Nuclear Charge Radii of Neutron-Deficient Lead Isotopes Beyond N=104 Midshell Investigated by In-Source Laser Spectroscopy

The shape of exotic even-mass 182–190Pb isotopes was probed by measurement of optical isotope shifts providing mean square charge radii (δ⟨r2⟩). The experiment was carried out at the isolde (cern) on-line mass separator, using in-source laser spectroscopy. Small deviations from the spherical droplet model are observed, but when compared to model calculations, those are explained by high sensitivity of δ⟨r2⟩ to beyond mean-field correlations and small admixtures of intruder configurations in the ground state. The data support the predominantly spherical shape of the ground state of the proton-magic Z=82 lead isotopes near neutron midshell (N=104)

Development of a RILIS ionisation scheme for gold at ISOLDE, CERN

At the ISOLDE on-line isotope separation facility, the resonance ionisation laser ion source (RILIS) can be used to ionise reaction products as they effuse from the target. The RILIS process of laser step-wise resonance ionisation of atoms in a hot metal cavity provides a highly element selective stage in the preparation of the radioactive ion beam. As a result, the ISOLDE mass separators can provide beams of a chosen isotope with greatly reduced isobaric contamination. With the addition of a new three-step ionisation scheme for gold, the RILIS is now capable of ionising 26 of the elements. The optimal scheme was determined during an extensive study of the atomic energy levels and auto-ionising states of gold, carried out by means of in-source resonance ionisation spectroscopy. Details of the ionisation scheme and a summary of the spectroscopy study are presente

Alkali suppression within laser ion-source cavities and time structure of the laser ionized ion-bunches

The chemical selectivity of the target and ion-source production system is an asset for Radioactive Ion-Beam (RIB) facilities equipped with mass separators. Ionization via laser induced multiple resonant steps Ionization has such selectivity. However, the selectivity of the ISOLDE Resonant Ionization Laser Ion-Source (RILIS), where ionization takes place within high temperature refractory metal cavities, suffers from unwanted surface ionization of low ionization potential alkalis. In order to reduce this type of isobaric contaminant, surface ionization within the target vessel was used. On-line measurements of the efficiency of this method is reported, suppression factors of alkalis up to an order of magnitude were measured as a function of their ionization potential. The time distribution of the ion bunches produced with the RILIS was measured for a variety of elements and high temperature cavity materials. While all ions are produced within a few nanoseconds, the ion bunch sometimes spreads over more than 100 ms. This demonstrates that ions are confined within high temperature metallic cavities. It is the internal electrical field of these cavities that causes the ions to drifts to the extraction region and defines the dwell time of the ions in the cavity. Beam optics calculations were carried out to simulate the pulse shape of a RILIS ion bunch and are compared to the actual measurements

The High Resolution Spectrometer at ISOLDE

ISOLDE's HRS (High Resolution isotope Separator) was recommissioned in mid 2000, after a period out of service. Since then, the separator has routinely run with a mass resolution of 3000-4500 and during 2001 it delivered 72% of ISOLDE's radioactive output. A concerted effort has been made to understand the ion optics and optimise performance. In this paper we present an overview of the HRS and investigate the factors which limit the attainable mass resolution: ion-source emittance; optical aberrations; beam instrumentation and magnet stability

First PAC studies on the hydrogen diffusion in III-V semiconductors

We report on first experiments which observe on a microscopic scale the migration of isolated hydrogen in InP, InAs and GaAs. Using the radioactive acceptor 117Cd, Cd-H pairs have been formed in these III-V semiconductors. After the decay of 117Cd to 117In, H is no longer bound to 117In and can diffuse freely. This diffusion has been observed by perturbed gg angular correlation (PAC) spectroscopy. At 10 K, the occupation of two different lattice sites by hydrogen has been observed

Off-line production of intense 7,10Be+^{7,10}Be^{+} beams

$^7$Be and $^{10}$Be were produced by 590~MeV proton bombardment of a graphite target at PSI. Parts of this graphite target were transferred into an ISOLDE target and ion source unit and ionized with the ISOLDE resonance ionization laser ion source (RILIS). Thus intense radioactive ion beams of 300~nA of $^{7,10}$Be$^+$ were produced off-line