152 research outputs found

    Microscopic processes controlling the Herschel-Bulkley exponent

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    The flow curve of various yield stress materials is singular as the strain rate vanishes, and can be characterized by the so-called Herschel-Bulkley exponent n=1/βn=1/\beta. A mean-field approximation due to Hebraud and Lequeux (HL) assumes mechanical noise to be Gaussian, and leads to β=2\beta=2 in rather good agreement with observations. Here we prove that the improved mean-field model where the mechanical noise has fat tails instead leads to β=1\beta=1 with logarithmic correction. This result supports that HL is not a suitable explanation for the value of β\beta, which is instead significantly affected by finite dimensional effects. From considerations on elasto-plastic models and on the limitation of speed at which avalanches of plasticity can propagate, we argue that β=1+1/(d−df)\beta=1+1/(d-d_f) where dfd_f is the fractal dimension of avalanches and dd the spatial dimension. Measurements of dfd_f then supports that β≈2.1\beta\approx 2.1 and β≈1.7\beta\approx 1.7 in two and three dimensions respectively. We discuss theoretical arguments leading to approximations of β\beta in finite dimensions.Comment: 9 pages, 3 figure

    Adaptive Elastic Networks as models of supercooled liquids

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    The thermodynamics and dynamics of supercooled liquids correlate with their elasticity. In particular for covalent networks, the jump of specific heat is small and the liquid is {\it strong} near the threshold valence where the network acquires rigidity. By contrast, the jump of specific heat and the fragility are large away from this threshold valence. In a previous work [Proc. Natl. Acad. Sci. U.S.A., 110, 6307 (2013)], we could explain these behaviors by introducing a model of supercooled liquids in which local rearrangements interact via elasticity. However, in that model the disorder characterizing elasticity was frozen, whereas it is itself a dynamic variable in supercooled liquids. Here we study numerically and theoretically adaptive elastic network models where polydisperse springs can move on a lattice, thus allowing for the geometry of the elastic network to fluctuate and evolve with temperature. We show numerically that our previous results on the relationship between structure and thermodynamics hold in these models. We introduce an approximation where redundant constraints (highly coordinated regions where the frustration is large) are treated as an ideal gas, leading to analytical predictions that are accurate in the range of parameters relevant for real materials. Overall, these results lead to a description of supercooled liquids, in which the distance to the rigidity transition controls the number of directions in phase space that cost energy and the specific heat.Comment: 12 pages, 14 figure

    Geometric interpretation of pre-vitrification in hard sphere liquids

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    We derive a microscopic criterion for the stability of hard sphere configurations, and we show empirically that this criterion is marginally satisfied in the glass. This observation supports a geometric interpretation for the initial rapid rise of viscosity with packing fraction, or pre-vitrification. It also implies that barely stable soft modes characterize the glass structure, whose spatial extension is estimated. We show that both the short-term dynamics and activation processes occur mostly along those soft modes, and we study some implications of these observations. This article synthesizes new and previous results [C. Brito and M. Wyart, Euro. Phys. Letters, {\bf 76}, 149-155, (2006) and C. Brito and M. Wyart, J. Stat. Mech., L08003 (2007) ] in a unified view.Comment: accepted for publication in the Journal of Chemical Physics (added discussion on RCP and ideal glass transition

    Unifying Suspension and Granular flows near Jamming

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    Rheological properties of dense flows of hard particles are singular as one approaches the jamming threshold where flow ceases, both for granular flows dominated by inertia, and for over-damped suspensions. Concomitantly, the lengthscale characterizing velocity correlations appears to diverge at jamming. Here we review a theoretical framework that gives a scaling description of stationary flows of frictionless particles. Our analysis applies both to suspensions and inertial flows of hard particles. We report numerical results in support of the theory, and show the phase diagram that results when friction is added, delineating the regime of validity of the frictionless theory.Comment: Short review to appear in Powders and Grains 201

    Stability at Random Close Packing

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    The requirement that packings of hard particles, arguably the simplest structural glass, cannot be compressed by rearranging their network of contacts is shown to yield a new constraint on their microscopic structure. This constraint takes the form a bound between the distribution of contact forces P(f) and the pair distribution function g(r): if P(f) \sim f^{\theta} and g(r) \sim (r-{\sigma})^(-{\gamma}), where {\sigma} is the particle diameter, one finds that {\gamma} \geq 1/(2+{\theta}). This bound plays a role similar to those found in some glassy materials with long-range interactions, such as the Coulomb gap in Anderson insulators or the distribution of local fields in mean-field spin glasses. There is ground to believe that this bound is saturated, offering an explanation for the presence of avalanches of rearrangements with power-law statistics observed in packings

    Correlations between vibrational entropy and dynamics in super-cooled liquids

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    A relation between vibrational entropy and particles mean square displacement is derived in super-cooled liquids, assuming that the main effect of temperature changes is to rescale the vibrational spectrum. Deviations from this relation, in particular due to the presence of a Boson Peak whose shape and frequency changes with temperature, are estimated. Using observations of the short-time dynamics in liquids of various fragility, it is argued that (i) if the crystal entropy is significantly smaller than the liquid entropy at TgT_g, the extrapolation of the vibrational entropy leads to the correlation TK≈T0T_K\approx T_0, where TKT_K is the Kauzmann temperature and T0T_0 is the temperature extracted from the Vogel-Fulcher fit of the viscosity. (ii) The jump in specific heat associated with vibrational entropy is very small for strong liquids, and increases with fragility. The analysis suggests that these correlations stem from the stiffening of the Boson Peak under cooling, underlying the importance of this phenomenon on the dynamical arrest.Comment: Eqs.2 and 7 corrected, results unchange

    Self-referential behaviour, overreaction and conventions in financial markets

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    We study a generic model for self-referential behaviour in financial markets, where agents attempt to use some (possibly fictitious) causal correlations between a certain quantitative information and the price itself. This correlation is estimated using the past history itself, and is used by a fraction of agents to devise active trading strategies. The impact of these strategies on the price modify the observed correlations. A potentially unstable feedback loop appears and destabilizes the market from an efficient behaviour. For large enough feedbacks, we find a `phase transition' beyond which non trivial correlations spontaneously set in and where the market switches between two long lived states, that we call conventions. This mechanism leads to overreaction and excess volatility, which may be considerable in the convention phase. A particularly relevant case is when the source of information is the price itself. The two conventions then correspond then to either a trend following regime or to a contrarian (mean reverting) regime. We provide some empirical evidence for the existence of these conventions in real markets, that can last for several decades.Comment: 15 pages, 12 .eps figure
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