3,021 research outputs found
Spin Dynamics of Double-Exchange Manganites with Magnetic Frustration
This work examines the effects of magnetic frustration due to competing
ferromagnetic and antiferromagnetic Heisenberg interactions on the spin
dynamics of the double-exchange model. When the local moments are non-colinear,
a charge-density wave forms because the electrons prefer to sit on lines of
sites that are coupled ferromagnetically. With increasing hopping energy, the
local spins become aligned and the average spin-wave stiffness increases. Phase
separation is found only within a narrow range of hopping energies. Results of
this work are applied to the field-induced jump in the spin-wave stiffness
observed in the manganite PrCaMnO with .Comment: 10 pages, 3 figure
Spin Dynamics of a Canted Antiferromagnet in a Magnetic Field
The spin dynamics of a canted antiferromagnet with a quadratic spin-wave
dispersion near \vq =0 is shown to possess a unique signature. When the
anisotropy gap is negligible, the spin-wave stiffness \dsw (\vq, B) =
(\omega_{\vq}-B)/q^2 depends on whether the limit of zero field or zero
wavevector is taken first. Consequently, \dsw is a strong function of
magnetic field at a fixed wavevector. Even in the presence of a sizeable
anisotropy gap, the field dependence of both \dsw and the gap energy
distinguishes a canted antiferromagnet from a phase-separated mixture
containing both ferromagnetic and antiferromagnetic regions.Comment: 10 pages, 3 figure
Ferromagnetic insulating phase in Pr{1-x}Ca{x}MnO3
A ferromagnetic insulating (FM-I) state in Pr0.75Ca0.25MnO3 has been studied
by neutron scattering experiment and theoretical calculation. The insulating
behavior is robust against an external magnetic field, and is ascribed to
neither the phase separation between a ferromagnetic metallic (FM-M) phase and
a non-ferromagnetic insulating one, nor the charge ordering. We found that the
Jahn-Teller type lattice distortion is much weaker than PrMnO3 and the magnetic
interaction is almost isotropic. These features resembles the ferromagnetic
metallic state of manganites, but the spin exchange interaction J is much
reduced compared to the FM-M state. The theoretical calculation based on the
staggered type orbital order well reproduces several features of the spin and
orbital state in the FM-I phase.Comment: REVTeX4, 10 pages, 9 figure
Ordering Process and Its Hole Concentration Dependence of the Stripe Order in La{2-x}Sr{x}NiO{4}
Ordering process of stripe order in La{2-x}Sr{x}NiO{4} with x being around
1/3 was investigated by neutron diffraction experiments. When the stripe order
is formed at high temperature, incommensurability \epsilon of the stripe order
has a tendency to show the value close to 1/3 for the samples with x at both
sides of 1/3. With decreasing temperature, however, \epsilon becomes close to
the value determined by the linear relation of \epsilon = n_h, where n_h is a
hole concentration. This variation of the \epsilon strongly affects the
character of the stripe order through the change of the carrier densities in
stripes and antiferromagnetic domains.Comment: 5 pages, 3 figures, REVTeX, to be published in Phys. Rev.
Double Exchange in a Magnetically Frustrated System
This work examines the magnetic order and spin dynamics of a double-exchange
model with competing ferromagnetic and antiferromagnetic Heisenberg
interactions between the local moments. The Heisenberg interactions are
periodically arranged in a Villain configuration in two dimensions with
nearest-neighbor, ferromagnetic coupling and antiferromagnetic coupling
. This model is solved at zero temperature by performing a
expansion in the rotated reference frame of each local moment.
When exceeds a critical value, the ground state is a magnetically
frustrated, canted antiferromagnet. With increasing hopping energy or
magnetic field , the local moments become aligned and the ferromagnetic
phase is stabilized above critical values of or . In the canted phase, a
charge-density wave forms because the electrons prefer to sit on lines of sites
that are coupled ferromagnetically. Due to a change in the topology of the
Fermi surface from closed to open, phase separation occurs in a narrow range of
parameters in the canted phase. In zero field, the long-wavelength spin waves
are isotropic in the region of phase separation. Whereas the average spin-wave
stiffness in the canted phase increases with or , it exhibits a more
complicated dependence on field. This work strongly suggests that the jump in
the spin-wave stiffness observed in PrCaMnO with at a field of 3 T is caused by the delocalization of the electrons rather
than by the alignment of the antiferromagnetic regions.Comment: 28 pages, 12 figure
Commensurate-Incommensurate transition in the melting process of the orbital ordering in Pr0.5Ca0.5MnO3: neutron diffraction study
The melting process of the orbital order in
Pr0.5Ca0.5MnO3 single crystal has been studied in detail as a function of
temperature by neutron diffraction. It is demonstrated that a
commensurate-incommensurate (C-IC) transition of the orbital ordering takes
place in a bulk sample, being consistent with the electron diffraction studies.
The lattice structure and the transport properties go through drastic changes
in the IC orbital ordering phase below the charge/orbital ordering temperature
Tco/oo, indicating that the anomalies are intimately related to the partial
disordering of the orbital order, unlike the consensus that it is related to
the charge disordering process. For the same T range, partial disorder of the
orbital ordering turns on the ferromagnetic spin fluctuations which were
observed in a previous neutron scattering study.Comment: 5 pages, 2 figures, REVTeX, to be published in Phys. Rev.
Charge and spin ordering in Nd{1/3}Sr{2/3}FeO{3}
We have investigated the charge and spin ordering in Nd{1/3}Sr{2/3}FeO{3}
with neutron diffraction technique. This sample undergoes a charge ordering
transition accompanying charge disproportionation of 2Fe4+ -> Fe3+ + Fe5+. We
measured the superlattice reflections due to the charge and spin ordering, and
confirmed that charges and spins order simultaneously at Tco = 185 K. The
ordering pattern of charges and spins in this sample can be viewed as three
dimensional stripe order, and is compared with two dimensional stripe order
observed in other transition metal oxides.Comment: REVTeX, 4 pages, 3 figures, to be published in J. Phys. Chem. Solid
Anomalous ferromagnetic spin fluctuations in an antiferromagnetic insulator Pr_{1-x}Ca_{x}MnO_{3}
The high temperature paramagnetic state in an antiferromagnetic (AFM)
insulator Pr_{1-x}Ca_{x}MnO_{3} is characterized by the ferromagnetic (FM) spin
fluctuations with an anomalously small energy scale. The FM fluctuations show a
precipitous decrease of the intensity at the charge ordering temperature
T_{CO}, but persist below T_{CO}, and vanish at the AFM transition temperature
T_{N}. These results demonstrate the importance of the spin ordering for the
complete switching of the FM fluctuation in doped manganites.Comment: REVTeX, 5 pages, 4 figures, submitted to Phys. Rev.
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