69,494 research outputs found
An {\it ab initio} study of the magnetic and electronic properties of Fe, Co, and Ni nanowires on Cu(001) surface
Magnetism at the nanoscale has been a very active research area in the past
decades, because of its novel fundamental physics and exciting potential
applications. We have recently performed an {\it ab intio} study of the
structural, electronic and magnetic properties of all 3 transition metal
(TM) freestanding atomic chains and found that Fe and Ni nanowires have a giant
magnetic anisotropy energy (MAE), indicating that these nanowires would have
applications in high density magnetic data storages. In this paper, we perform
density functional calculations for the Fe, Co and Ni linear atomic chains on
Cu(001) surface within the generalized gradient approximation, in order to
investigate how the substrates would affect the magnetic properties of the
nanowires. We find that Fe, Co and Ni linear chains on Cu(001) surface still
have a stable or metastable ferromagnetic state. When spin-orbit coupling (SOC)
is included, the spin magnetic moments remain almost unchanged, due to the
weakness of SOC in 3 TM chains, whilst significant orbital magnetic moments
appear and also are direction-dependent. Finally, we find that the MAE for Fe,
and Co remains large, i.e., being not much affected by the presence of Cu
substrate.Comment: 4 pages, 2 figure
Magnetic moment and magnetic anisotropy of linear and zigzag 4{\it d} and 5{\it d} transition metal nanowires: First-principles calculations
An extensive {\it ab initio} study of the physical properties of both linear
and zigzag atomic chains of all 4 and 5 transition metals (TM) within the
GGA by using the accurate PAW method, has been carried out. All the TM linear
chains are found to be unstable against the corresponding zigzag structures.
All the TM chains, except Nb, Ag and La, have a stable (or metastable) magnetic
state in either the linear or zigzag or both structures. Magnetic states appear
also in the sufficiently stretched Nb and La linear chains and in the largely
compressed Y and La chains. The spin magnetic moments in the Mo, Tc, Ru, Rh, W,
Re chains could be large (1.0 /atom). Structural transformation
from the linear to zigzag chains could suppress the magnetism already in the
linear chain, induce the magnetism in the zigzag structure, and also cause a
change of the magnetic state (ferromagnetic to antiferroamgetic or vice verse).
The calculations including the spin-orbit coupling reveal that the orbital
moments in the Zr, Tc, Ru, Rh, Pd, Hf, Ta, W, Re, Os, Ir and Pt chains could be
rather large (0.1 /atom). Importantly, large magnetic anisotropy
energy (1.0 meV/atom) is found in most of the magnetic TM chains,
suggesting that these nanowires could have fascinating applications in
ultrahigh density magnetic memories and hard disks. In particular, giant
magnetic anisotropy energy (10.0 meV/atom) could appear in the Ru, Re,
Rh, and Ir chains. Furthermore, the magnetic anisotropy energy in several
elongated linear chains could be as large as 40.0 meV/atom. A
spin-reorientation transition occurs in the Ru, Ir, Ta, Zr, La and Zr, Ru, La,
Ta and Ir linear chains when they are elongated. Remarkably, all the 5 as
well as Tc and Pd chains show the colossal magnetic anisotropy (i.e., it is
impossible to rotate magnetization into certain directions). Finally, the
electronic band structure and density of states of the nanowires have also been
calculated in order to understand the electronic origin of the large magnetic
anisotropy and orbital magnetic moment as well as to estimate the conduction
electron spin polarization.Comment: To appear in Phys. Rev.
Systematic {\it ab initio} study of the magnetic and electronic properties of all 3d transition metal linear and zigzag nanowires
It is found that all the zigzag chains except the nonmagnetic (NM) Ni and
antiferromagnetic (AF) Fe chains which form a twisted two-legger ladder, look
like a corner-sharing triangle ribbon, and have a lower total energy than the
corresponding linear chains. All the 3d transition metals in both linear and
zigzag structures have a stable or metastable ferromagnetic (FM) state. The
electronic spin-polarization at the Fermi level in the FM Sc, V, Mn, Fe, Co and
Ni linear chains is close to 90% or above. In the zigzag structure, the AF
state is more stable than the FM state only in the Cr chain. It is found that
the shape anisotropy energy may be comparable to the electronic one and always
prefers the axial magnetization in both the linear and zigzag structures. In
the zigzag chains, there is also a pronounced shape anisotropy in the plane
perpendicular to the chain axis. Remarkably, the axial magnetic anisotropy in
the FM Ni linear chain is gigantic, being ~12 meV/atom. Interestingly, there is
a spin-reorientation transition in the FM Fe and Co linear chains when the
chains are compressed or elongated. Large orbital magnetic moment is found in
the FM Fe, Co and Ni linear chains
Plasmon assisted transmission of high dimensional orbital angular momentum entangled state
We present an experimental evidence that high dimensional orbital angular
momentum entanglement of a pair of photons can be survived after a
photon-plasmon-photon conversion. The information of spatial modes can be
coherently transmitted by surface plasmons. This experiment primarily studies
the high dimensional entangled systems based on surface plasmon with
subwavelength structures. It maybe useful in the investigation of spatial mode
properties of surface plasmon assisted transmission through subwavelength hole
arrays.Comment: 7 pages,6 figure
Projection Measurement of the Maximally Entangled N-Photon State for a Demonstration of N-Photon de Broglie Wavelength
We construct a projection measurement process for the maximally entangled
N-photon state (the NOON-state) with only linear optical elements and
photodetectors. This measurement process will give null result for any N-photon
state that is orthogonal to the NOON state. We examine the projection process
in more detail for N=4 by applying it to a four-photon state from type-II
parametric down-conversion. This demonstrates an orthogonal projection
measurement with a null result. This null result corresponds to a dip in a
generalized Hong-Ou-Mandel interferometer for four photons. We find that the
depth of the dip in this arrangement can be used to distinguish a genuine
entangled four-photon state from two separate pairs of photons. We next apply
the NOON state projection measurement to a four-photon superposition state from
two perpendicularly oriented type-I parametric down-conversion processes. A
successful NOON state projection is demonstrated with the appearance of the
four-photon de Broglie wavelength in the interference fringe pattern.Comment: 8 pages, 3 figures, new title, some content change, replaced Fig.
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