radiative decay of the excited nucleus, and radiative recombination (RR). In order to derive the interference cross section, a Feshbach projection operator formalism is used. The electromagnetic field is considered by means of multipole fields. The nucleus is described by a phenomenological collective model and by making use of experimental data. The Fano profile parameters as well as the interference cross section for electric and magnetic multipole transitions in various heavy ions are presented. We discuss the experimental possibility of discerning NEEC from the RR background

Coupling highly excited nuclei to the atomic shell in dense astrophysical plasmas

In dense astrophysical plasmas, neutron capture populates highly excited nuclear states close to the neutron threshold. The impact of additional low-energy nuclear excitations via coupling to the atomic shell on the ability of the so-formed compound nucleus to retain the captured neutron is investigated. We focus on the mechanism of nuclear excitation by electron capture in plasmas characterized by electron fluxes typical for the slow neutron capture process of stellar nucleosynthesis. The small effect of this further excitation on the neutron capture and gamma decay sequence relevant for nucleosynthesis is quantified and compared to the corresponding effect of an additional low-energy photoexcitation step.Comment: 11 pages, 10 figures; v2 minor modifications to match the published version, results unchange

Quantum interference effects in an ensemble of 229^{229}Th nuclei interacting with coherent light

As a unique feature, the $^{229}$Th nucleus has an isomeric transition in the vacuum ultraviolet that can be accessed by optical lasers. The interference effects occurring in the interaction between coherent optical light and an ensemble of $^{229}$Th nuclei are investigated theoretically. We consider the scenario of nuclei doped in vacuum ultraviolet-vacuum ultraviolet transparent crystals and take into account the effect of different doping sites and therefore different lattice fields that broaden the nuclear transition width. This effect is shown to come in interplay with interference effects due to the hyperfine splitting of the ground and isomeric nuclear states. We investigate possible experimentally available situations involving two-, three- and four-level schemes of quadrupole sublevels of the ground and isomeric nuclear states coupling to one or two coherent fields. Specific configurations which offer clear signatures of the isomer excitation advantageous for the more precise experimental determination of the transition energy are identified. Furthermore, it is shown that population trapping into the isomeric state can be achieved. This paves the way for further nuclear quantum optics applications with $^{229}$Th such as nuclear coherent control.Comment: 14 papes, 13 figure

The electric quadrupole channel of the 7.8 eV 229Th~^{229}\mathrm{Th} transition

The unique isomeric transition at 7.8 eV in $~^{229}\mathrm{Th}$ has a magnetic dipole ($M1$) and an electric quadrupole ($E2$) multipole mixing. So far, the $E2$ component has been widely disregarded. Here, we investigate the nuclear physics nature and the impact of the $E2$ decay channel for the nuclear coupling to the atomic shell based on the newest theoretical predictions for the corresponding reduced nuclear transition probabilities. Our results show that the contribution of the $E2$ channel is dominant or at least of the same order of magnitude for internal conversion or electronic bridge transitions involving the atomic orbitals $7p$, $6d$ and $5f$. Notable exceptions are the internal conversion of the $7s$ electron and the electronic bridge between the electronic states $7s$ and $7p$, for which the $M1$ component dominates by two to three orders of magnitude. Caution is therefore advised when considering isomeric excitation or decay via nuclear coupling to the atomic shell, as the involved orbitals determine which multipole transition component dominates