Realization of Rydberg-dressed quantum magnets

Interacting ultracold atomic quantum gases provide an ideal test bed to study strongly correlated quantum matter. The interactions between atoms in such an ultracold quantum gas are typically short-ranged and well described by an effective contact potential. Introducing longer-range interactions promises the realization of novel quantum phases which are absent in systems with only short-range interactions. Trapped atoms, resonantly laser-coupled to highly excited, strongly interacting Rydberg states have been proposed as a versatile platform to realize such long-range interacting quantum matter. In a first experiment presented in this thesis, we combined the single-atom-sensitive local preparation and detection enabled by a quantum gas microscope to prepare and microscopically characterize an ensemble of rubidium-87 atoms trapped in an optical lattice in the regime of strong Rydberg blockade. There, we observe collectively enhanced optical coupling in an effective two-level system, the so-called “superatom”, and infer the presence of entanglement. Detuned optical coupling to Rydberg states, termed “Rydberg dressing”, has been proposed as an alternative approach to induce long-range interactions. Rather than directly exciting an atom to a Rydberg state, the properties of the latter are admixed to a ground state, which consequently acquires long-range interactions. In the context of this thesis, we have designed a laser system in the ultraviolet spectral range to admix Rydberg P-state character to the ground state of atoms in an optical lattice. In an emerging Ising quantum magnet, the presence of Rydberg-dressed interactions was demonstrated by an interferometric technique combined with spatially resolved spin correlation measurements. The theoretically predicted tunability of the isotropy and range of the interaction were confirmed experimentally. While these initial measurements exhibited unexpected dissipation, in a subsequent experiment in a one-dimensional spin chain this dissipation was overcome. We substantiated the improved coherence times by tracking the time evolution of the magnetization upon suddenly switching on interactions and observing coherent collapse and revival dynamics, one of the hallmarks of coherent quantum evolution. Our results establish Rydberg-dressed interactions in ultracold gases and pave the way to realize and study novel exotic quantum phases

Microscopy of a scalable superatom

Strong interactions can amplify quantum effects such that they become important on macroscopic scales. Controlling these coherently on a single particle level is essential for the tailored preparation of strongly correlated quantum systems and opens up new prospects for quantum technologies. Rydberg atoms offer such strong interactions which lead to extreme nonlinearities in laser coupled atomic ensembles. As a result, multiple excitation of a Micrometer sized cloud can be blocked while the light-matter coupling becomes collectively enhanced. The resulting two-level system, often called "superatom", is a valuable resource for quantum information, providing a collective Qubit. Here we report on the preparation of two orders of magnitude scalable superatoms utilizing the large interaction strength provided by Rydberg atoms combined with precise control of an ensemble of ultracold atoms in an optical lattice. The latter is achieved with sub shot noise precision by local manipulation of a two-dimensional Mott insulator. We microscopically confirm the superatom picture by in-situ detection of the Rydberg excitations and observe the characteristic square root scaling of the optical coupling with the number of atoms. Furthermore, we verify the presence of entanglement in the prepared states and demonstrate the coherent manipulation of the superatom. Finally, we investigate the breakdown of the superatom picture when two Rydberg excitations are present in the system, which leads to dephasing and a loss of coherence.Comment: 7 pages, 5 figure

Spatially Resolved Detection of a Spin-Entanglement Wave in a Bose-Hubbard Chain

Entanglement is an essential property of quantum many-body systems. However, its local detection is challenging and was so far limited to spin degrees of freedom in ion chains. Here we measure entanglement between the spins of atoms located on two lattice sites in a one-dimensional Bose-Hubbard chain which features both local spin- and particle-number fluctuations. Starting with an initially localized spin impurity, we observe an outwards propagating entanglement wave and show quantitatively how entanglement in the spin sector rapidly decreases with increasing particle-number fluctuations in the chain.Comment: 6 pages, 4 figure

Coherent many-body spin dynamics in a long-range interacting Ising chain

Coherent many-body quantum dynamics lies at the heart of quantum simulation and quantum computation. Both require coherent evolution in the exponentially large Hilbert space of an interacting many-body system. To date, trapped ions have defined the state of the art in terms of achievable coherence times in interacting spin chains. Here, we establish an alternative platform by reporting on the observation of coherent, fully interaction-driven quantum revivals of the magnetization in Rydberg-dressed Ising spin chains of atoms trapped in an optical lattice. We identify partial many-body revivals at up to about ten times the characteristic time scale set by the interactions. At the same time, single-site-resolved correlation measurements link the magnetization dynamics with inter-spin correlations appearing at different distances during the evolution. These results mark an enabling step towards the implementation of Rydberg atom based quantum annealers, quantum simulations of higher dimensional complex magnetic Hamiltonians, and itinerant long-range interacting quantum matter.Comment: 11 pages, 9 figure

Quantum gas microscopy of Rydberg macrodimers

A microscopic understanding of molecules is essential for many fields of natural sciences but their tiny size hinders direct optical access to their constituents. Rydberg macrodimers - bound states of two highly-excited Rydberg atoms - feature bond lengths easily exceeding optical wavelengths. Here we report on the direct microscopic observation and detailed characterization of such macrodimers in a gas of ultracold atoms in an optical lattice. The size of about 0.7 micrometers, comparable to the size of small bacteria, matches the diagonal distance of the lattice. By exciting pairs in the initial two-dimensional atom array, we resolve more than 50 vibrational resonances. Using our spatially resolved detection, we observe the macrodimers by correlated atom loss and demonstrate control of the molecular alignment by the choice of the vibrational state. Our results allow for precision testing of Rydberg interaction potentials and establish quantum gas microscopy as a powerful new tool for quantum chemistry.Comment: 13 pages, 9 figure

Tracking evaporative cooling of a mesoscopic atomic quantum gas in real time

The fluctuations in thermodynamic and transport properties in many-body systems gain importance as the number of constituent particles is reduced. Ultracold atomic gases provide a clean setting for the study of mesoscopic systems; however, the detection of temporal fluctuations is hindered by the typically destructive detection, precluding repeated precise measurements on the same sample. Here, we overcome this hindrance by utilizing the enhanced light--matter coupling in an optical cavity to perform a minimally invasive continuous measurement and track the time evolution of the atom number in a quasi two-dimensional atomic gas during evaporation from a tilted trapping potential. We demonstrate sufficient measurement precision to detect atom number fluctuations well below the level set by Poissonian statistics. Furthermore, we characterize the non-linearity of the evaporation process and the inherent fluctuations of the transport of atoms out of the trapping volume through two-time correlations of the atom number. Our results establish coupled atom--cavity systems as a novel testbed for observing thermodynamics and transport phenomena in mesosopic cold atomic gases and, generally, pave the way for measuring multi-time correlation functions of ultracold quantum gases.Comment: Significantly extended discussion of Fig. 4. Accepted for publication in Phys. Rev.

A subwavelength atomic array switched by a single Rydberg atom

Enhancing light-matter coupling at the level of single quanta is essential for numerous applications in quantum science. The cooperative optical response of subwavelength atomic arrays was recently found to open new pathways for such strong light-matter couplings, while simultaneously offering access to multiple spatial modes of the light field. Efficient single-mode free-space coupling to such arrays has been reported, but the spatial control over the modes of outgoing light fields has remained elusive. Here we demonstrate such spatial control over the optical response of an atomically thin mirror formed by a subwavelength array of atoms in free space using a single controlled ancilla atom excited to a Rydberg state. The switching behavior is controlled by the admixture of a small Rydberg fraction to the atomic mirror, and consequently strong dipolar Rydberg interactions with the ancilla. Driving Rabi oscillations on the ancilla atom, we demonstrate coherent control of the transmission and reflection of the array. Our results pave the way towards realizing novel quantum coherent metasurfaces, creating controlled atom-photon entanglement and deterministic engineering of quantum states of light.Comment: 8 pages, 5 figures + 9 pages Supplementary Informatio

Observation of brane parity order in programmable optical lattices

The Mott-insulating phase of the two-dimensional (2d) Bose-Hubbard model is expected to be characterized by a non-local brane parity order. Parity order captures the presence of microscopic particle-hole fluctuations and entanglement, whose properties depend on the underlying lattice geometry. We realize 2d Bose-Hubbard models in dynamically tunable lattice geometries, using neutral atoms in a novel passively phase-stable tunable optical lattice in combination with programmable site-blocking potentials. We benchmark the performance of our system by single-particle quantum walks in the square, triangular, kagome and Lieb lattice. In the strongly correlated regime, we microscopically characterize the geometry dependence of the quantum fluctuations and experimentally validate the brane parity as a proxy for the non-local order parameter signaling the superfluid-to-Mott insulating phase transition.Comment: Fixed typos and formattin

Computational Capabilities and Compiler Development for Neutral Atom Quantum Processors: Connecting Tool Developers and Hardware Experts

Neutral Atom Quantum Computing (NAQC) emerges as a promising hardware platform primarily due to its long coherence times and scalability. Additionally, NAQC offers computational advantages encompassing potential long-range connectivity, native multi-qubit gate support, and the ability to physically rearrange qubits with high fidelity. However, for the successful operation of a NAQC processor, one additionally requires new software tools to translate high-level algorithmic descriptions into a hardware executable representation, taking maximal advantage of the hardware capabilities. Realizing new software tools requires a close connection between tool developers and hardware experts to ensure that the corresponding software tools obey the corresponding physical constraints. This work aims to provide a basis to establish this connection by investigating the broad spectrum of capabilities intrinsic to the NAQC platform and its implications on the compilation process. To this end, we first review the physical background of NAQC and derive how it affects the overall compilation process by formulating suitable constraints and figures of merit. We then provide a summary of the compilation process and discuss currently available software tools in this overview. Finally, we present selected case studies and employ the discussed figures of merit to evaluate the different capabilities of NAQC and compare them between two hardware setups.Comment: 32 pages, 13 figures, 2 table