Controlling the phase of a light beam with a single molecule

We employ heterodyne interferometry to investigate the effect of a single organic molecule on the phase of a propagating laser beam. We report on the first phase-contrast images of individual molecules and demonstrate a single-molecule electro-optical phase switch by applying a voltage to the microelectrodes embedded in the sample. Our results may find applications in single-molecule holography, fast optical coherent signal processing, and single-emitter quantum operations

Dynamical heat channels

We consider heat conduction in a 1D dynamical channel. The channel consists of a group of noninteracting particles, which move between two heat baths according to some dynamical process. We show that the essential thermodynamic properties of the heat channel can be evaluated from the diffusion properties of the underlying particles. Emphasis is put on the conduction under anomalous diffusion conditions. \\{\bf PACS number}: 05.40.+j, 05.45.ac, 05.60.cdComment: 4 figure

Survival Probability in a Random Velocity Field

The time dependence of the survival probability, S(t), is determined for diffusing particles in two dimensions which are also driven by a random unidirectional zero-mean velocity field, v_x(y). For a semi-infinite system with unbounded y and x>0, and with particle absorption at x=0, a qualitative argument is presented which indicates that S(t)~t^{-1/4}. This prediction is supported by numerical simulations. A heuristic argument is also given which suggests that the longitudinal probability distribution of the surviving particles has the scaling form P(x,t)~ t^{-1}u^{1/3}g(u). Here the scaling variable u is proportional to x/t^{3/4}, so that the overall time dependence of P(x,t) is proportional to t^{-5/4}, and the scaling function g(u) has the limiting dependences g(u) approaching a constant as u--->0 and g(u)~exp(-u^{4/3}) as u--->infinity. This argument also suggests an effective continuum equation of motion for the infinite system which reproduces the correct asymptotic longitudinal probability distribution.Comment: 6 pages, RevTeX, 5 figures includes, to be submitted to Phys. Rev.

Strong extinction of a laser beam by a single molecule

We present an experiment where a single molecule strongly affects the amplitude and phase of a laser field emerging from a subwavelength aperture. We achieve a visibility of -6% in direct and +10% in cross-polarized detection schemes. Our analysis shows that a close to full extinction should be possible using near-field excitation.Comment: 5 pages, 4 figures, submitted to PR

Anomalous diffusion and dynamical localization in a parabolic map

We study numerically classical and quantum dynamics of a piecewise parabolic area preserving map on a cylinder which emerges from the bounce map of elongated triangular billiards. The classical map exhibits anomalous diffusion. Quantization of the same map results in a system with dynamical localization and pure point spectrum.Comment: 4 pages in RevTeX (4 ps-figures included

Quantum Interference of Tunably Indistinguishable Photons from Remote Organic Molecules

We demonstrate two-photon interference using two remote single molecules as bright solid-state sources of indistinguishable photons. By varying the transition frequency and spectral width of one molecule, we tune and explore the effect of photon distinguishability. We discuss future improvements on the brightness of single-photon beams, their integration by large numbers on chips, and the extension of our experimental scheme to coupling and entanglement of distant molecules

Photon Channelling in Foams

Experiments by Gittings, Bandyopadhyay, and Durian [Europhys. Lett.\ \textbf{65}, 414 (2004)] demonstrate that light possesses a higher probability to propagate in the liquid phase of a foam due to total reflection. The authors term this observation photon channelling which we investigate in this article theoretically. We first derive a central relation in the work of Gitting {\em et al.} without any free parameters. It links the photon's path-length fraction $f$ in the liquid phase to the liquid fraction $\epsilon$. We then construct two-dimensional Voronoi foams, replace the cell edges by channels to represent the liquid films and simulate photon paths according to the laws of ray optics using transmission and reflection coefficients from Fresnel's formulas. In an exact honeycomb foam, the photons show superdiffusive behavior. It becomes diffusive as soon as disorder is introduced into the foams. The dependence of the diffusion constant on channel width and refractive index is explained by a one-dimensional random-walk model. It contains a photon channelling state that is crucial for the understanding of the numerical results. At the end, we shortly comment on the observation that photon channelling only occurs in a finite range of $\epsilon$.Comment: 9 pages, minor change

L\'evy Distribution of Single Molecule Line Shape Cumulants in Low Temperature Glass

We investigate the distribution of single molecule line shape cumulants, $\kappa_1,\kappa_2,...$, in low temperature glasses based on the sudden jump, standard tunneling model. We find that the cumulants are described by L\'evy stable laws, thus generalized central limit theorem is applicable for this problem.Comment: 5 pages, 3 figure

From deterministic dynamics to kinetic phenomena

We investigate a one-dimenisonal Hamiltonian system that describes a system of particles interacting through short-range repulsive potentials. Depending on the particle mean energy, $\epsilon$, the system demonstrates a spectrum of kinetic regimes, characterized by their transport properties ranging from ballistic motion to localized oscillations through anomalous diffusion regimes. We etsablish relationships between the observed kinetic regimes and the "thermodynamic" states of the system. The nature of heat conduction in the proposed model is discussed.Comment: 4 pages, 4 figure