3,367 research outputs found
Differential Scattering Cross-Sections for the Different Product Vibrational States in the Ion-Molecule Reaction Ar+ + N2
The charge transfer reaction Ar+ + N2 --> Ar + N2+ has been investigated in a
crossed beam experiment in combination with three-dimensional velocity map
imaging. Angular differential state-to-state cross sections were determined as
a function of the collision energy. We found that scattering into the first
excited vibrational level dominates as expected, but only for scattering in the
forward direction. Higher vibrational excitations up to v'=6 have been observed
for larger scattering angles. For decreasing collision energy, scattering into
higher scattering angles becomes increasingly important for all kinematically
allowed quantum states. Our detailed measurements indicate that a quantitative
agreement between experiment and theory for this basic ion-molecule reaction
now comes within reach.Comment: accepted to Phys. Rev. Let
How can a 22-pole ion trap exhibit 10 local minima in the effective potential?
The column density distribution of trapped OH ions in a 22-pole ion trap
is measured for different trap parameters. The density is obtained from
position-dependent photodetachment rate measurements. Overall, agreement is
found with the effective potential of an ideal 22-pole. However, in addition we
observe 10 distinct minima in the trapping potential, which indicate a breaking
of the 22-fold symmetry. Numerical simulations show that a displacement of a
subset of the radiofrequency electrodes can serve as an explanation for this
symmetry breaking
Photodetachment of cold OH- in a multipole ion trap
The absolute photodetachment cross section of OH- anions at a rotational and
translational temperature of 170K is determined by measuring the
detachment-induced decay rate of the anions in a multipole radio-frequency ion
trap. In comparison with previous results, the obtained cross section shows the
importance of the initial rotational state distribution. Using a tomography
scan of the photodetachment laser through the trapped ion cloud, the derived
cross section is model-independent and thus features a small systematic
uncertainty. The tomography also yields the column density of the OH- anions in
the 22-pole ion trap in good agreement with the expected trapping potential of
a large field free region bound by steep potential walls.Comment: Phys. Rev. Lett., in pres
Formation of ultracold LiCs molecules
We present the first observation of ultracold LiCs molecules. The molecules
are formed in a two-species magneto-optical trap and detected by two-photon
ionization and time-of-flight mass spectrometry. The production rate
coefficient is found to be in the range 10^{-18}\unit{cm^3s^{-1}} to
10^{-16}\unit{cm^3s^{-1}}, at least an order of magnitude smaller than for
other heteronuclear diatomic molecules directly formed in a magneto-optical
trap.Comment: 8 pages, 2 figure
Saturation of Cs2 Photoassociation in an Optical Dipole Trap
We present studies of strong coupling in single-photon photoassociation of
cesium dimers using an optical dipole trap. A thermodynamic model of the trap
depletion dynamics is employed to extract absolute rate coefficents. From the
dependence of the rate coefficient on the photoassociation laser intensity, we
observe saturation of the photoassociation scattering probability at the
unitarity limit in quantitative agreement with the theoretical model by Bohn
and Julienne [Phys. Rev. A, 60, 414 (1999)]. Also the corresponding power
broadening of the resonance width is measured. We could not observe an
intensity dependent light shift in contrast to findings for lithium and
rubidium, which is attributed to the absence of a p or d-wave shape resonance
in cesium
The Tails of the Crossing Probability
The scaling of the tails of the probability of a system to percolate only in
the horizontal direction was investigated numerically for correlated
site-bond percolation model for .We have to demonstrate that the
tails of the crossing probability far from the critical point have shape
where is the correlation
length index, is the probability of a bond to be closed. At
criticality we observe crossover to another scaling . Here is a scaling index describing the
central part of the crossing probability.Comment: 20 pages, 7 figures, v3:one fitting procedure is changed, grammatical
change
Influence of a Feshbach resonance on the photoassociation of LiCs
We analyse the formation of ultracold 7Li133Cs molecules in the rovibrational
ground state through photoassociation into the B1Pi state, which has recently
been reported [J. Deiglmayr et al., Phys. Rev. Lett. 101, 133004 (2008)].
Absolute rate constants for photoassociation at large detunings from the atomic
asymptote are determined and are found to be surprisingly large. The
photoassociation process is modeled using a full coupled-channel calculation
for the continuum state, taking all relevant hyperfine states into account. The
enhancement of the photoassociation rate is found to be caused by an `echo' of
the triplet component in the singlet component of the scattering wave function
at the inner turning point of the lowest triplet a3Sigma+ potential. This
perturbation can be ascribed to the existence of a broad Feshbach resonance at
low scattering energies. Our results elucidate the important role of couplings
in the scattering wave function for the formation of deeply bound ground state
molecules via photoassociation.Comment: Added Erratum, 20 pages, 9 figure
Evaporation of buffer gas-thermalized anions out of a multipole rf ion trap
We identify plain evaporation of ions as the fundamental loss mechanism out
of a multipole ion trap. Using thermalized negative Cl- ions we find that the
evaporative loss rate is proportional to a Boltzmann factor. This thermodynamic
description sheds new light on the dynamics of particles in time-varying
confining potentials. It specifically allows us to extract the effective depth
of the ion trap as the activation energy for evaporation. As a function of the
rf amplitude we find two distinct regimes related to the stability of motion of
the trapped ions. For low amplitudes the entire trap allows for stable motion
and the trap depth increases with the rf field. For larger rf amplitudes,
however, rapid energy transfer from the field to the ion motion can occur at
large trap radii, which leads to a reduction of the effective trapping volume.
In this regime the trap depth decreases again with increasing rf amplitude. We
give an analytical parameterization of the trap depth for various multipole
traps that allows predictions of the most favorable trapping conditions.Comment: Phys. Rev. Lett., in pres
Search for antiproton decay at the Fermilab Antiproton Accumulator
A search for antiproton decay has been made at the Fermilab Antiproton
Accumulator. Limits are placed on thirteen antiproton decay modes. The results
include the first explicit experimental limits on the muonic decay modes of the
antiproton, and the first limits on the decay modes e- gamma gamma, and e-
omega. The most stringent limit is for the decay mode pbar-> e- gamma. At 90%
C.L. we find that tau/B(pbar-> e- gamma) > 7 x 10^5 yr. The most stringent
limit for decay modes with a muon in the final state is for the decay pbar->
mu- gamma. At 90% C.L. we find that tau/B(pbar-> mu- gamma) > 5 x 10^4 yr.Comment: 20 pages, 8 figures. Submitted to Phys. Rev. D. Final results on 13
channels (was 15) are presente
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