Electronic Raman response in anisotropic metals

Using a generalized response theory we derive the electronic Raman response function for metals with anisotropic relaxation rates. The calculations account for the long--range Coulomb interaction and treat the collision operator within a charge conserving relaxation time approximation. We extend earlier treatments to finite wavenumbers ($|{\bf q}|\ll k_{\rm F}$) and incorporate inelastic electron--electron scattering besides elastic impurity scattering. Moreover we generalize the Lindhard density response function to the Raman case. Numerical results for the quasiparticle scattering rate and the Raman response function for cuprate superconductors are presented.Comment: 5 pages, 4figures. accepted in PRB (Brief Report), in pres

Charge transfer fluctuation, d−d-wave superconductivity, and the B1gB_{1g} Raman phonon in the Cuprates: A detailed analysis

The Raman spectrum of the $B_{1g}$ phonon in the superconducting cuprate materials is investigated theoretically in detail in both the normal and superconducting phases, and is contrasted with that of the $A_{1g}$ phonon. A mechanism involving the charge transfer fluctuation between the two oxygen ions in the CuO$_2$ plane coupled to the crystal field perpendicular to the plane is discussed and the resulting electron-phonon coupling is evaluated. Depending on the symmetry of the phonon the weight of different parts of the Fermi surface in the coupling is different. This provides the opportunity to obtain information on the superconducting gap function at certain parts of the Fermi surface. The lineshape of the phonon is then analyzed in detail both in the normal and superconducting states. The Fano lineshape is calculated in the normal state and the change of the linewidth with temperature below T$_{c}$ is investigated for a $d_{x^{2}-y^{2}}$ pairing symmetry. Excellent agreement is obtained for the $B_{1g}$ phonon lineshape in YBa$_{2}$Cu$_{3}$O$_{7}$. These experiments, however, can not distinguish between $d_{x^{2}-y^{2}}$ and a highly anisotropic $s$-wave pairing.Comment: Revtex, 21 pages + 4 postscript figures appended, tp

Theory of Orbital Kondo Effect with Assisted Hopping in Strongly Correlated Electron Systems: Parquet Equations, Superconductivity and Mass Enhancement

Orbital Kondo effect is treated in a model, where additional to the conduction band there are localized orbitals close to the Fermi energy. If the hopping between the conduction band and the localized heavy orbitals depends on the occupation of the atomic orbitals in the conduction band then orbital Kondo correlation occurs. The noncommutative nature of the coupling required for the Kondo effect is formally due to the form factors associated with the assisted hopping which in the momentum representation depends on the momenta of the conduction electrons involved. The leading logarithmic vertex corrections are due to the local Coulomb interaction between the electrons on the heavy orbital and in the conduction band. The renormalized vertex functions are obtained as a solution of a closed set of differential equations and they show power behavior. The amplitude of large renormalization is determined by an infrared cutoff due to finite energy and dispersion of the heavy particles. The enhanced assisted hopping rate results in mass enhancement and attractive interaction in the conduction band. The superconductivity transition temperature calculated is largest for intermediate mass enhancement, $m^*/m \approx 2-3$. For larger mass enhancement the small one particle weight ($Z$) in the Green's function reduces the transition temperature which may be characteristic for otherComment: 32 pages, RevTeX 3.0, figures on reques

Symmetry dependence of phonon lineshapes in superconductors with anisotropic gaps

The temperature dependence below $T_{c}$ of the lineshape of optical phonons of different symmetry as seen in Raman scattering is investigated for superconductors with anisotropic energy gaps. It is shown that the symmetry of the electron-phonon vertex produces non-trivial couplings to an anisotropic energy gap which leads to unique changes in the phonon lineshape for phonons of different symmetry. The phonon lineshape is calculated in detail for $B_{1g}$ and $A_{1g}$ phonons in a superconductor with $d_{x^{2}-y^{2}}$ pairing symmetry. The role of satellite peaks generated by the electron-phonon coupling are also addressed. The theory accounts for the substantial phonon narrowing of the $B_{1g}$ phonon, while narrowing of the $A_{1g}$ phonon which is indistinguishable from the normal state is shown, in agreement with recent measurements on BSCCO.Comment: 15 pages (3 Figures available upon request), Revtex, 1

Enhanced Electron-Phonon Coupling and its Irrelevance to High Tc_{c} Superconductivity

It is argued that the origin of the buckling of the CuO$_{2}$ planes in certain cuprates as well as the strong electron-phonon coupling of the $B_{1g}$ phonon is due to the electric field across the planes induced by atoms with different valence above and below. The magnitude of the electric field is deduced from new Raman results on YBa$_{2}$Cu$_{3}$O$_{6+x}$ and Bi$_{2}$Sr$_{2}$(Ca$_{1-x}$Y$_{x}$)Cu$_{2}$O$_{8}$ with different O and Y doping, respectively. In the latter case it is shown that the symmetry breaking by replacing Ca partially by Y enhances the coupling by an order of magnitude, while the superconducting $T_c$ drops to about two third of its original value.Comment: 4 pages, 2 figures. This and other papers can be downloaded from http://gwis2.circ.gwu.edu/~tp

Orbital Kondo behavior from dynamical structural defects

The interaction between an atom moving in a model double-well potential and the conduction electrons is treated using renormalization group methods in next-to-leading logarithmic order. A large number of excited states is taken into account and the Kondo temperature $T_K$ is computed as a function of barrier parameters. We find that for special parameters $T_K$ can be close to $1 {\rm K}$ and it can be of the same order of magnitude as the renormalized splitting $\Delta$. However, in the perturbative regime we always find that T_K \alt \Delta with a T_K \alt 1 {\rm K} [Aleiner {\em et al.}, Phys. Rev. Lett. {\bf 86}, 2629 (2001)]. We also find that $\Delta$ remains unrenormalized at energies above the Debye frequency, $\omega_{\rm Debye}$.Comment: 9 pages, 9 figures, RevTe

Instability of the marginal commutative model of tunneling centers interacting with metallic environment: Role of the electron-hole symmetry breaking

The role of the electron-hole symmetry breaking is investigated for a symmetrical commutative two-level system in a metal using the multiplicative renormalization group in a straightforward way. The role of the symmetries of the model and the path integral technique are also discussed in detail. It is shown that the electron-hole symmetry breaking may make the model non-commutative and generate the assisted tunneling process which is, however, too small itself to drive the system into the vicinity of the two-channel Kondo fixed point. While these results are in qualitative agreement with those of Moustakas and Fisher (Phys. Rev. B 51, 6908 (1995), ibid 53, 4300 (1996)) the scaling equations turn out to be essentially different. We show that the main reason for this difference is that the procedure for the elimination of the high energy degrees of freedom used by Moustakas and Fisher leaves only the free energy invariant, however, the couplings generated are not connected to the dynamical properties in a straightforward way and should be interpreted with care. These latter results might have important consequences in other cases where the path integral technique is used to produce the scaling equations and calculate physical quantities.Comment: latex, figures in ps file adde

Kondo Temperature for the Two-Channel Kondo Models of Tunneling Centers

The possibility for a two-channel Kondo ($2CK$) non Fermi liquid state to appear in a metal as a result of the interaction between electrons and movable structural defects is revisited. As usual, the defect is modeled by a heavy particle moving in an almost symmetric double-well potential (DWP). Taking into account only the two lowest states in DWP is known to lead to a Kondo-like Hamiltonian with rather low Kondo temperature, $T_K$. We prove that, in contrast to previous believes, the contribution of higher excited states in DWP does not enhance $T_K$. On the contrary, $T_K$ is reduced by three orders of magnitude as compared with the two-level model: the prefactor in $T_K$ is determined by the spacing between the second and the third levels in DWP rather than by the electron Fermi energy. Moreover, $T_K$, turns out to be parametrically smaller than the splitting between the two lowest levels. Therefore, there is no microscopic model of movable defects which may justify non-Fermi liquid $2CK$ phenomenology.Comment: 5 pages, 4 .eps figure

Physical origin of the buckling in CuO2_2: Electron-phonon coupling and Raman spectra

It is shown theoretically that the buckling of the CuO$_{2}$ planes in certain cuprate systems can be explained in terms of an electric field across the planes which originates from different valences of atoms above and below the plane. This field results also in a strong coupling of the Raman-active out-of-phase vibration of the oxygen atoms ($B_{1g}$ mode) to the electronic charge transfer between the two oxygens in the CuO$_{2}$ plane. Consequently, the electric field can be deduced from the Fano-type line shape of the $B_{1g}$ phonon. Using the electric field estimated from the electron-phonon coupling the amplitude of the buckling is calculated and found to be in good agreement with the structural data. Direct experimental support for the idea proposed is obtained in studies of YBa$_{2}$Cu$_{3}$O$_{6+x}$ and Bi$_{2}$Sr$_{2}$(Ca$_{1-x}$Y$_{x}$)Cu$_{2}$O$_{8}$ with different oxygen and yttrium doping, respectively, including antiferromagnetic samples. In the latter compound, symmetry breaking by replacing Ca partially by Y leads to an enhancement of the electron-phonon coupling by an order of magnitude.Comment: 12 pages, 4 figures, and 1 tabl