15 research outputs found
Tapping.mp4
The camera, installed on an unsecured gimbal without a fixed lock, experiences minor pose shifts with a gentle tap
Media 1: Dynamic 3D imaging based on acousto-optic heterodyne fringe interferometry
Originally published in Optics Letters on 15 June 2014 (ol-39-12-3678
Visualization 1: Suppression of projector distortion in phase-measuring profilometry by projecting adaptive fringe patterns
3D reconstruction result with the proposed method Originally published in Optics Express on 19 September 2016 (oe-24-19-21846
Elucidating the Intercalation Pseudocapacitance Mechanism of MoS<sub>2</sub>–Carbon Monolayer Interoverlapped Superstructure: Toward High-Performance Sodium-Ion-Based Hybrid Supercapacitor
Two-dimensional
(2D) layered materials have shown great promise for electrochemical
energy storage applications. However, they are usually limited by
the sluggish kinetics and poor cycling stability. Interface modification
on 2D layered materials provides an effective way for increasing the
active sites, improving the electronic conductivity, and enhancing
the structure stability so that it can potentially solve the major
issues on fabricating energy storage devices with high performance.
Herein, we synthesize a novel MoS<sub>2</sub>–carbon (MoS<sub>2</sub>–C) monolayer interoverlapped superstructure via a
facile interface-modification route. This interlayer overlapped structure
is demonstrated to have a wide sodium-ion intercalation/deintercalation
voltage range of 0.4–3.0 V and the typical pseudocapacitive
characteristics in fast kinetics, high reversibility, and robust structural
stability, thus displaying a large reversible capacity, a high rate
capability, and an improved cyclability. A full cell of sodium-ion
hybrid supercapacitor based on this MoS<sub>2</sub>–C hybrid
architecture can operate up to 3.8 V and deliver a high energy density
of 111.4 Wh kg<sup>–1</sup> and a high power density exceeding
12 000 W kg<sup>–1</sup>. Furthermore, a long cycle
life of 10 000 cycles with over 77.3% of capacitance retention
can be achieved
Visualization 1: Structured light field 3D imaging
A brief presentation of the procedure and result of the proposed method. Originally published in Optics Express on 05 September 2016 (oe-24-18-20324
Dual-Functional Carbon Dots Pattern on Paper Chips for Fe<sup>3+</sup> and Ferritin Analysis in Whole Blood
Though
microfluidic paper analytical devices (μPADs) have
attracted paramounting attentions in recent years as promising devices
for low cost point-of-care tests, their real applications for blood
analysis are still challenged by integrating sample preparation with
different detection modes on a same μPAD. Herein, we developed
a novel μPAD, which well coupled automatic serum extraction
with reliable dual mode iron health tests: fluorescent analysis for
Fe<sup>3+</sup> and colorimetric ELISA for ferritin. All these functions
are made available by in situ carbon dots (CDs) and AuNPs sequential
patterning techniques. For CDs immobilization, hydrothermal reaction
was taken on paper, to which a patterned through-hole polydimethylsiloxane
(PDMS) mask was applied. None fluorescence CDs (nF-CDs) were generated
on exposed regions, while the fluorescent CDs (F-CDs) were generated
simultaneously on covered regions. Sensitive serum iron quantification
was realized on the F-CDs modified regions, where Fe<sup>3+</sup> ion
can selectively quench the fluorescence of F-CDs. For AuNPs immobilization,
electroless plating was taken on nF-CDs modified regions. The resulting
AuNPs on nF-CDs layer on one hand triggered the coagulation of blood
cells and thus led to the longest ever wicking distance for serum
separation, on the other hand facilitated colorimetric enzyme linked
immunosorbent assay (ELISA) for detection of serum ferritin. Combining
the two readings, the μPAD can provide reliable measurement
for serum iron and serum ferritin in whole blood. Furthermore, as
CDs and AuNPs modified μPAD has the features of easy handling,
low-cost, lightweight, and disposability, it is accounting for a promising
prototype for whole blood point-of-care analysis
Mesoporous TiO<sub>2</sub> Nanocrystals/Graphene as an Efficient Sulfur Host Material for High-Performance Lithium–Sulfur Batteries
Rechargeable lithium–sulfur
(Li–S) batteries are promising in high-energy storage due to
the large specific energy density of about 2600 W h kg<sup>–1</sup>. However, the low conductivity of sulfur and discharge products
as well as polysulfide-shuttle effect between the cathode and anode
hamper applications of Li–S batteries. Herein, we describe
a novel and efficient S host material consisting of mesoporous TiO<sub>2</sub> nanocrystals (NCs) fabricated in situ on reduced graphene
oxide (rGO) for Li–S batteries. The TiO<sub>2</sub>@rGO hybrid
can be loaded with 72 wt % sulfur. The strong chemisorption ability
of the TiO<sub>2</sub> NCs toward polysulfide combined with high electrical
conductivity of rGO effectively localize the soluble polysulfide species
within the cathode and facilitate electron and Li ions transport to/from
the cathode materials. The sulfur-incorporated TiO<sub>2</sub>@rGO
hybrid (S/TiO<sub>2</sub>@rGO) shows large capacities of 1116 and
917 mA h g<sup>–1</sup> at the current densities of 0.2 and
1 C (1 C = 1675 mA g<sup>–1</sup>) after 100 cycles, respectively.
When the current density is increased 20 times from 0.2 to 4 C, 60%
capacity is retained, thereby demonstrating good cycling stability
and rate capability. The synergistic effects of TiO<sub>2</sub> NCs
toward effective chemisorption of polysulfides and conductive rGO
with high electron mobility make a promising application of S/TiO<sub>2</sub>@rGO hybrid in high-performance Li–S batteries
Large-Scale Synthesis and Mechanism of β‑SiC Nanoparticles from Rice Husks by Low-Temperature Magnesiothermic Reduction
Silicon
carbide (SiC) nanomaterials have many applications in semiconductor,
refractories, functional ceramics, and composite reinforcement due
to their unique chemical and physical properties. However, large-scale
and cost-effective synthesis of SiC nanomaterials at a low temperature
is still challenging. Herein, a low-temperature and scalable process
to produce β-phase SiC nanoparticles from rice husks (RHs) by
magnesiothermic reduction (MR) at a relative low temperature of 600
°C is described. The SiC nanoparticles could inherit the morphology
of biogenetic nano-SiO<sub>2</sub> in RHs with a size of about 20–30
nm. The MR reaction mechanism and role of intermediate species are
investigated. The result shows that SiO<sub>2</sub> is first reduced
to Mg<sub>2</sub>Si in the rapid exothermic process and the intermediate
product, Mg<sub>2</sub>Si, further reacts with residual SiO<sub>2</sub> and C to produce SiC. Moreover, the SiC shows considerable electromagnetic
wave absorption with a minimum reflection loss of −5.88 dB
and reflection loss bandwidth < −5 dB of 1.78 GHz. This
paper provides a large-scale, cost-effective, environmental friendly,
and sustainable process to produce high-quality β-phase SiC
nanoparticles from biomass at a low temperature, which is applicable
to functional ceramics and optoelectronics