Impedance-matched cavity quantum memory

We consider an atomic frequency comb based quantum memory inside an asymmetric optical cavity. In this configuration it is possible to absorb the input light completely in a system with an effective optical depth of one, provided that the absorption per cavity round trip exactly matches the transmission of the coupling mirror ("impedance matching"). We show that the impedance matching results in a readout efficiency only limited by irreversible atomic dephasing, whose effect can be made very small in systems with large inhomogeneous broadening. Our proposal opens up an attractive route towards quantum memories with close to unit efficiency.Comment: 4 pages, 2 figure

Temporally multiplexed quantum repeaters with atomic gases

We propose a temporally multiplexed version of the Duan-Lukin-Cirac-Zoller (DLCZ) quantum repeater protocol using controlled inhomogeneous spin broadening in atomic gases. A first analysis suggests that the advantage of multiplexing is negated by noise due to spin wave excitations corresponding to unobserved directions of Stokes photon emission. However, this problem can be overcome with the help of a moderate-finesse cavity which is in resonance with Stokes photons, but invisible to the anti-Stokes photons. Our proposal promises greatly enhanced quantum repeater performance with atomic gases.Comment: 5 pages, 1 figur

Spectral noise in quantum frequency down-conversion from the visible to the telecommunication C-band

We report a detailed study of the noise properties of a visible-to-telecom photon frequency converter based on difference frequency generation (DFG). The device converts 580 nm photons to 1541 nm using a strong pump laser at 930 nm, in a periodically poled lithium niobate ridge waveguide. The converter reaches a maximum device efficiency of 46 % (internal efficiency of 67 %) at a pump power of 250 mW. The noise produced by the pump laser is investigated in detail by recording the noise spectra both in the telecom and visible regimes, and measuring the power dependence of the noise rates. The noise spectrum in the telecom is very broadband, as expected from previous work on similar DFG converters. However, we also observe several narrow dips in the telecom spectrum, with corresponding peaks appearing in the 580 nm noise spectrum. These features are explained by sum frequency generation of the telecom noise at wavelengths given by the phase matching condition of different spatial modes in the waveguide. The proposed noise model is in good agreement with all the measured data, including the power-dependence of the noise rates, both in the visible and telecom regime. These results are applicable to the class of DFG converters where the pump laser wavelength is in between the input and target wavelength.Comment: 10 page

Multi-mode and long-lived quantum correlations between photons and spins in a crystal

The realization of quantum networks and quantum repeaters remains an outstanding challenge in quantum communication. These rely on entanglement of remote matter systems, which in turn requires creation of quantum correlations between a single photon and a matter system. A practical way to establish such correlations is via spontaneous Raman scattering in atomic ensembles, known as the DLCZ scheme. However, time multiplexing is inherently difficult using this method, which leads to low communication rates even in theory. Moreover, it is desirable to find solid-state ensembles where such matter-photon correlations could be generated. Here we demonstrate quantum correlations between a single photon and a spin excitation in up to 12 temporal modes, in a $^{151}$Eu$^{3+}$ doped Y$_2$SiO$_5$ crystal, using a novel DLCZ approach that is inherently multimode. After a storage time of 1 ms, the spin excitation is converted into a second photon. The quantum correlation of the generated photon pair is verified by violating a Cauchy - Schwarz inequality. Our results show that solid-state rare-earth crystals could be used to generate remote multi-mode entanglement, an important resource for future quantum networks

Single-photon-level optical storage in a solid-state spin-wave memory

A long-lived quantum memory is a firm requirement for implementing a quantum repeater scheme. Recent progress in solid-state rare-earth-ion-doped systems justifies their status as very strong candidates for such systems. Nonetheless an optical memory based on spin-wave storage at the single-photon-level has not been shown in such a system to date, which is crucial for achieving the long storage times required for quantum repeaters. In this letter we show that it is possible to execute a complete atomic frequency comb (AFC) scheme, including spin-wave storage, with weak coherent pulses of $\bar{n} = 2.5 \pm 0.6$ photons per pulse. We discuss in detail the experimental steps required to obtain this result and demonstrate the coherence of a stored time-bin pulse. We show a noise level of $(7.1 \pm 2.3)10^{-3}$ photons per mode during storage, this relatively low-noise level paves the way for future quantum optics experiments using spin-waves in rare-earth-doped crystals

Mapping multiple photonic qubits into and out of one solid-state atomic ensemble

The future challenge of quantum communication are scalable quantum networks, which require coherent and reversible mapping of photonic qubits onto stationary atomic systems (quantum memories). A crucial requirement for realistic networks is the ability to efficiently store multiple qubits in one quantum memory. Here we demonstrate coherent and reversible mapping of 64 optical modes at the single photon level in the time domain onto one solid-state ensemble of rare-earth ions. Our light-matter interface is based on a high-bandwidth (100 MHz) atomic frequency comb, with a pre-determined storage time of 1 microseconds. We can then encode many qubits in short <10 ns temporal modes (time-bin qubits). We show the good coherence of the mapping by simultaneously storing and analyzing multiple time-bin qubits.Comment: 7 pages, 6 figures + Supplementary materia

Analysis of a quantum memory for photons based on controlled reversible inhomogeneous broadening

We present a detailed analysis of a quantum memory for photons based on controlled and reversible inhomogeneous broadening (CRIB). The explicit solution of the equations of motion is obtained in the weak excitation regime, making it possible to gain insight into the dependence of the memory efficiency on the optical depth, and on the width and shape of the atomic spectral distributions. We also study a simplified memory protocol which does not require any optical control fields.Comment: 9 pages, 4 figures (Accepted for publication in Phys. Rev. A

Atomic frequency comb memory with spin wave storage in 153Eu3+:Y2SiO5

153Eu3+:Y2SiO5 is a very attractive candidate for a long lived, multimode quantum memory due to the long spin coherence time (~15 ms), the relatively large hyperfine splitting (100 MHz) and the narrow optical homogeneous linewidth (~100 Hz). Here we show an atomic frequency comb memory with spin wave storage in a promising material 153Eu3+:Y2SiO5, reaching storage times slightly beyond 10 {\mu}s. We analyze the efficiency of the storage process and discuss ways of improving it. We also measure the inhomogeneous spin linewidth of 153Eu3+:Y2SiO5, which we find to be 69 \pm 3 kHz. These results represent a further step towards realising a long lived multi mode solid state quantum memory.Comment: 7 pages and 7 figure

Electric control of collective atomic coherence in an Erbium doped solid

We demonstrate fast and accurate control of the evolution of collective atomic coherences in an Erbium doped solid using external electric fields. This is achieved by controlling the inhomogeneous broadening of Erbium ions emitting at 1536 nm using an electric field gradient and the linear Stark effect. The manipulation of atomic coherence is characterized with the collective spontaneous emission (optical free induction decay) emitted by the sample after an optical excitation, which does not require any previous preparation of the atoms. We show that controlled dephasing and rephasing of the atoms by the electric field result in collapses and revivals of the optical free induction decay. Our results show that the use of external electric fields does not introduce any substantial additional decoherence and enables the manipulation of collective atomic coherence with a very high degree of precision on the time scale of tens of ns. This provides an interesting resource for photonic quantum state storage and quantum state manipulation.Comment: 10 pages, 5 figure