170 research outputs found
Spin Fluctuations and the Pseudogap in Organic Superconductors
We show that there are strong similarities in the spin lattice relaxation of
non-magnetic organic charge transfer salts, and that these similarities can be
understood in terms of spin fluctuations. Further, we show that, in all of the
kappa-phase organic superconductors for which there is nuclear magnetic
resonance data, the energy scale for the spin fluctuations coincides with the
energy scale for the pseudogap. This suggests that the pseudogap is caused by
short-range spin correlations. In the weakly frustrated metals
k-(BEDT-TTF)_2Cu[N(CN)_2]Br, k-(BEDT-TTF)_2Cu(NCS)_2, and
k-(BEDT-TTF)_2Cu[N(CN)_2]Cl (under pressure) the pseudogap opens at the same
temperature as coherence emerges in the (intralayer) transport. We argue that
this is because the spin correlations are cut off by the loss of intralayer
coherence at high temperatures. We discuss what might happen to these two
energy scales at high pressures, where the electronic correlations are weaker.
In these weakly frustrated materials the data is well described by the chemical
pressure hypothesis (that anion substitution is equivalent to hydrostatic
pressure). However, we find important differences in the metallic state of
k-(BEDT-TTF)_2Cu_2(CN)_3, which is highly frustrated and displays a spin liquid
insulating phase. We also show that the characteristic temperature scale of the
spin fluctuations in (TMTSF)_2ClO_4 is the same as superconducting critical
temperature, which may be evidence that spin fluctuations mediate the
superconductivity in the Bechgaard salts.Comment: 7 pages, 4 figures; to appear in PR
Novel Crossover in Coupled Spin Ladders
We report a novel crossover behavior in the long-range-ordered phase of a
prototypical spin- Heisenberg antiferromagnetic ladder compound
. The staggered order was previously evidenced
from a continuous and symmetric splitting of N NMR spectral lines on
lowering temperature below mK, with a saturation towards
mK. Unexpectedly, the split lines begin to further separate away
below mK while the line width and shape remain completely
invariable. This crossover behavior is further corroborated by the NMR
relaxation rate measurements. A very strong suppression reflecting
the ordering, , observed above , is replaced by
below . These original NMR features are indicative of
unconventional nature of the crossover, which may arise from a unique
arrangement of the ladders into a spatially anisotropic and frustrated coupling
network.Comment: 5 pages, 3 figure
Field Induced Staggered Magnetization and Magnetic Ordering in
We present a D NMR investigation of the gapped spin-1/2 compound . Our measurements reveal the presence of a magnetic
field induced transverse staggered magnetization (TSM) which persists well
below and above the field-induced 3D long-range magnetically ordered (FIMO)
phase. The symmetry of this TSM is different from that of the TSM induced by
the order parameter of the FIMO phase. Its origin, field dependence and
symmetry can be explained by an intra-dimer Dzyaloshinskii-Moriya interaction,
as shown by DMRG calculations on a spin-1/2 ladder. This leads us to predict
that the transition into the FIMO phase is not in the BEC universality class.Comment: 4 page
Perturbation Theory on the Transition Temperature and Electronic Properties of Organic Superconductor
We study the superconducting transition temperature and the electronic
properties of the metallic phase of -type (BEDT-TTF)X which shows
unconventional properties in experiments, on the basis of the third order
perturbation theory for a simple effective Hubbard model of a nearly triangular
lattice. Appropriate transition temperatures and symmetry of the
gap function are obtained in good agreement with experimental results. We also
calculate the transition temperature by the fluctuation-exchange
approximation(FLEX) in order to compare the two approaches; FLEX gives higher
transition temperatures rather than the perturbation approach. However, it is
also found that the vertex corrections, which are ignored in FLEX, have a
crucial effect on for strongly frustrated systems. The density of
states and the normal self-energy calculated in this perturbation scheme show
the nature of the conventional Fermi liquid near the Mott-insulator. Thus, our
perturbation approach is applicable to the conventional metallic phase of this
compound, while it cannot explain the (pseudo-)spin gap phenomenon which
signals the non-Fermi liquid
Incipient charge order observed by NMR in the normal state of YBa2Cu3Oy
The pseudogap regime of high-temperature cuprates harbours diverse
manifestations of electronic ordering whose exact nature and universality
remain debated. Here, we show that the short-ranged charge order recently
reported in the normal state of YBa2Cu3Oy corresponds to a truly static
modulation of the charge density. We also show that this modulation impacts on
most electronic properties, that it appears jointly with intra-unit-cell
nematic, but not magnetic, order, and that it exhibits differences with the
charge density wave observed at lower temperatures in high magnetic fields.
These observations prove mostly universal, they place new constraints on the
origin of the charge density wave and they reveal that the charge modulation is
pinned by native defects. Similarities with results in layered metals such as
NbSe2, in which defects nucleate halos of incipient charge density wave at
temperatures above the ordering transition, raise the possibility that
order-parameter fluctuations, but no static order, would be observed in the
normal state of most cuprates if disorder were absent.Comment: Updated version. Free download at Nature Comm. website (doi below
Evidence of Andreev bound states as a hallmark of the FFLO phase in -(BEDT-TTF)Cu(NCS)
Superconductivity is a quantum phenomena arising, in its simplest form, from
pairing of fermions with opposite spin into a state with zero net momentum.
Whether superconductivity can occur in fermionic systems with unequal number of
two species distinguished by spin, atomic hyperfine states, flavor, presents an
important open question in condensed matter, cold atoms, and quantum
chromodynamics, physics. In the former case the imbalance between spin-up and
spin-down electrons forming the Cooper pairs is indyced by the magnetic field.
Nearly fifty years ago Fulde, Ferrell, Larkin and Ovchinnikov (FFLO) proposed
that such imbalanced system can lead to exotic superconductivity in which pairs
acquire finite momentum. The finite pair momentum leads to spatially
inhomogeneous state consisting of of a periodic alternation of "normal" and
"superconducting" regions. Here, we report nuclear magnetic resonance (NMR)
measurements providing microscopic evidence for the existence of this new
superconducting state through the observation of spin-polarized quasiparticles
forming so-called Andreev bound states.Comment: 6 pages, 5 fig
Antiferromagnetic Spin Fluctuations in the Metallic Phase of Quasi-Two-Dimensional Organic Superconductors
We give a quantitative analysis of the previously published nuclear magnetic
resonance (NMR) experiments in the k-(ET)2X family of organic charge transfer
salts by using the phenomenological spin fluctuation model of Moriya, and
Millis, Monien and Pines (M-MMP). For temperatures above T_nmr ~ 50 K, the
model gives a good quantitative description of the data in the metallic phases
of several k-(ET)2X materials. These materials display antiferromagnetic
correlation lengths which increase with decreasing temperature and grow to
several lattice constants by T_nmr. It is shown that the fact that the
dimensionless Korringa ratio is much larger than unity is inconsistent with a
broad class of theoretical models (such as dynamical mean-field theory) which
neglects spatial correlations and/or vertex corrections. For materials close to
the Mott insulating phase the nuclear spin relaxation rate, the Knight shift
and the Korringa ratio all decrease significantly with decreasing temperature
below T_nmr. This cannot be described by the M-MMP model and the most natural
explanation is that a pseudogap, similar to that observed in the underdoped
cuprate superconductors, opens up in the density of states below T_nmr. Such a
pseudogap has recently been predicted to occur in the dimerised organic charge
transfer salts materials by the resonating valence bond (RVB) theory. We
propose specific new experiments on organic superconductors to elucidate these
issues. For example, measurements to see if high magnetic fields or high
pressures can be used to close the pseudogap would be extremely valuable.Comment: 11 pages, 2 figures. Accepted for publication in Phys. Rev.
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