Higher variations for free L\'evy processes

For a general free L\'evy process, we prove the existence of its higher variation processes as limits in distribution, and identify the limits in terms of the L\'evy-It\^o representation of the original process. For a general free compound Poisson process, this convergence holds almost uniformly, This implies joint convergence in distribution to a $k$-tuple of higher variation processes, and so the existence of $k$-fold stochastic integrals as almost uniform limits. If the existence of moments of all orders is assumed, the result holds for free additive (not necessarily stationary) processes and more general approximants. In the appendix we note relevant properties of symmetric polynomials in non-commuting variables

Numerically exact, time-dependent study of correlated electron transport in model molecular junctions

The multilayer multiconfiguration time-dependent Hartree theory within second quantization representation of the Fock space is applied to study correlated electron transport in models of single-molecule junctions. Extending previous work, we consider models which include both electron-electron and electronic-vibrational interaction. The results show the influence of the interactions on the transient and the stationary electrical current. The underlying physical mechanisms are analyzed in conjunction with the nonequilibrium electronic population of the molecular bridge.Comment: arXiv admin note: substantial text overlap with arXiv:1103.494