1,657 research outputs found
The reduction of nitric-oxide by hydrogen over Pt, Rh and Pt-Rh single crystal surfaces
R.A. van Santen: question, p. 35
The partially asymmetric zero range process with quenched disorder
We consider the one-dimensional partially asymmetric zero range process where
the hopping rates as well as the easy direction of hopping are random
variables. For this type of disorder there is a condensation phenomena in the
thermodynamic limit: the particles typically occupy one single site and the
fraction of particles outside the condensate is vanishing. We use extreme value
statistics and an asymptotically exact strong disorder renormalization group
method to explore the properties of the steady state. In a finite system of
sites the current vanishes as , where the dynamical exponent,
, is exactly calculated. For the transport is realized by active particles, which move with a constant velocity, whereas for
the transport is due to the anomalous diffusion of a single Brownian
particle. Inactive particles are localized at a second special site and their
number in rare realizations is macroscopic. The average density profile of
inactive particles has a width of, , in terms of the
asymmetry parameter, . In addition to this, we have investigated the
approach to the steady state of the system through a coarsening process and
found that the size of the condensate grows as for large
times. For the unbiased model is formally infinite and the coarsening is
logarithmically slow.Comment: 12 pages, 9 figure
Theoretical investigation of CH4 decomposition on Ni: electronic structure calculations and dynamics
Fourier-transform infrared study of the protonation of the zeolitic lattice. Influence of silicon : aluminium ratio and structure
Dynamics of an exclusion process with creation and annihilation
We examine the dynamical properties of an exclusion process with creation and
annihilation of particles in the framework of a phenomenological domain-wall
theory, by scaling arguments and by numerical simulation. We find that the
length- and time scale are finite in the maximum current phase for finite
creation- and annihilation rates as opposed to the algebraically decaying
correlations of the totally asymmetric simple exclusion process (TASEP).
Critical exponents of the transition to the TASEP are determined. The case
where bulk creation- and annihilation rates vanish faster than the inverse of
the system size N is also analyzed. We point out that shock localization is
possible even for rates proportional to 1/N^a, 1<a<2.Comment: 16 pages, 8 figures, typos corrected, references added, section 4
revise
Electronic structure calculations and dynamics of methane activation on nickel and cobalt
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