64 research outputs found
Magnetic field induced effects on the electric polarization in RMnO3 R Dy,Gd
X-ray resonant magnetic scattering studies of rare earth magnetic ordering
were performed on perovskite manganites RMnO3 (R = Dy, Gd) in an applied
magnetic field. The data reveal that the field-induced three-fold polarization
enhancement for H || a (H approx. 20 kOe) observed in DyMnO3 below 6.5 K is due
to a re-emergence of the Mn-induced Dy spin order with propagation vector k(Dy)
= k(Mn) = 0.385 b*, which accompanies the suppression of the independent Dy
magnetic ordering, k(Dy) = 1/2 b*. For GdMnO3, the Mn-induced ordering of Gd
spins is used to track the Mn-ordering propagation vector. The data confirm the
incommensurate ordering reported previously, with k(Mn) varying from 0.245 to
0.16 b* on cooling from T_N(Mn) down to a transition temperature T'. New
superstructure reflections which appear below T' suggest a propagation vector
k(Mn) = 1/4 b* in zero magnetic field, which may coexist with the previously
reported A-type ordering of Mn. The Gd spins order with the same propagation
vector below 7 K. Within the ordered state of Gd at T = 1.8 K we find a phase
boundary for an applied magnetic field H || b, H = 10 kOe, which coincides with
the previously reported transition between the ground state paraelectric and
the ferroelectric phase of GdMnO3. Our results suggest that the magnetic
ordering of Gd in magnetic field may stabilize a cycloidal ordering of Mn that,
in turn, produces ferroelectricity.Comment: 8 Figures, v2: improved figure layou
The Structure of Nanoscale Polaron Correlations in La1.2Sr1.8Mn2O7
A system of strongly-interacting electron-lattice polarons can exhibit charge
and orbital order at sufficiently high polaron concentrations. In this study,
the structure of short-range polaron correlations in the layered colossal
magnetoresistive perovskite manganite, La1.2Sr1.8Mn2O7, has been determined by
a crystallographic analysis of broad satellite maxima observed in diffuse X-ray
and neutron scattering data. The resulting q=(0.3,0,1) modulation is a
longitudinal octahedral-stretch mode, consistent with an incommensurate
Jahn-Teller-coupled charge-density-wave fluctuations, that implies an unusual
orbital-stripe pattern parallel to the directions.Comment: Reformatted with RevTe
Soft X-ray resonant scattering study of single-crystal LaSrMnO
Soft X-ray resonant scattering studies at the Mn - and
the La - edges of single-crystal LaSrMnO are
reported. At low temperatures, below K, energy scans
with a fixed momentum transfer at the \emph{A}-type antiferromagnetic (0 0 1)
reflection around the Mn -edges with incident linear
and polarizations show strong resonant enhancements. The
splitting of the energy spectra around the Mn -edges may
indicate the presence of a mixed valence state, e.g., Mn/Mn. The
relative intensities of the resonance and the clear shoulder-feature as well as
the strong incident and polarization dependences strongly
indicate its complex electronic origin. Unexpected enhancement of the charge
Bragg (0 0 2) reflection at the La -edges with
polarization has been observed up to 300 K, with an anomaly appearing around
the orbital-ordering transition temperature, K,
suggesting a strong coupling (competition) between them.Comment: Accepted by European Physical Journal
Temperature-dependent Raman spectroscopy in BaRuO systems
We investigated the temperature-dependence of the Raman spectra of a
nine-layer BaRuO single crystal and a four-layer BaRuO epitaxial film,
which show pseudogap formations in their metallic states. From the polarized
and depolarized spectra, the observed phonon modes are assigned properly
according to the predictions of group theory analysis. In both compounds, with
decreasing temperature, while modes show a strong hardening, (or
) modes experience a softening or no significant shift. Their different
temperature-dependent behaviors could be related to a direct Ru metal-bonding
through the face-sharing of RuO. It is also observed that another
mode of the oxygen participating in the face-sharing becomes split at low
temperatures in the four layer BaRuO. And, the temperature-dependence of
the Raman continua between 250 600 cm is strongly correlated to
the square of the plasma frequency. Our observations imply that there should be
a structural instability in the face-shared structure, which could be closely
related to the pseudogap formation of BaRuO systems.Comment: 8 pages, 6 figures. to be published in Phys. Rev.
Average Lattice Symmetry and Nanoscale Structural Correlations in Magnetoresistive Manganites
We report x-ray scattering studies of nanoscale structural correlations in
the paramagnetic phases of the perovskite manganites
La(CaSr)MnO,
LaSrMnO, and NdSrMnO. We find
that these correlations are present in the orthorhombic phase in
La(CaSr)MnO, but they disappear
abruptly at the orthorhombic-to-rhombohedral transition in this compound. The
orthorhombic phase exhibits increased electrical resistivity and reduced
ferromagnetic coupling, in agreement with the association of the nanoscale
correlations with insulating regions. In contrast, the correlations were not
detected in the two other compounds, which exhibit rhombohedral and tetragonal
phases. Based on these results, as well as on previously published work, we
propose that the local structure of the paramagnetic phase correlates strongly
with the average lattice symmetry, and that the nanoscale correlations are an
important factor distinguishing the insulating and the metallic phases in these
compounds.Comment: a note on recent experimental work, and a new reference adde
Manganites at Quarter Filling: Role of Jahn-Teller Interactions
We have analyzed different correlation functions in a realistic spin-orbital
model for half-doped manganites. Using a finite-temperature diagonalization
technique the CE phase was found in the charge-ordered phase in the case of
small antiferromagnetic interactions between electrons. It is shown
that a key ingredient responsible for stabilization of the CE-type spin and
orbital-ordered state is the cooperative Jahn-Teller (JT) interaction between
next-nearest Mn neighbors mediated by the breathing mode distortion of
Mn octahedra and displacements of Mn ions. The topological phase
factor in the Mn-Mn hopping leading to gap formation in one-dimensional models
for the CE phase as well as the nearest neighbor JT coupling are not able to
produce the zigzag chains typical for the CE phase in our model.Comment: 16 pages with 16 figures, contains a more detailed parameter estimate
based on the structural data by Radaelli et al. (accepted for publication in
Phys. Rev. B
Dynamical Mean Field Theory for Self-Generated Quantum Glasses
We present a many body approach for non-equilibrium behavior and
self-generated glassiness in strongly correlated quantum systems. It combines
the dynamical mean field theory of equilibrium systems with the replica theory
for classical glasses without quenched disorder. We apply this approach to
study a quantized version of the Brazovskii model and find a self-generated
quantum glass that remains in a quantum mechanically mixed state as T -> 0.
This quantum glass is formed by a large number of competing states spread over
an energy region which is determined within our theory.Comment: 10 pages, 4 figure
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