503 research outputs found
Electronic correlations and Hund's coupling effects in SrMoO revealed by photoemission spectroscopy
We investigate the electronic structure of a perovskite-type Pauli paramagnet
SrMoO3 (t2g2) thin film using hard x-ray photoemission spectroscopy and compare
the results to the realistic calculations that combine the density functional
theory within the local-density approximation (LDA) with the dynamical-mean
field theory (DMFT). Despite the clear signature of electron correlations in
the electronic specific heat, the narrowing of the quasiparticle bands is not
observed in the photoemission spectrum. This is explained in terms of the
characteristic effect of Hund's rule coupling for partially-filled t2g bands,
which induces strong quasiparticle renormalization already for values of
Hubbard interaction which are smaller than the bandwidth. The interpretation is
supported by additional model DMFT calculations including Hund's rule coupling,
that show renormalization of low-energy quasiparticles without affecting the
overall bandwidth. The photoemission spectra show additional spectral weight
around -2 eV that is not present in the LDA+DMFT. We interpret this weight as a
plasmon satellite, which is supported by measured Mo, Sr and Oxygen core-hole
spectra that all show satellites at this energy.Comment: 8 pages, 7 figure
Anisotropic spin-density distribution and magnetic anisotropy of strained LaSrMnO thin films: Angle-dependent x-ray magnetic circular dichroism
Magnetic anisotropies of ferromagnetic thin films are induced by epitaxial
strain from the substrate via strain-induced anisotropy in the orbital magnetic
moment and that in the spatial distribution of spin-polarized electrons.
However, the preferential orbital occupation in ferromagnetic metallic
LaSrMnO (LSMO) thin films studied by x-ray linear dichroism
(XLD) has always been found out-of-plane for both tensile and compressive
epitaxial strain and hence irrespective of the magnetic anisotropy. In order to
resolve this mystery, we directly probed the preferential orbital occupation of
spin-polarized electrons in LSMO thin films under strain by angle-dependent
x-ray magnetic circular dichroism (XMCD). Anisotropy of the spin-density
distribution was found to be in-plane for the tensile strain and out-of-plane
for the compressive strain, consistent with the observed magnetic anisotropy.
The ubiquitous out-of-plane preferential orbital occupation seen by XLD is
attributed to the occupation of both spin-up and spin-down out-of-plane
orbitals in the surface magnetic dead layer.Comment: 20 pages, 4 figure
Uncoupling of neurogenesis and differentiation during retinal development
Conventionally, neuronal development is regarded to follow a stereotypic sequence of neurogenesis, migration, and differentiation. We demonstrate that this notion is not a general principle of neuronal development by documenting the timing of mitosis in relation to multiple differentiation events for bipolar cells (BCs) in the zebrafish retina using in vivo imaging. We found that BC progenitors undergo terminal neurogenic divisions while in markedly disparate stages of neuronal differentiation. Remarkably, the differentiation state of individual BC progenitors at mitosis is not arbitrary but matches the differentiation state of post-mitotic BCs in their surround. By experimentally shifting the relative timing of progenitor division and differentiation, we provide evidence that neurogenesis and differentiation can occur independently of each other. We propose that the uncoupling of neurogenesis and differentiation could provide neurogenic programs with flexibility, while allowing for synchronous neuronal development within a continuously expanding cell pool
Built-in and induced polarization across LaAlO/SrTiO heterojunctions
Ionic crystals terminated at oppositely charged polar surfaces are inherently
unstable and expected to undergo surface reconstructions to maintain
electrostatic stability. Essentially, an electric field that arises between
oppositely charged atomic planes gives rise to a built-in potential that
diverges with thickness. In ultra thin film form however the polar crystals are
expected to remain stable without necessitating surface reconstructions, yet
the built-in potential has eluded observation. Here we present evidence of a
built-in potential across polar \lao ~thin films grown on \sto ~substrates, a
system well known for the electron gas that forms at the interface. By
performing electron tunneling measurements between the electron gas and a
metallic gate on \lao ~we measure a built-in electric field across \lao ~of 93
meV/\AA. Additionally, capacitance measurements reveal the presence of an
induced dipole moment near the interface in \sto, illuminating a unique
property of \sto ~substrates. We forsee use of the ionic built-in potential as
an additional tuning parameter in both existing and novel device architectures,
especially as atomic control of oxide interfaces gains widespread momentum.Comment: 6 pages, 4 figures. Submitted to Nature physics on May 1st, 201
Oikonomia, incarnation and immediacy : the figure of the Jew in St John of Damascus
Selected Figure panel dat
- …