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Structural features that optimize high temperature superconductivity
For example, various defects can be introduced into the blocking layer to provide the optimum carrier concentration, but defects that form in or adjacent to the CuO{sub 2} layers will lower T{sub c} and eventually destroy superconductivity. After these requirements are satisfied, the highest T{sub c}`s are observed for compounds (such as the HgBa{sub 2}Ca{sub n-1}CuO{sub 2n{plus}2{plus}x} family) that have flat and square CuO{sub 2} planes and long apical Cu-O bonds. This conclusion is confirmed by the study of materials in which the flatness of the CuO{sub 2} plane can be varied in a systematic way. In more recent work, attention has focused on how the structure can be modified, for example, by chemical substitution, to improve flux pinning properties. Two strategies are being investigated: (1) Increasing the coupling of pancake vortices to form vortex-lines by shortening or ``metallizing`` the blocking layer; and (2) the formation of defects that pin flux
Spin and orbital ordering in double-layered manganites
We study theoretically the phase diagram of the double-layered perovskite
manganites taking into account the orbital degeneracy, the strong Coulombic
repulsion, and the coupling with the lattice deformation. Observed spin
structural changes as the increased doping are explained in terms of the
orbital ordering and the bond-length dependence of the hopping integral along
-axis. Temperature dependence of the neutron diffraction peak corresponding
to the canting structure is also explained. Comparison with the 3D cubic system
is made.Comment: 7 figure
Magnetic field induced effects on the electric polarization in RMnO3 R Dy,Gd
X-ray resonant magnetic scattering studies of rare earth magnetic ordering
were performed on perovskite manganites RMnO3 (R = Dy, Gd) in an applied
magnetic field. The data reveal that the field-induced three-fold polarization
enhancement for H || a (H approx. 20 kOe) observed in DyMnO3 below 6.5 K is due
to a re-emergence of the Mn-induced Dy spin order with propagation vector k(Dy)
= k(Mn) = 0.385 b*, which accompanies the suppression of the independent Dy
magnetic ordering, k(Dy) = 1/2 b*. For GdMnO3, the Mn-induced ordering of Gd
spins is used to track the Mn-ordering propagation vector. The data confirm the
incommensurate ordering reported previously, with k(Mn) varying from 0.245 to
0.16 b* on cooling from T_N(Mn) down to a transition temperature T'. New
superstructure reflections which appear below T' suggest a propagation vector
k(Mn) = 1/4 b* in zero magnetic field, which may coexist with the previously
reported A-type ordering of Mn. The Gd spins order with the same propagation
vector below 7 K. Within the ordered state of Gd at T = 1.8 K we find a phase
boundary for an applied magnetic field H || b, H = 10 kOe, which coincides with
the previously reported transition between the ground state paraelectric and
the ferroelectric phase of GdMnO3. Our results suggest that the magnetic
ordering of Gd in magnetic field may stabilize a cycloidal ordering of Mn that,
in turn, produces ferroelectricity.Comment: 8 Figures, v2: improved figure layou
Quasiparticlelike peaks, kinks, and electron phonon coupling at the pi,0 regions in the CMR oxide La2 2xSr1 2xMn2O7
Using Angle Resolved Photoemission ARPES , we present the first observation of sharp quasiparticle like peaks in a CMR manganite. We focus on the pi,0 regions of k space and study their electronic scattering rates and dispersion kinks, uncovering the critical energy scales, momentum scales, and strengths of the interactions that renormalize the electrons. To identify these bosons we measured phonon dispersions in the energy range of the kink by inelastic neutron scattering INS , finding a good match in both energy and momentum to the oxygen bond stretching phonon
The Structure of Nanoscale Polaron Correlations in La1.2Sr1.8Mn2O7
A system of strongly-interacting electron-lattice polarons can exhibit charge
and orbital order at sufficiently high polaron concentrations. In this study,
the structure of short-range polaron correlations in the layered colossal
magnetoresistive perovskite manganite, La1.2Sr1.8Mn2O7, has been determined by
a crystallographic analysis of broad satellite maxima observed in diffuse X-ray
and neutron scattering data. The resulting q=(0.3,0,1) modulation is a
longitudinal octahedral-stretch mode, consistent with an incommensurate
Jahn-Teller-coupled charge-density-wave fluctuations, that implies an unusual
orbital-stripe pattern parallel to the directions.Comment: Reformatted with RevTe
Soft X-ray resonant scattering study of single-crystal LaSrMnO
Soft X-ray resonant scattering studies at the Mn - and
the La - edges of single-crystal LaSrMnO are
reported. At low temperatures, below K, energy scans
with a fixed momentum transfer at the \emph{A}-type antiferromagnetic (0 0 1)
reflection around the Mn -edges with incident linear
and polarizations show strong resonant enhancements. The
splitting of the energy spectra around the Mn -edges may
indicate the presence of a mixed valence state, e.g., Mn/Mn. The
relative intensities of the resonance and the clear shoulder-feature as well as
the strong incident and polarization dependences strongly
indicate its complex electronic origin. Unexpected enhancement of the charge
Bragg (0 0 2) reflection at the La -edges with
polarization has been observed up to 300 K, with an anomaly appearing around
the orbital-ordering transition temperature, K,
suggesting a strong coupling (competition) between them.Comment: Accepted by European Physical Journal
Competition of charge, orbital, and ferromagnetic correlations in layered manganites
The competition of charge, orbital, and ferromagnetic interactions in layered
manganites is investigated by magneto-Raman scattering spectroscopy. We find
that the colossal magnetoresistance effect in the layered compounds results
from the interplay of the orbital and ferromagnetic double-exchange
correlations. Inelastic scattering by charge-order fluctuations dominates the
quasiparticle dynamics in the ferromagnetic-metal state. The scattering is
suppressed at low frequencies, consistent with the opening of a charge-density
wave pseudogap.Comment: 10 pages, 4 figure
Temperature-dependent Raman spectroscopy in BaRuO systems
We investigated the temperature-dependence of the Raman spectra of a
nine-layer BaRuO single crystal and a four-layer BaRuO epitaxial film,
which show pseudogap formations in their metallic states. From the polarized
and depolarized spectra, the observed phonon modes are assigned properly
according to the predictions of group theory analysis. In both compounds, with
decreasing temperature, while modes show a strong hardening, (or
) modes experience a softening or no significant shift. Their different
temperature-dependent behaviors could be related to a direct Ru metal-bonding
through the face-sharing of RuO. It is also observed that another
mode of the oxygen participating in the face-sharing becomes split at low
temperatures in the four layer BaRuO. And, the temperature-dependence of
the Raman continua between 250 600 cm is strongly correlated to
the square of the plasma frequency. Our observations imply that there should be
a structural instability in the face-shared structure, which could be closely
related to the pseudogap formation of BaRuO systems.Comment: 8 pages, 6 figures. to be published in Phys. Rev.
Coherent X-ray Scattering from Manganite Charge and Orbital Domains
We report coherent x-ray scattering studies of charge and orbital domains in
manganite systems. The experiments were carried out on LaMnO_3 and
Pr_{0.6}Ca_{0.4}MnO_3, with the incident photon energy tuned near the Mn K
edge. At room temperature, the orbital speckle pattern of LaMnO_3 was observed
to be constant over a timescale of at least minutes, which is indicative of
static orbital domains on this timescale. For Pr_{0.6}Ca_{0.4}MnO_3, both
charge and orbital speckle patterns were observed. The observation of the
latter rules out the presence of fast orbital fluctuations, while long time
series data-- on the order of several minutes-- were suggestive of slow dynamic
behavior. In contrast, the charge order speckle patterns were static.Comment: 6 pages, 4 figure
Average Lattice Symmetry and Nanoscale Structural Correlations in Magnetoresistive Manganites
We report x-ray scattering studies of nanoscale structural correlations in
the paramagnetic phases of the perovskite manganites
La(CaSr)MnO,
LaSrMnO, and NdSrMnO. We find
that these correlations are present in the orthorhombic phase in
La(CaSr)MnO, but they disappear
abruptly at the orthorhombic-to-rhombohedral transition in this compound. The
orthorhombic phase exhibits increased electrical resistivity and reduced
ferromagnetic coupling, in agreement with the association of the nanoscale
correlations with insulating regions. In contrast, the correlations were not
detected in the two other compounds, which exhibit rhombohedral and tetragonal
phases. Based on these results, as well as on previously published work, we
propose that the local structure of the paramagnetic phase correlates strongly
with the average lattice symmetry, and that the nanoscale correlations are an
important factor distinguishing the insulating and the metallic phases in these
compounds.Comment: a note on recent experimental work, and a new reference adde
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