Quantum correlations and violation of Bell inequality induced by External Field in a two photon radiative cascade

We study the polarization dependent second order correlation of a pair of photons emitted in a four level radiative cascade driven by an external field. It is found that the quantum correlations of the emitted photons, degraded by the energy splitting of the intermediate levels in the radiative cascade can be efficiently revived by a far detuned external field. The physics of this revival is linked to an induced stark shift and the formation of dressed states in the system by the non-resonant external field. Further, we investigated the competition between the effect of the coherent external field and incoherent dephasing of the intermediate levels. We found that the degradation of quantum correlations due to the incoherent dephasing can be content for small dephasing with the external field. We also studied the non-locality of the correlations by evaluating the Bell's inequality in the linear polarization basis for the radiative cascade. We find that the Bell parameter decreases rapidly with increase in the intermediate level energy splitting or incoherent dephasing rate to the extent that there is no violation. However, the presence of an external field leads to control over the degrading mechanisms and preservation of nonlocal correlation among the photons. This in turn can induce, violation of Bell's inequality in the radiative cascade for arbitrary intermediate level splitting and small incoherent dephasing

Synthetic gauge potential and effective magnetic field in a Raman medium undergoing molecular modulation

We theoretically demonstrate non-trivial topological effects for a probe field in a Raman medium undergoing molecular modulation processes. The medium is driven by two non-collinear pump beams. We show that the angle between the pumps is related to an effective gauge potential and an effective magnetic field for the probe field in the synthetic space consisting of a synthetic frequency dimension and a spatial dimension. As a result of such effective magnetic field, the probe field can exhibit topologically-protected one-way edge state in the synthetic space, as well as Landau levels which manifests as suppression of both diffraction and sideband generation. Our work identifies a previously unexplored route towards creating topological photonics effects, and highlights an important connection between topological photonics and nonlinear optics

Quantum Coherence and Superradiant Emission: From Lasing Without Inversion to Sky Laser and the QASER

This work is focused on quantum coherence and superradiant emission in a dense pencil-like multi-level medium where many novel effects appear such as transient lasing without inversion, coherence-brightened sky laser, and quantum amplification by superradiant emission of radiation. We start from an interesting cascade model where quantum coherence effects can lead to surprising phenomena, gain without population inversion and gain suppression, under different parameters. We further show superradiant emission inside helium plasma. The population evolution shows the decay is significantly faster than collisional decoherence and spontaneous decay rates. This indicates superradiant coherent behavior of the atomic system inside the plasma. Based on these results, we demonstrate lasing without inversion on a time scale shorter than the decoherence time. The possibility of transient lasing without inversion holds promise for lasing in the extreme-ultraviolet/x-ray regime. We propose experiments to demonstrate this in helium or helium-like ions plasma. We also study coherent emission from ambient air and demonstrate efficient generation of laser-like beams directed both forward and backward with respect to a nanosecond ultraviolet pumping laser beam. The emission process exhibits nonadiabatic quantum coherence, which is similar in nature to Dicke superradiance. This coherence-brightened backward light source in air provides possibility for atmospheric remote sensing through a phase-matched coherent Raman scattering process. Finally, we present a new kind of quantum amplifier, the QASER (quantum amplification by superradiant emission of radiation), based on collective superradiant emission which does not require initial population in the excited state. We show that parametric resonance between the driving field and collective superradiant oscillations of the atomic polarization can yield light amplification at high frequencies. The resulting superradiant amplifier is many orders of magnitude more efficient than nonlinear multiphoton excitation and holds promise as a new way to generate high-frequency coherent radiation