Beam-Size Invariant Spectropolarimeters Using Gap-Plasmon Metasurfaces

Metasurfaces enable exceptional control over the light with surface-confined planar components, offering the fascinating possibility of very dense integration and miniaturization in photonics. Here, we design, fabricate and experimentally demonstrate chip-size plasmonic spectropolarimeters for simultaneous polarization state and wavelength determination. Spectropolarimeters, consisting of three gap-plasmon phase-gradient metasurfaces that occupy 120{\deg} circular sectors each, diffract normally incident light to six predesigned directions, whose azimuthal angles are proportional to the light wavelength, while contrasts in the corresponding diffraction intensities provide a direct measure of the incident polarization state through retrieval of the associated Stokes parameters. The proof-of-concept 96-{\mu}m-diameter spectropolarimeter operating in the wavelength range of 750-950nm exhibits the expected polarization selectivity and high angular dispersion. Moreover, we show that, due to the circular-sector design, polarization analysis can be conducted for optical beams of different diameters without prior calibration, demonstrating thereby the beam-size invariant functionality. The proposed spectropolarimeters are compact, cost-effective, robust, and promise high-performance real-time polarization and spectral measurements

Direct amplitude-phase near-field observation of higher-order anapole states

Anapole states associated with the resonant suppression of electric-dipole scattering exhibit minimized extinction and maximized storage of electromagnetic energy inside a particle. Using numerical simulations, optical extinction spectroscopy and amplitude-phase near-field mapping of silicon dielectric disks, we demonstrate high-order anapole states in the near-infrared wavelength range (900-1700 nm). We develop the procedure for unambiguously identifying anapole states by monitoring the normal component of the electric near-field and experimentally detect the first two anapole states as verified by far-field extinction spectroscopy and confirmed with the numerical simulations. We demonstrate that higher order anapole states possess stronger energy concentration and narrower resonances, a remarkable feature that is advantageous for their applications in metasurfaces and nanophotonics components, such as non-linear higher-harmonic generators and nanoscale lasers

High-efficiency silicon metasurface mirror on a sapphire substrate

For a possible implementation of high-efficiency Si-nanosphere metasurface mirrors functioning at telecom wavelengths in future gravitational wave detectors, exact dimensional and configuration parameters of the total system, including substrate and protective coating, have to be determined a priori. The reflectivity of such multi-layer metasurfaces with embedded Si nanoparticles and their potential limitations need to be investigated. Here we present the results on how the substrate and protective layer influence optical properties and demonstrate how dimensional and material characteristics of the structure alter light reflectivity. Additionally, we consider the impact of manufacturing imperfections, such as fluctuations of Si nanoparticle sizes and their exact placement, on the metasurface reflectivity. Finally, we demonstrate how high reflectivity of the system can be preserved under variations of the protective layer thickness, incident angle of light, and its polarization

High-index and low-loss topological insulators for mid-infrared nanophotonics

Topological insulators generally have dielectric bulk and conductive surface states. Consequently, some of these materials have been shown to support polaritonic modes at visible and THz frequencies. At the same time, the optical properties of topological insulators in the mid-infrared (IR) remain poorly investigated. We employ near-field imaging to probe the mid-IR response from the exfoliated flakes of bismuth (Bi) / selenide (Se) / telluride (Te) / antimony (Sb) crystals with varying stoichiometry - Bi2Se3, Bi2Te2Se, and Bi1.5Sb0.5Te1.7Se1.3 - in pristine form as well as covered by thin flakes of hexagonal boron nitride (hBN). Contrary to theoretical expectations, all three materials exhibit a dielectric response with a high refractive index and with a loss below the experimental detection limit. Particularly, the near-field mapping of propagating phonon-polaritons in hBN demonstrates that these van der Waals crystals act as a practically lossless dielectric substrate with an ultra-high refractive index of up to 7.5 in Bi2Te2Se. Such a unique dielectric crystal would be of great advantage for numerous nanophotonic applications in the mid-IR

White light generation and anisotropic damage in gold films near percolation threshold

Strongly enhanced and confined electromagnetic fields generated in metal nanostructures upon illumination are exploited in many emerging technologies by either fabricating sophisticated nanostructures or synthesizing colloid nanoparticles. Here we study effects driven by field enhancement in vanishingly small gaps between gold islands in thin films near the electrically determined percolation threshold. Optical explorations using two-photon luminescence (TPL) and near-field microscopies reveals super-cubic TPL power dependencies with white-light spectra, establishing unequivocally that the strongest TPL signals are generated with close to the percolation threshold films, and occurrence of extremely confined (~ 30 nm)and strongly enhanced (~ 100 times) fields at the illumination wavelength. For linearly polarized and sufficiently powerful light, we observe pronounced optical damage with TPL images being sensitive to both wavelength and polarization of illuminating light. We relate these effects to thermally induced morphological changes observed with scanning electron microscopy images. Fascinating physics involved in light interaction with near-percolation metal films along with their straightforward and scalable one-step fabrication procedure promises a wide range of fascinating developments and technological applications within diverse areas of modern nanotechnology, from bio-molecule optical sensing to ultra-dense optical data storage.Comment: 42 pages in total of the main (27 pages) and supplementary (15 pages) material with 4 main and 10 supplementary figure