Unified model of hyperthermia via hysteresis heating in systems of interacting magnetic nanoparticles

We present a general study of frequency and magnetic field dependence of the specific heat power produced during field-driven hysteresis cycles in magnetic nanoparticles with relevance to hyperthermia applications in biomedicine. Employing a kinetic Monte-Carlo method with natural time scales allows us to go beyond the assumptions of small driving field amplitudes and negligible inter-particle interactions, which are fundamental to applicability of the standard approach based on linear response theory. The method captures the superparamagnetic and fully hysteretic regimes and the transition between them. Our results reveal unexpected dipolar interaction-induced enhancement or suppression of the specific heat power, dependent on the intrinsic statistical properties of particles, which cannot be accounted for by the standard theory. Although the actual heating power is difficult to predict because of the effects of interactions, optimum heating is in the transition region between the superparamagnetic and fully hysteretic regimes

Effect of damping on the time variation of fields produced by a small pole tip with a soft under layer

The time variation of magnetostatic fields generated by space and time varying magnetization configurations in small perpendicular pole tips is studied. The magnetization configurations are a response to external fields driving the pole tip and soft under layer (SUL). When the system damping is sufficiently small the magnetization excitations persist for a long time after reversal. The effects of damping parameter, position in the media, and discretization cell size on the magnitude of the time varying magnetostatic fields will be given. Decreasing the damping parameter increases the magnitude of the magnetostatic field variation

Modeling of long-time thermal magnetization decay in interacting granular magnetic materials

We present a general method to evaluate the long-time magnetization decay in granular magnetic systems. The method is based on Arrhenius-Neel kinetics with the evaluation of the energy barriers in a multidimensional space. To establish a possible reversal mode, we suggest the use of Metropolis Monte Carlo and for the mode statistical sampling-the kinetic Monte Carlo criteria. The examples considered include long-time magnetization decay in CoCrPt low-magnetization longitudinal recording media and in a collection of Co particles with different concentrations

Implementation of the "hyperdynamics of infrequent events" method for acceleration of thermal switching dynamics of magnetic moments

For acceleration of the calculations of thermal magnetic switching, we report the use of the Voter method, recently proposed in chemical physics (also called "hyperdynamics of the infrequent events"). The method consists of modification of the magnetic potential so that the transition state remains unchanged. We have found that the method correctly describes the mean first passage time even in the case of small damping (precessional case) and for an oblique angle between the anisotropy and the field directions. Due to the costly evaluation of the lowest energy eigenvalue, the actual acceleration depends on its fast computation. In the current implementation, it is limited to intermediate time scale and to small system size

Theory of rotational processes in perpendicular media and application to anisotropy measurement

Numerical and analytical calculations of rotational process in perpendicular recording media are presented. The work supports recent experimental studies that suggest that the measurement of rotational magnetization processes can be used to determine the value of the anisotropy constant. An expression for the rotational magnetization for a noninteracting system is derived taking into account the dispersion of K and the easy-axis orientation. The calculations show that the experiments determine the mean value of H-K, essentially independent of the angular dispersion. A numerical (Monte-Carlo based) micromagnetic model is used to study the effects of magnetostatic and exchange interactions at nonzero temperatures. It is shown that for small values of KV/kT, irreversible magnetization processes take place, which precludes the use of the rotational magnetization method to determine K values. This effect is enhanced by the presence of the magnetostatic interaction. However, the presence of exchange interactions is found to enforce coherent rotation in small fields, reducing the irreversible processes and allowing the determination of H-K. Under these circumstances, it is shown that the exchange does not significantly affect the value of HK, and that a well-defined demagnetization correction of 4piM is appropriate. Finally, a comparison with experimental data gives good agreement for multilayer and granular media and shows the role of domain formation on the rotational magnetization process

Parametric optimization for terabit perpendicular recording

The design of media for ultrahigh-density perpendicular recording is discussed in depth. Analytical and semianalytical models are developed to determine the constraints upon the media to fulfill requirements of writability and thermal stability, and the effect of intergranular exchange coupling is examined. The role of vector fields during the write process is examined, and it is shown that one-dimensional models of perpendicular recording have significant deficiencies. A micromagnetic model is described and the results of simulations of recording undertaken with the model are presented. The paper demonstrates that there is no physical reason why perpendicular recording should not be possible at or above 1 Tb/in(2)