Heterodyne analysis of high-order partial waves in attosecond photoionization of Helium

Partial wave analysis is key to interpretation of the photoionization of atoms and molecules on the attosecond timescale. Here we propose a heterodyne analysis approach, based on the delay-resolved anisotropy parameters to reveal the role played by high-order partial waves during photoionization. This extends the Reconstruction of Attosecond Beating By Interference of Two-photon Transitions technique into the few-photon regime. We demonstrate that even for moderate (∼ 1TW/cm2) intensities, near-infrared-assisted photoionization of helium through Rydberg states results in a tiny contribution from the g0 wave, which has a significant impact on the photoelectron angular distributions via interference with the s- and d0-waves. This modulation also causes a substantial deviation in the angular distribution of the recovered spectral phase shift. Our analysis provides an efficient method to resolve isolated partial wave contributions beyond the perturbative regime, and paves the way towards understanding resonance-enhancement of partial waves

A laboratory study of wind impact on steep unidirectional waves in a long tank

Understanding the effect of wind forcing on steep unidirectional waves is important for the study of wind-wave interaction. In this paper, unidirectional random wave experiments are carried out in a large-scale wave tank in which waves interacted with turbulent wind generated by wind fans. The properties and evolution of deep-water gravity waves subject to following wind forcing are investigated through parametric laboratory experiments. The effect of wind forcing on the significant wave height varies with the initial wave steepness. Wind forcing increases the growth of waves of small initial steepness but attenuates large, steep waves, as a result of the vertical angle of the wind to the free surface in our experiments. The energy input by wind forcing increases the highfrequency tail of the wave spectra, and this effect increases with fetch. The mean frequency increases under wind forcing. The effect of wind forcing on the probability of extreme events is investigated. Wind forcing enhances wave steepness, resulting in a deviation of the exceedance probability from first-order and second-order theoretical distributions and an increased value of kurtosis but not skewness

Atomic partial wave meter by attosecond coincidence metrology

Attosecond chronoscopy is central to the understanding of ultrafast electron dynamics in matter from gas to the condensed phase with attosecond temporal resolution. It has, however, not yet been possible to determine the timing of individual partial waves, and steering their contribution has been a substantial challenge. Here, we develop a polarization-skewed attosecond chronoscopy serving as a partial wave meter to reveal the role of each partial wave from the angle-resolved photoionization phase shifts in rare gas atoms. We steer the relative ratio between different partial waves and realize a magnetic-sublevel-resolved atomic phase shift measurement. Our experimental observations are well supported by time-dependent R-matrix numerical simulations and analytical soft-photon approximation analysis. The symmetry-resolved, partial-wave analysis identifies the transition rate and phase shift property in the attosecond photoelectron emission dynamics. Our findings provide critical insights into the ubiquitous attosecond optical timer and the underlying attosecond photoionization dynamics