37 research outputs found
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Role of initial magnetic disorder: A time-dependent ab initio study of ultrafast demagnetization mechanisms.
Despite more than 20 years of development, the underlying physics of the laser-induced demagnetization process is still debated. We present a fast, real-time time-dependent density functional theory (rt-TDDFT) algorithm together with the phenomenological atomic Landau-Lifshitz-Gilbert model to investigate this problem. Our Hamiltonian considers noncollinear magnetic moment, spin-orbit coupling (SOC), electron-electron, electron-phonon, and electron-light interactions. The algorithm for time evolution achieves hundreds of times of speedup enabling calculation of large systems. Our simulations yield a demagnetization rate similar to experiments. We found that (i) the angular momentum flow from light to the system is not essential and the spin Zeeman effect is negligible. (ii) The phonon can play a role but is not essential. (iii) The initial spin disorder and the self-consistent update of the electron-electron interaction play dominant roles and enhance the demagnetization to the experimentally observed rate. The spin disorder connects the electronic structure theory with the phenomenological three-temperature model
Electron Accumulation and Emergent Magnetism in LaMnO3/SrTiO3 Heterostructures
Emergent phenomena at polar-nonpolar oxide interfaces have been studied
intensely in pursuit of next-generation oxide electronics and spintronics. Here
we report the disentanglement of critical thicknesses for electron
reconstruction and the emergence of ferromagnetism in polar-mismatched
LaMnO3/SrTiO3 (001) heterostructures. Using a combination of element-specific
X-ray absorption spectroscopy and dichroism, and first-principles calculations,
interfacial electron accumulation and ferromagnetism have been observed within
the polar, antiferromagnetic insulator LaMnO3. Our results show that the
critical thickness for the onset of electron accumulation is as thin as 2 unit
cells (UC), significantly thinner than the observed critical thickness for
ferromagnetism of 5 UC. The absence of ferromagnetism below 5 UC is likely
induced by electron over-accumulation. In turn, by controlling the doping of
the LaMnO3, we are able to neutralize the excessive electrons from the polar
mismatch in ultrathin LaMnO3 films and thus enable ferromagnetism in films as
thin as 3 UC, extending the limits of our ability to synthesize and tailor
emergent phenomena at interfaces and demonstrating manipulation of the
electronic and magnetic structures of materials at the shortest length scales.Comment: Accepted by Phys. Rev. Let
Evidence for topological surface states in amorphous BiSe
Crystalline symmetries have played a central role in the identification of
topological materials. The use of symmetry indicators and band representations
have enabled a classification scheme for crystalline topological materials,
leading to large scale topological materials discovery. In this work we address
whether amorphous topological materials, which lie beyond this classification
due to the lack of long-range structural order, exist in the solid state. We
study amorphous BiSe thin films, which show a metallic behavior and
an increased bulk resistance. The observed low field magnetoresistance due to
weak antilocalization demonstrates a significant number of two dimensional
surface conduction channels. Our angle-resolved photoemission spectroscopy data
is consistent with a dispersive two-dimensional surface state that crosses the
bulk gap. Spin resolved photoemission spectroscopy shows this state has an
anti-symmetric spin-texture resembling that of the surface state of crystalline
BiSe. These experimental results are consistent with theoretical
photoemission spectra obtained with an amorphous tight-binding model that
utilizes a realistic amorphous structure. This discovery of amorphous materials
with topological properties uncovers an overlooked subset of topological matter
outside the current classification scheme, enabling a new route to discover
materials that can enhance the development of scalable topological devices.Comment: 40 pages (21 main + 19 supplemental), 15 figures (4 main + 11
supplemental
Recommended from our members
Role of initial magnetic disorder: A time-dependent ab initio study of ultrafast demagnetization mechanisms.
Despite more than 20 years of development, the underlying physics of the laser-induced demagnetization process is still debated. We present a fast, real-time time-dependent density functional theory (rt-TDDFT) algorithm together with the phenomenological atomic Landau-Lifshitz-Gilbert model to investigate this problem. Our Hamiltonian considers noncollinear magnetic moment, spin-orbit coupling (SOC), electron-electron, electron-phonon, and electron-light interactions. The algorithm for time evolution achieves hundreds of times of speedup enabling calculation of large systems. Our simulations yield a demagnetization rate similar to experiments. We found that (i) the angular momentum flow from light to the system is not essential and the spin Zeeman effect is negligible. (ii) The phonon can play a role but is not essential. (iii) The initial spin disorder and the self-consistent update of the electron-electron interaction play dominant roles and enhance the demagnetization to the experimentally observed rate. The spin disorder connects the electronic structure theory with the phenomenological three-temperature model
PTPRC functions as a prognosis biomarker in the tumor microenvironment of cutaneous melanoma
Abstract Cutaneous melanoma is one of the most malignant types of skin cancer, with an extremely poor prognosis. Immune cells infiltrated in the tumor microenvironment (TME) affects melanoma initiation, progression, prognosis and immunotherapy strategies in melanoma. The potential utility of TME-related genes as a prognostic model for melanoma and as a predictor of immunotherapeutic response merits further exploration. In this study, we determined that an immune-related gene, protein tyrosine phosphatase receptor type C (PTPRC), was positively correlated with the positive prognosis of melanoma patients. Integration of this gene with TNM classification created a predictive model that showed better performance in determining overall survival than others. PTPRC expression was positively correlated with the levels of immune checkpoint molecules, and PTPRC knockdown significantly enhanced the migration, invasion, and proliferation of melanoma cells. Finally, immunohistochemical results from HPA and Real-time quantitative PCR of clinical tissues confirmed that PTPRC expression was higher in melanoma than in normal skin. In conclusion, PTPRC served as a potential predictor of survival and response to immunotherapy in melanoma patients. The risk model combining the PTPRC and TNM classifications holds the potential to be a promising tool for prognostic prediction of cutaneous melanoma. This will help in the effective clinical management of melanoma patients
Analysis of orthogonal signal of dual-mass micro-machined gyroscope
The dual-mass Silicon micro-machined gyroscope was processed by micro-fabrication technology. It could lead to quadrature coupling error and influence the output of the silicon micro-gyroscope. We select two commonly used gyroscope structures and analyze their quadrature coupling coefficient. Firstly, the complete dynamic model is proposed for the DMSG and the theoretical models of sensitivity and orthogonal signals are given by the dynamic model. Second, the influence of support structure on sensitivity and orthogonal signals are analyzed. The sensitivity and orthogonal signal of the two types of DMSG are derived and compared. The results show that the theoretical accuracy of the sensitivity and orthogonal signals can be improved about 50% and 30% after considering the support structure. The type-B gyroscope are insensitive to the Coriolis force (≈13% reduction) when compared to Type-A gyroscope. On the other hand the type-B gyroscope are insensitive to coupling stiffness (≈85% reduction) when compared to Type-A gyroscope. At last, the reliability of the theory is verified by simulations and experiments
Cloning, Expression, and Tobacco Overexpression Analyses of a PISTILLATA/GLOBOSA-like (OfGLO1) Gene from Osmanthus fragrans
GLOBOSA (GLO), a B-class MADS-box gene, is involved in floral organ determination but has rarely been studied in Osmanthus fragrans, which is a very popular ornamental tree species in China. Here, the full-length cDNA of a homologous GLO1 gene (named OfGLO1) was cloned from a flower bud of O. fragrans using the RACE technique. The OfGLO1 has a 645 bp open reading frame, encoding 214 amino acids. Similar to other PI/GLO proteins, OfGLO1 has two conserved domains, MADS MEF2-like and K-box, and a 16-amino-acid PI motif in the C terminal region. Our phylogeny analysis classified OfGLO1 as a PI-type member of the B-class MADS-box gene family. The qRT-PCR assay showed that the expression of OfGLO1 in O. fragrans was continuously upregulated from the tight bud stage to the full flowering stage but barely expressed in the pistils, sepals, and non-floral organs, such as root, leaf, and stem. The genetic effect of OfGLO1 was assayed by ectopic expression in tobacco plants. Compared with the wild-type, OfGLO1 transformants showed reduced plant size, earlier flowering, shorter stamens, and lower seed setting rates. Furthermore, some stamens were changed into petal-like structures. These findings indicate that OfGLO1 plays an important role in the regulation of flower development. This study improved our understanding of class B gene function in woody plants