Exciton Recombination in One-Dimensional Organic Mott Insulators

We present a theory for the recombination of (charged) holons and doublons in one-dimensional organic Mott insulators, which is responsible for the decay of a photoexcited metallic state. Due to the charge-spin separation, the dominant mechanism for recombination at low density of charges involves a multi-phonon emission. We show that a reasonable coupling to phonons is sufficient to explain the fast recombination observed by pump-probe experiments in ET-F$_2$TCNQ, whereby we can also account for the measured pressure dependence of the recombination rate.Comment: 5 + 3 pages, 2 figure

Iterative construction of conserved quantities in dissipative nearly integrable systems

Integrable systems offer rare examples of solvable many-body problems in the quantum world. Due to the fine-tuned structure, their realization in nature and experiment is never completely accurate, therefore effects of integrability are observed only transiently. One way to surpass that is to couple nearly integrable systems to baths and driving: these will stabilize integrable effects up to arbitrary time, as encoded in the time dependent, and eventually, the stationary state of form of a generalized Gibbs ensemble. However, the description of such driven dissipative nearly integrable models is challenging and no exact analytical methods have been proposed so far. Here we develop an iterative scheme in which integrability breaking perturbations (baths) determine the most necessary conserved quantities to be added into a truncated generalized Gibbs ensemble description. Our scheme significantly reduces the complexity of the problem, paving the way for thermodynamic results.Comment: 10 pages, 5 figures (including Supplemental Material

Holon-Doublon Binding as the Mechanism for the Mott transition

We study the binding of a holon to a doublon in a half-filled Hubbard model as the mechanism of the zero-temperature metal-insulator transition. In a spin polarized system and a non-bipartite lattice a single holon-doublon (HD) pair exhibits a binding transition (e.g., on a face-centred cubic lattice), or a sharp crossover (e.g., on a triangular lattice) corresponding well to the standard Mott transition in unpolarized systems. We extend the HD-pair study towards non-polarized systems by considering more general spin background and by treating the finite HD density within a BCS-type approximation. Both approaches lead to a discontinuous transition away from the fully polarized system and give density correlations consistent with numerical results on a triangular lattice.Comment: 6 pages, 4 figure

Dielectric breakdown in spin polarized Mott insulator

Nonlinear response of a Mott insulator to external electric field, corresponding to dielectric breakdown phenomenon, is studied within of a one-dimensional half-filled Hubbard model. It is shown that in the limit of nearly spin polarized insulator the decay rate of the ground state into excited holon-doublon pairs can be evaluated numerically as well to high accuracy analytically. Results show that the threshold field depends on the charge gap as $F_{th} \propto \Delta^{3/2}$. Numerical results on small systems indicate on the persistence of a similar mechanism for the breakdown for decreasing magnetization down to unpolarised system.Comment: 4 pages, 6 figure

Reconstructing effective Hamiltonians from nonequilibrium (pre-)thermal steady states

Reconstructing Hamiltonians from local measurements is key to enabling reliable quantum simulation: both validating the implemented model, and identifying any left-over terms with sufficient precision is a problem of increasing importance. Here we propose a deep-learning-assisted variational algorithm for Hamiltonian reconstruction by pre-processing a dataset that is diagnosed to contain thermal measurements of local operators. We demonstrate the efficient and precise reconstruction of local Hamiltonians, while long-range interacting Hamiltonians are reconstructed approximately. Away from equilibrium, for periodically and random multipolar driven systems, we reconstruct the effective Hamiltonian widely used for Floquet engineering of metastable steady states. Moreover, our approach allows us to reconstruct an effective quasilocal Hamiltonian even in the heating regime beyond the validity of the prethermal plateau, where perturbative expansions fail.Comment: 13 pages, 5 figure