Comparative study of ordered and disordered Y1-xSrxCoO3-d

We have succeeded in preparing A-site ordered- and disordered-Y1/4Sr3/4CoO3-d with various oxygen deficiencies delta, and have made comparative study of their structural and physical properties. In the A-site ordered structure, oxygen vacancies order, and d = 0.34 sample shows a weak ferromagnetic transition beyond 300 K. On the other hand, in the A-site disordered structure, no oxygen vacancy ordering is observed, and d = 0.16 sample shows a ferromagnetic metallic transition around 150 K. A-site disordering destroys the orderings of oxygen-vacancies and orbitals, leading to the strong modification of the electronic phases.Comment: 3 pages, 3 figures, proceeding of 52nd Mangetism and Magnetic Materials Conference (MMM 2007), published in Journal of Applied Physic

Reduction of critical field for magnetic and orbital-ordering phase transition in impurity-substituted Nd0.45_{0.45}Sr0.55_{0.55}MnO3_3 crystal

We have investigated the Mn-site substitution effect in Nd$_{0.45}$Sr$_{0.55}$MnO$_3$ single crystal, which has an $A$-type layered antiferromagnetic ($A$-AFM) phase with the 3$d_{x^2-y^2}$-type orbital-order. Substitution of Fe or Ga for Mn-site suppresses both the $A$-AFM order and competing ferromagnetic (FM) correlation whereas Cr substitution suppresses only the $A$-AFM order but reactivates the underlying FM correlation via double-exchange mechanism along the AFM coupled $c$-direction. In Nd$_{0.45}$Sr$_{0.55}$Mn$_{0.95}$Cr$_{0.05}$O$_3$, the $A$-AFM state with the orbital-order is changed into the orbital-disordered three-dimensional FM metallic state by applying magnetic field of $\mu_0 H = 12$ T, which is much smaller than that of the parent compound Nd$_{0.45}$Sr$_{0.55}$MnO$_3$.Comment: 5 pages, 4 figures, to appear in APL Material

Cr-doping effect on the orbital fluctuation of heavily doped Nd1-xSrxMnO3 (x ~ 0.625)

We have investigated the Cr-doping effect of Nd0.375Sr0.625MnO3 near the phase boundary between the x2-y2 and 3z2-r2 orbital ordered states, where a ferromagnetic correlation and concomitant large magnetoresistance are observed owing to orbital fluctuation. Cr-doping steeply suppresses the ferromagnetic correlation and magnetoresistance in Nd0.375Sr0.625Mn1-yCryO3 with 0 < y < 0.05, while they reappear in 0.05 < y < 0.10. Such a reentrant behavior implies that a phase boundary is located at y = 0.05, or a phase crossover occurs across y = 0.05.Comment: 3 pages, 3 figures, to be published in Journal of Applied Physic

A New Technique For the Histochemical Demonstration of Phosphatase in Hard Tissue

この論文は国立情報学研究所の学術雑誌公開支援事業により電子化されました。A new histochemical technique for the demonstration of alkaline phosphatase in hard tissues was described. This method is characterized by the following three points. First, a neutral mixture solution of tetra- and disodium salt of ethylen diamin tetraacetic acid is adopted as a suitable decalcifying solution for histochemical use. Secondly, neutral formol solution is applied as a reducing reagent for silver phosphate which is produced by histochemical procedure instead of other Kossa's method. Last of all metallic silver which yielded a reaction product is replaced in metallic gold by immersing in a gold chloride solution. By this method, the procedure became easier and excellent figures were obtainable

Entropy-Driven Reentrant Behavior in CMR Manganites

We discuss the origin of the reentrant behaviors of insulating states above the Curie temperature of the colossal magnetoresistance manganites. We consider a system where charge ordering and ferromagnetism compete with each other. In the presence of randomness which pins charge order fluctuations, entropy-driven reentrant behaviors will appear, which explains the typical temperature dependence of the resistivity for CMR manganites.Comment: 2 pages, 1 figure, submitted to SCES'0

Magnetoelectric Properties of (Ca1−x_{1-x}Srx_{x})2_2CoSi2_2O7_7 Crystals

We have investigated the magnetoelectric properties of (Ca$_{1-x}$Sr$_{x}$)$_2$CoSi$_2$O$_7$ ($0\leq x\leq 1$) crystals with a quasi-two-dimensional structure. In Ca$_2$CoSi$_2$O$_7$ ($x=0$), a canted antiferromagnetic transition occurs at 5.6 K. The transition temperature $T_{\rm N}$ is increasing with increasing Sr concentration, and the rises of the magnetization and dielectric constant become larger. Since the dielectric constant shows large change at $T_{\rm N}$ and the magnetocapacitance effect is observed below $T_{\rm N}$, a coupling between the magnetism and dielectricity is strong in (Ca$_{1-x}$Sr$_{x}$)$_2$CoSi$_2$O$_7$. The positive magnetocapacitance is reduced by Sr substitution, and is not observed in $x\geq 0.5$. Namely, the compound of $x\geq 0.5$ does not show the magnetic-field-induced electric polarization. On the other hand, the negative magnetocapacitance is enhanced by Sr substitution.Comment: 4 pages, 2figures, proceeding of International Conference on Magnetism 200

I=2I=2 ππ\pi\pi potential in the HAL QCD method with all-to-all propagators

In this paper, we perform the first application of the hybrid method (exact low modes plus stochastically estimated high modes) for all-to-all propagators to the HAL QCD method. We calculate the HAL QCD potentials in the $I=2$ $\pi\pi$ scattering in order to see how statistical fluctuations of the potential behave under the hybrid method. All of the calculations are performed with the 2+1 flavor gauge configurations on $16^3 \times 32$ lattice at the lattice spacing $a \approx 0.12$ fm and $m_{\pi} \approx 870$ MeV. It is revealed that statistical errors for the potential are enhanced by stochastic noises introduced by the hybrid method, which, however, are shown to be reduced by increasing the level of dilutions, in particular, that of space dilutions. From systematic studies, we obtain a guiding principle for a choice of dilution types/levels and a number of eigenvectors to reduce noise contaminations to the potential while keeping numerical costs reasonable. We also confirm that we can obtain the scattering phase shifts for the $I=2$ $\pi\pi$ system by the hybrid method within a reasonable numerical cost, which are consistent with the result obtained with the conventional method. The knowledge we obtain in this study will become useful to investigate hadron resonances which require quark annihilation diagrams such as the $\rho$ meson by the HAL QCD potential with the hybrid method.Comment: 20 pages, 10 figures, published version in PTE

Electron- and Hole-Doping Effects on AA-site Ordered NdBaMn2_2O6_6

We have investigated electron- and hole-doping effects on $A$-site ordered perovskite manganite NdBaMn$_2$O$_6$, which has the $A$-type (layered) antiferromagnetic (AFM) ground state. Electrons (holes) are introduced by partial substitution of Ba$^{2+}$ (Nd$^{3+}$) with Nd$^{3+}$ (Ba$^{2+}$). Electron-doping generates ferromagnetic (FM) clusters in the $A$-type AFM matrix. With increasing the electron-doping level, the volume fraction of the FM phase or the number of the FM clusters is abruptly increasing. In contrast, the $A$-type AFM phase is robust against the hole-doping, and no FM correlation is observed in the hole-doped NdBaMn$_2$O$_6$.Comment: 8 pages, 5 figures, to be published in Journal of the Physical Society of Japa