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Al-Substitution Effects on Physical Properties of the Colossal Magnetoresistance Compouns La0.67ca0.33mno3
We present a detailed study of the polycrystalline perovskite manganites
La0.67Ca0.33AlxMn1-xO3 (x = 0, 0.1, 0.15, 0.5) at low temperatures and high
magnetic fields, including electrical resistance, magnetization, ac
susceptibility. The static magnetic susceptibility was also measured up to 1000
K. All the samples show colossal magnetoresistance behavior and the Curie
temperatures decrease with Al doping. The data suggest the presence of
correlated magnetic clusters near by the ferromagnetic transition. This appears
to be a consequence of the structural and magnetic disorder created by the
random distribution of Al atoms.Comment: 13 pages including 5 figure
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