353 research outputs found
High efficiency and low absorption Fresnel compound zone plates for hard X-ray focusing
Circular and linear zone plates have been fabricated on the surface of
silicon crystals for the energy of 8 keV by electron beam lithography and deep
ion plasma etching methods. Various variants of compound zone plates with
first, second, third diffraction orders have been made. The zone relief height
is about 10 mkm, the outermost zone width of the zone plate is 0.4 mkm. The
experimental testing of the zone plates has been conducted on SPring-8 and ESRF
synchrotron radiation sources. A focused spot size and diffraction efficiency
measured by knife-edge scanning are accordingly 0.5 mkm and 39% for the first
order circular zone plate.Comment: 5 pages, 7 figure
Search for Photon-Photon Elastic Scattering in the X-ray Region
We report the first results of a search for real photon-photon scattering
using X rays. A novel system is developed to split and collide X-ray pulses by
applying interferometric techniques. A total of pulses (each
containing about photons) from an X-ray Free-Electron Laser are
injected into the system. No scattered events are observed, and an upper limit
of (95% C.L.) is obtained on the
photon-photon elastic scattering cross section at 6.5 keV
Revisiting the valence-band and core-level photoemission spectra of NiO
We have re-examined the valence-band (VB) and core-level electronic structure
of NiO by means of hard and soft x-ray photoemission spectroscopy (PES). The
spectral weight of the lowest energy state found to be enhanced in the bulk
sensitive Ni 2p core-level PES. A configuration-interaction model including the
bound state screening has shown significant agreement with the core-level
spectra, and the off and on-resonance VB spectra. These results identify the
lowest energy state in core-level and VB-PES as the Zhang-Rice doublet bound
state, consistent with the spin-fermion model and recent ab initio calculation
with dynamical mean-field theory (LDA + DMFT).Comment: 4 pages, 3 figure
Temperature-Dependence of Magnetically-Active Charge Excitations in Magnetite across the Verwey Transition
We have studied the electronic structure of bulk single crystals and
epitaxial films of magnetite FeO. Fe core-level spectra show clear
differences between hard x-ray (HAX-) and soft x-ray (SX-) photoemission
spectroscopy (PES), indicative of surface effects. The bulk-sensitive spectra
exhibit temperature ()-dependent charge excitations across the Verwey
transition at =122 K, which is missing in the surface-sensitive spectra.
An extended impurity Anderson model full-multiplet analysis reveals roles of
the three distinct Fe-species (A-Fe, B-Fe, B-Fe) below
for the Fe spectra, and its dependent evolution. The Fe
HAXPES spectra show a clear magnetic circular dichroism (MCD) in the metallic
phase of magnetized 100-nm-thick films. The model calculations also reproduce
the MCD and identify the magnetically distinct sites associated with the charge
excitations. Valence band HAXPES shows finite density of states at for
the polaronic metal with remnant order above , and a clear gap formation
below . The results indicate that the Verwey transition is driven by
changes in the strongly correlated and magnetically active B-Fe and
B-Fe electronic states, consistent with resistivity and bulk-sensitive
optical spectra.Comment: 5 pages, 4 figures Accepted in Physical Review Letter
Evidence for a correlated insulator to antiferromagnetic metal transition in CrN
We investigate the electronic structure of Chromium Nitride (CrN) across the
first-order magneto-structural transition at T_N ~ 286 K. Resonant
photoemission spectroscopy shows a gap in the 3d partial density of states at
the Fermi level and an On-site Coulomb energy U ~ 4.5 eV, indicating strong
electron-electron correlations. Bulk-sensitive high resolution (6 meV) laser
photoemission reveals a clear Fermi edge indicating an antiferromagnetic metal
below T_N. Hard x-ray Cr 2p core-level spectra show T-dependent changes across
T_N which originate from screening due to coherent states as substantiated by
cluster model calculations using the experimentally observed U. The electrical
resistivity confirms an insulator above T_N (E_g ~ 70 meV) which becomes a
disordered metal below T_N. The results indicate CrN transforms from a
correlated insulator to an antiferromagnetic metal, coupled to the
magneto-structural transition.Comment: Submitted to Physical Review Letters (February 2010) 11 pages, 3
figures in the main text, 1 Supplementary Informatio
Coherent Acoustic Perturbation of Second-Harmonic-Generation in NiO
We investigate the structural and magnetic origins of the unusual ultrafast
second-harmonicgeneration (SHG) response of femtosecond-laser-excited nickel
oxide (NiO) previously attributed to oscillatory reorientation dynamics of the
magnetic structure induced by d-d excitations. Using time-resolved x-ray
diffraction from the (3/2 3/2 3/2) magnetic planes, we show that changes in the
magnitude of the magnetic structure factor following ultrafast optical
excitation are limited to = 1.5% in the first 30 ps. An
extended investigation of the ultrafast SHG response reveals a strong
dependence on wavelength as well as characteristic echoes, both of which give
evidence for an acoustic origin of the dynamics. We therefore propose an
alternative mechanism for the SHG response based on perturbations of the
nonlinear susceptibility via optically induced strain in a spatially confined
medium. In this model, the two observed oscillation periods can be understood
as the times required for an acoustic strain wave to traverse one coherence
length of the SHG process in either the collinear or anti-collinear geometries.Comment: 26 pages, 7 figure
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