1,338 research outputs found
Single crystal growth and anisotropy of CeRuPO
We report on the single crystal growth of the ferromagnetic Kondo lattice
system CeRuPO using a Sn flux method. Magnetic susceptibility and electrical
resistivity measurements indicate strong anisotropy of this structurally
layered compound. They evidence that the magnetic moments order
ferromagnetically along the c-direction of the tetragonal unit cell, whereas
the crystal electric field (CEF) anisotropy favors the ab-plane. Therefore,
CeRuPO presents the unusual case within rare earth systems, where the
anisotropy of the interionic exchange interaction overcomes the single ion
anisotropy due to the CEF interaction.Comment: 13 pages, 7 figures, high quality figures:
http://www.cpfs.mpg.de/~krellner
Magnetic field dependence of the antiferromagnetic phase transitions in Co-doped YbRh_2Si_2
We present first specific-heat data of the alloy Yb(Rh_(1-x)Co_x)_2Si_2 at
intermediate Co-contents x=0.18, 0.27, and 0.68. The results already point to a
complex magnetic phase diagram as a function of composition. Co-doping of
YbRh_2Si_2 (T_N^{x=0}=72 mK) stabilizes the magnetic phase due to the volume
decrease of the crystallographic unit cell. The magnetic phase transitions are
clearly visible as pronounced anomalies in C^{4f}(T)/T and can be suppressed by
applying a magnetic field. Going from x=0.18 to x=0.27 we observe a change from
two mean-field (MF) like magnetic transitions at T_N^{0.18}=1.1 K and
T_L^{0.18}=0.65 K to one sharp \lambda-type transition at T_N^{0.27}=1.3 K.
Preliminary measurements under magnetic field do not confirm the field-induced
first-order transition suggested in the literature. For x=0.68 we find two
transitions at T_N^{0.68}=1.14 K and T_L^{0.68}=1.06 K.Comment: Accepted for the ICM proceedings 200
Magnetization study on the field-induced quantum critical point in YbRh_2Si_2
We study the field-induced quantum critical point (QCP) in YbRhSi by
low-temperature magnetization, , and magnetic Gr\"uneisen ratio,
, measurements and compare the results with previous thermal
expansion, , and critical Gr\"uneisen ratio, , data
on YbRh(SiGe). In the latter case, a slightly
negative chemical pressure has been used to tune the system towards its
zero-field QCP. The magnetization derivative is far more singular than
thermal expansion, reflecting a strongly temperature dependent pressure
derivative of the field at constant entropy,
(: molar volume), which saturates at T/GPa for .
The line , previously observed in Hall- and thermodynamic
measurements, separates regimes in - phase space of stronger
) and weaker ) divergent .Comment: 4 Pages, 3 Figures, submitted to Proceedings of ICM 2009 (Karlsruhe
Electron Spin Resonance of the Yb 4f moment in Yb(Rh1-xCox)2Si2
[published in Phys. Rev. B 85, 035119 (2012)] The evolution of spin dynamics
from the quantum critical system YbRh2Si2 to the stable trivalent Yb system
YbCo2Si2 was investigated by Electron Spin Resonance (ESR) spectroscopy. While
the Kondo temperature changes by one order of magnitude, all compositions of
the single crystalline series Yb(Rh1-xCox)2Si2 show well defined ESR spectra
with a clear Yb3+ character for temperatures below \approx 20 K. With
increasing Co-content the ESR g-factor along the c-direction strongly increases
indicating a continuous change of the ground state wave function and, thus, a
continuous change of the crystal electric field. The linewidth presents a
complex dependence on the Co-content and is discussed in terms of the Co-doping
dependence of the Kondo interaction, the magnetic anisotropy and the influence
of ferromagnetic correlations between the 4f states. The results provide
evidence that, for low Co-doping, the Kondo interaction allows narrow ESR
spectra despite the presence of a large magnetic anisotropy, whereas at high
Co-concentrations, the linewidth is controlled by ferromagnetic correlations. A
pronounced broadening due to critical correlations at low temperatures is only
observed at the highest Co-content. This might be related to the presence of
incommensurate magnetic fluctuations.Comment: 8 pages, 8 Figure
Itinerant and local-moment magnetism in EuCr2As2 single crystals
We report on the crystal structure, physical properties, and electronic
structure calculations for the ternary pnictide compound EuCr2As2. X-ray
diffraction studies confirmed that EuCr2As2 crystalizes in the ThCr2Si2-type
tetragonal structure (space group I4/mmm). The Eu ions are in a stable divalent
state in this compound. Eu moments in EuCr2As2 order magnetically below Tm = 21
K. A sharp increase in the magnetic susceptibility below Tm and the positive
value of the paramagnetic Curie temperature obtained from the Curie-Weiss fit
suggest dominant ferromagnetic interactions. The heat capacity exhibits a sharp
{\lambda}-shape anomaly at Tm, confirming the bulk nature of the magnetic
transition. The extracted magnetic entropy at the magnetic transition
temperature is consistent with the theoretical value Rln(2S+1) for S = 7/2 of
the Eu2+ ion. The temperature dependence of the electrical resistivity
\r{ho}(T) shows metallic behavior along with an anomaly at 21 K. In addition,
we observe a reasonably large negative magneto-resistance (~ -24%) at lower
temperature. Electronic structure calculations for EuCr2As2 reveal a moderately
high density of states of Cr-3d orbitals at the Fermi energy, indicating that
the nonmagnetic state of Cr is unstable against magnetic order. Our density
functional calculations for EuCr2As2 predict a G-type AFM order in the Cr
sublattice. The electronic structure calculations suggest a weak interlayer
coupling of the Eu moments.Comment: 9 pages, 7 figure
Temperature - pressure phase diagram of CeCoSi: Pressure induced high-temperature phase
We have studied the temperature-pressure phase diagram of CeCoSi by
electrical-resistivity experiments under pressure. Our measurements revealed a
very unusual phase diagram. While at low pressures no dramatic changes and only
a slight shift of the Ne\'{e}l temperature ( K) are observed,
at about 1.45 GPa a sharp and large anomaly, indicative of the opening of a
spin-density-wave (SDW) gap, appears at a comparatively high temperature K. With further increasing pressure shifts rapidly to low
temperatures and disappears at about 2.15 GPa, likely continuously in a quantum
critical point, but without evidence for superconductivity. Even more
surprisingly, we observed a clear shift of to higher temperatures upon
applying a magnetic field. We discuss two possible origins for , either
magnetic ordering of Co or a meta-orbital type of transition of Ce.Comment: 6 pages, 5 figure
Structural and magnetic transition in CeFeAsO: separated or connected?
Using an adapted Sn-flux growth technique we obtained comparatively large
CeFeAsO single crystals of better quality than previously reported polycrystals
or single crystals, as evidenced by much sharper anomalies at the structural
and magnetic phase transitions as well as a much higher residual resistivity
ratio of 12. In the magnetically ordered phase we observe a very pronounced
metallic behavior of the in-plane resistivity, which excludes a Mott insulator
regime at low temperature. The separation Delta_T = T_0 - T_N between
structural and magnetic ordering temperatures decreases with increasing sample
quality, from 18 K in the initial reports to 6 K in the present single
crystals, demonstrating that this separation is not an intrinsic property of
the RFeAsO systems. Our results indicate that the coupling between magnetic
ordering and structural distortion is very similar in AFe2As2 and RFeAsO type
of compounds, much more similar than previously thought. The implications of
our experimental results give arguments both in favor and against the nematic
phase model.Comment: published in PRB with the title 'Coupling between the structural and
magnetic transition in CeFeAsO
Ferromagnetic quantum critical fluctuations in YbRh_2(Si_{0.95}Ge_{0.05})_2
The bulk magnetic susceptibility of
YbRh(SiGe) has been investigated %by ac-and
dc-magnetometry at low temperatures and close to the field-induced quantum
critical point at T. For T a Curie-Weiss law with a
negative Weiss temperature is observed at temperatures below 0.3 K. Outside
this region, the susceptibility indicates ferromagnetic quantum critical
fluctuations: above 0.3 K, while at low temperatures
the Pauli susceptibility follows and scales with
the coefficient of the term in the electrical resistivity. The
Sommerfeld-Wilson ratio is highly enhanced and increases up to 30 close to the
critical field.Comment: Physical Review Letters, to be publishe
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