2,212 research outputs found

    An analysis of the fluctuation potential in the modified Poisson-Boltzmann theory for restricted primitive model electrolytes

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    An approximate analytical solution to the fluctuation potential problem in the modified Poisson-Boltzmann theory of electrolyte solutions in the restricted primitive model is presented. The solution is valid for all inter-ionic distances, including contact values. The fluctuation potential solution is implemented in the theory to describe the structure of the electrolyte in terms of the radial distribution functions, and to calculate some aspects of thermodynamics, viz., configurational reduced energies, and osmotic coefficients. The calculations have been made for symmetric valence 1:1 systems at the physical parameters of ionic diameter 4.25×10104.25 \times 10^{-10} m, relative permittivity 78.5, absolute temperature 298 K, and molar concentrations 0.1038, 0.425, 1.00, and 1.968. Radial distribution functions are compared with the corresponding results from the symmetric Poisson-Boltzmann, and the conventional and modified Poisson-Boltzmann theories. Comparisons have also been done for the contact values of the radial distributions, reduced configurational energies, and osmotic coefficients as functions of electrolyte concentration. Some Monte Carlo simulation data from the literature are also included in the assessment of the thermodynamic predictions. Results show a very good agreement with the Monte Carlo results and some improvement for osmotic coefficients and radial distribution functions contact values relative to these theories. The reduced energy curve shows excellent agreement with Monte Carlo data for molarities up to 1 mol/dm3^{3}.Comment: 16 pages, 8 figures, 3 table

    Anisotropic electron g-factor in quantum dots with spin-orbit interaction

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    g-factor tuning of electrons in quantum dots is studied as function of in-plane and perpendicular magnetic fields for different confinements. Rashba and Dresselhaus effects are considered, and comparison is made between wide- and narrow-gap materials. The interplay between magnetic fields and intrinsic spin-orbit coupling is analyzed, with two distinct phases found in the spectrum for GaAs in perpendicular field. The anisotropy of the g-factor is reported, and good agreement with available experimental findings is obtained.Comment: 5 pages, 4 figs. (higher resol. figs. under request

    Kondo screening suppression by spin-orbit interaction in quantum dots

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    We study the transport properties of a quantum dot embedded in an Aharonov-Bohm ring in the presence of spin-orbit interactions. Using a numerical renormalization group analysis of the system in the Kondo regime, we find that the competition of Aharonov-Bohm and spin-orbit dynamical phases induces a strong suppression of the Kondo state singlet, somewhat akin to an effective intrinsic magnetic field in the system. This effective field breaks the spin degeneracy of the localized state and produces a finite magnetic moment in the dot. By introducing an {\em in-plane} Zeeman field we show that the Kondo resonance can be fully restored, reestablishing the spin singlet and a desired spin filtering behavior in the Kondo regime, which may result in full spin polarization of the current through the ring.Comment: 4 pages, 4 figure

    Charge qubits and limitations of electrostatic quantum gates

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    We investigate the characteristics of purely electrostatic interactions with external gates in constructing full single qubit manipulations. The quantum bit is naturally encoded in the spatial wave function of the electron system. Single-electron{transistor arrays based on quantum dots or insulating interfaces typically allow for electrostatic controls where the inter-island tunneling is considered constant, e.g. determined by the thickness of an insulating layer. A representative array of 3x3 quantum dots with two mobile electrons is analyzed using a Hubbard Hamiltonian and a capacitance matrix formalism. Our study shows that it is easy to realize the first quantum gate for single qubit operations, but that a second quantum gate only comes at the cost of compromising the low-energy two-level system needed to encode the qubit. We use perturbative arguments and the Feshbach formalism to show that the compromising of the two-level system is a rather general feature for electrostatically interacting qubits and is not just related to the specific details of the system chosen. We show further that full implementation requires tunable tunneling or external magnetic fields.Comment: 7 pages, 5 figures, submitted to PR

    Impurity-enhanced Aharonov-Bohm effect in neutral quantum-ring magnetoexcitons

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    We study the role of impurity scattering on the photoluminescence (PL) emission of polarized magnetoexcitons. We consider systems where both the electron and hole are confined on a ring structure (quantum rings) as well as on a type-II quantum dot. Despite their neutral character, excitons exhibit strong modulation of energy and oscillator strength in the presence of magnetic fields. Scattering impurities enhance the PL intensity on otherwise "dark" magnetic field windows and non-zero PL emission appears for a wide magnetic field range even at zero temperature. For higher temperatures, impurity-induced anticrossings on the excitonic spectrum lead to unexpected peaks and valleys on the PL intensity as function of magnetic field. Such behavior is absent on ideal systems and can account for prominent features in recent experimental results.Comment: 7 pages, 7 figures, RevTe

    Spatial correlations in chaotic nanoscale systems with spin-orbit coupling

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    We investigate the statistical properties of wave functions in chaotic nanostructures with spin-orbit coupling (SOC), focussing in particular on spatial correlations of eigenfunctions. Numerical results from a microscopic model are compared with results from random matrix theory in the crossover from the gaussian orthogonal to the gaussian symplectic ensembles (with increasing SOC); one- and two-point distribution functions were computed to understand the properties of eigenfunctions in this crossover. It is found that correlations of wave function amplitudes are suppressed with SOC; nevertheless, eigenfunction correlations play a more important role in the two-point distribution function(s), compared to the case with vanishing SOC. Experimental consequences of our results are discussed.Comment: Submitted to PR

    Zero-field Kondo splitting and quantum-critical transition in double quantum dots

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    Double quantum dots offer unique possibilities for the study of many-body correlations. A system containing one Kondo dot and one effectively noninteracting dot maps onto a single-impurity Anderson model with a structured (nonconstant) density of states. Numerical renormalization-group calculations show that while band filtering through the resonant dot splits the Kondo resonance, the singlet ground state is robust. The system can also be continuously tuned to create a pseudogapped density of states and access a quantum critical point separating Kondo and non-Kondo phases.Comment: 4 pages, 4 figures; Accepted for publication in Physical Review Letter
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