417 research outputs found
Superparamagnetic-like ac susceptibility behavior in a "partially disordered antiferromagnetic" compound, CaCoRhO
We report the results of dc and ac magnetization measurements as a function
of temperature (1.8 - 300 K) for the spin chain compound, CaCoRhO,
which has been recently reported to exhibit a partially disordered
antiferromagnetic (PDAF) structure in the range 30 - 90 K and spin-glass
freezing below 30 K. We observe an unexpectedly large frequency dependence of
ac susceptibility in the T range 30 - 90 K, typical of superparamagnets. In
addition, we find that there is no difference in the isothermal remanent
magnetization behavior for the two regimes below 90 K. These findings call for
more investigations to understand the magnetism of this compound.Comment: 4 pages, 3 figure
An Accurate Determination of the Exchange Constant in Sr_2CuO_3 from Recent Theoretical Results
Data from susceptibility measurements on Sr_2CuO_3 are compared with recent
theoretical predictions for the magnetic susceptibility of the
antiferromagnetic spin-1/2 Heisenberg chain. The experimental data fully
confirms the theoretical predictions and in turn we establish that Sr_2CuO_3
behaves almost perfectly like a one-dimensional antiferromagnet with an
exchange coupling of J = 1700^{+150}_{-100}K.Comment: revised and reformatted paper with new title to appear in Phys. Rev B
(Feb.1996). 3 pages (revtex) with 3 embedded figures (macro included). A
complete postscript file is available from
http://fy.chalmers.se/~eggert/expsusc.ps or by request from
[email protected]
Susceptibility of the Spin 1/2 Heisenberg Antiferromagnetic Chain
Highly accurate results are presented for the susceptibility, of
the Heisenberg antiferromagnetic chain for all temperatures, using the
Bethe ansatz and field theory methods. After going through a rounded peak,
approaches its asympotic zero-temperature value with infinite slope.Comment: 8 pages and 3 postscript figures appended (uuencoded), Revtex, Report
#:UBCTP-94-00
On the ground state energy scaling in quasi-rung-dimerized spin ladders
On the basis of periodic boundary conditions we study perturbatively a large
N asymptotics (N is the number of rungs) for the ground state energy density
and gas parameter of a spin ladder with slightly destroyed rung-dimerization.
Exactly rung-dimerized spin ladder is treated as the reference model. Explicit
perturbative formulas are obtained for three special classes of spin ladders.Comment: 4 page
CuSiO_3 : a quasi - one - dimensional S=1/2 antiferromagnetic chain system
CuSiO_3, isotypic to the spin - Peierls compound CuGeO_3, was discovered
recently as a metastable decomposition product of the silicate mineral
dioptase, Cu_6Si_6O_{18}\cdot6H_2O. We investigated the physical properties of
CuSiO_3 using susceptibility, magnetization and specific heat measurements on
powder samples. The magnetic susceptibility \chi(T) is reproduced very well
above T = 8 K by theoretical calculations for an S=1/2 antiferromagnetic
Heisenberg linear chain without frustration (\alpha = 0) and a nearest -
neighbor exchange coupling constant of J/k_{B} = 21 K, much weaker than in
CuGeO_3. Below 8 K the susceptibility exhibits a substantial drop. This feature
is identified as a second - order phase transition at T_{0} = 7.9 K by specific
heat measurements. The influence of magnetic fields on T_{0} is weak, and ac -
magnetization measurements give strong evidence for a spin - flop - phase at
\mu_0H_{SF} ~ 3 T. The origin of the magnetic phase transition at T_{0} = 7.9 K
is discussed in the context of long - range antiferromagnetic order (AF) versus
spin - Peierls(SP)order. Susceptibility and specific heat results support the
AF ordered ground state. Additional temperature dependent ^{63,65}Cu nuclear
quadrupole resonance experiments have been carried out to probe the Cu^{2+}
electronic state and the spin dynamics in CuSiO_3
Coexistence of double alternating antiferromagnetic chains in (VO)_2P_2O_7 : NMR study
Nuclear magnetic resonance (NMR) of 31P and 51V nuclei has been measured in a
spin-1/2 alternating-chain compound (VO)_2P_2O_7. By analyzing the temperature
variation of the 31P NMR spectra, we have found that (VO)_2P_2O_7 has two
independent spin components with different spin-gap energies. The spin gaps are
determined from the temperature dependence of the shifts at 31P and 51V sites
to be 35 K and 68 K, which are in excellent agreement with those observed in
the recent inelastic neutron scattering experiments [A.W. Garrett et al., Phys.
Rev. Lett. 79, 745 (1997)]. This suggests that (VO)_2P_2O_7 is composed of two
magnetic subsystems showing distinct magnetic excitations, which are associated
with the two crystallographically-inequivalent V chains running along the b
axis. The difference of the spin-gap energies between the chains is attributed
to the small differences in the V-V distances, which may result in the
different exchange alternation in each magnetic chain. The exchange
interactions in each alternating chain are estimated and are discussed based on
the empirical relation between the exchange interaction and the interatomic
distance.Comment: 10 pages, 11 embedded eps figures, REVTeX, Submitted to Phys. Rev.
Threshold temperature for pairwise and many-particle thermal entanglement in the isotropic Heisenberg model
We study the threshold temperature for pairwise thermal entanglement in the
spin-1/2 isotropic Heisenberg model up to 11 spins and find that the threshold
temperature for odd and even number of qubits approaches the thermal dynamical
limit from below and above, respectively. The threshold temperature in the
thermodynamical limit is estimated. We investigate the many-particle
entanglement in both ground states and thermal states of the system, and find
that the thermal state in the four-qubit model is four-particle entangled
before a threshold temperature.Comment: 4 pages with 1 fig. More discussions on many-particle ground-state
and thermal entanglement in the multiqubit Heisenberg model from 2 to 11
qubits are adde
Investigation of thermal and magnetic properties of defects in a spin-gap compound NaV2O5
The specific heat, magnetic susceptibility and ESR signals of a Na-deficient
vanadate Na_xV_2O_5 (x=1.00 - 0.90) were studied in the temperature range 0.07
- 10 K, well below the transition point to a spin-gap state. The contribution
of defects provided by sodium vacancies to the specific heat was observed. It
has a low temperature part which does not tend to zero till at least 0.3 K and
a high temperature power-like tail appears above 2 K. Such dependence may
correspond to the existence of local modes and correlations between defects in
V-O layers. The magnetic measurements and ESR data reveal S=1/2 degrees of
freedom for the defects, with their effective number increasing in temperature
and under magnetic field. The latter results in the nonsaturating magnetization
at low temperature. No long-range magnetic ordering in the system of defects
was found. A model for the defects based on electron jumps near vacancies is
proposed to explain the observed effects. The concept of a frustrated
two-dimensional correlated magnet induced by the defects is considered to be
responsible for the absence of magnetic ordering.Comment: 6 pages, 8 figure
Semiclassical approach to the thermodynamics of spin chains
Using the PQSCHA semiclassical method, we evaluate thermodynamic quantities
of one-dimensional Heisenberg ferro- and antiferromagnets. Since the PQSCHA
reduces their evaluation to classical-like calculations, we take advantage of
Fisher's exact solution to get all results in an almost fully analytical way.
Explicitly considered here are the specific heat, the correlations length and
susceptibility. Good agreement with Monte Carlo simulations is found for S>1
antiferromagnets, showing that the relevance of the topological terms and of
the Haldane gap is significant only for the lowest spin values and
temperatures.Comment: 4 pages, 7 figure
Thermodynamic Properties of the One-Dimensional Extended Quantum Compass Model in the Presence of a Transverse Field
The presence of a quantum critical point can significantly affect the
thermodynamic properties of a material at finite temperatures. This is
reflected, e.g., in the entropy landscape S(T; c) in the vicinity of a quantum
critical point, yielding particularly strong variations for varying the tuning
parameter c such as magnetic field. In this work we have studied the
thermodynamic properties of the quantum compass model in the presence of a
transverse field. The specific heat, entropy and cooling rate under an
adiabatic demagnetization process have been calculated. During an adiabatic
(de)magnetization process temperature drops in the vicinity of a field-induced
zero-temperature quantum phase transitions. However close to field-induced
quantum phase transitions we observe a large magnetocaloric effect
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