4,034 research outputs found
Optimizing thermal transport in the Falicov-Kimball model: binary-alloy picture
We analyze the thermal transport properties of the Falicov-Kimball model
concentrating on locating regions of parameter space where the thermoelectric
figure-of-merit ZT is large. We focus on high temperature for power generation
applications and low temperature for cooling applications. We constrain the
static particles (ions) to have a fixed concentration, and vary the conduction
electron concentration as in the binary-alloy picture of the Falicov-Kimball
model. We find a large region of parameter space with ZT>1 at high temperature
and we find a small region of parameter space with ZT>1 at low temperature for
correlated systems, but we believe inclusion of the lattice thermal
conductivity will greatly reduce the low-temperature figure-of-merit.Comment: 13 pages, 14 figures, typeset with ReVTe
Inelastic X-ray scattering in correlated (Mott) insulators
We calculate the inelastic light scattering from X-rays, which allows the
photon to transfer both energy and momentum to the strongly correlated charge
excitations. We find that the charge transfer peak and the low energy peak both
broaden and disperse through the Brillouin zone similar to what is seen in
experiments in materials like Ca_2 Cu O_2 Cl_2.Comment: 5 pages Revtex4, 6 figure
Non Fermi Liquid Behaviour near a spin-glass transition
In this paper we study the competition between the Kondo effect and RKKY
interactions near the zero-temperature quantum critical point of an Ising-like
metallic spin-glass. We consider the mean-field behaviour of various physical
quantities. In the `quantum- critical regime' non-analytic corrections to the
Fermi liquid behaviour are found for the specific heat and uniform static
susceptibility, while the resistivity and NMR relaxation rate have a non-Fermi
liquid dependence on temperature.Comment: 15 pages, RevTex 3.0, 1 uuencoded ps. figure at the en
Raman scattering through a metal-insulator transition
The exact solution for nonresonant A1g and B1g Raman scattering is presented
for the simplest model that has a correlated metal-insulator transition--the
Falicov-Kimball model, by employing dynamical mean field theory. In the general
case, the A1g response includes nonresonant, resonant, and mixed contributions,
the B1g response includes nonresonant and resonant contributions (we prove the
Shastry-Shraiman relation for the nonresonant B1g response) while the B2g
response is purely resonant. Three main features are seen in the nonresonant
B1g channel: (i) the rapid appearance of low-energy spectral weight at the
expense of higher-energy weight; (b) the frequency range for this low-energy
spectral weight is much larger than the onset temperature, where the response
first appears; and (iii) the occurrence of an isosbestic point, which is a
characteristic frequency where the Raman response is independent of temperature
for low temperatures. Vertex corrections renormalize away all of these
anomalous features in the nonresonant A1g channel. The calculated results
compare favorably to the Raman response of a number of correlated systems on
the insulating side of the quantum-critical point (ranging from Kondo
insulators, to mixed-valence materials, to underdoped high-temperature
superconductors). We also show why the nonresonant B1g Raman response is
``universal'' on the insulating side of the metal-insulator transition.Comment: 12 pages, 11 figures, ReVTe
A partition functional and thermodynamic properties of the infinite-dimensional Hubbard model
An approximate partition functional is derived for the infinite-dimensional
Hubbard model. This functional naturally includes the exact solution of the
Falicov-Kimball model as a special case, and is exact in the uncorrelated and
atomic limits. It explicitly keeps spin-symmetry. For the case of the
Lorentzian density of states, we find that the Luttinger theorem is satisfied
at zero temperature. The susceptibility crosses over smoothly from that
expected for an uncorrelated state with antiferromagnetic fluctuations at high
temperature to a correlated state at low temperature via a Kondo-type anomaly
at a characteristic temperature . We attribute this anomaly to the
appearance of the Hubbard pseudo-gap. The specific heat also shows a peak near
. The resistivity goes to zero at zero temperature, in contrast to
other approximations, rises sharply around and has a rough linear
temperature dependence above .Comment: 18 pages, 6 figures upon request, latex, (to appear in Phys. Rev. B
Stalking influenza by vaccination with pre-fusion headless HA mini-stem.
Inaccuracies in prediction of circulating viral strain genotypes and the possibility of novel reassortants causing a pandemic outbreak necessitate the development of an anti-influenza vaccine with increased breadth of protection and potential for rapid production and deployment. The hemagglutinin (HA) stem is a promising target for universal influenza vaccine as stem-specific antibodies have the potential to be broadly cross-reactive towards different HA subtypes. Here, we report the design of a bacterially expressed polypeptide that mimics a H5 HA stem by protein minimization to focus the antibody response towards the HA stem. The HA mini-stem folds as a trimer mimicking the HA prefusion conformation. It is resistant to thermal/chemical stress, and it binds to conformation-specific, HA stem-directed broadly neutralizing antibodies with high affinity. Mice vaccinated with the group 1 HA mini-stems are protected from morbidity and mortality against lethal challenge by both group 1 (H5 and H1) and group 2 (H3) influenza viruses, the first report of cross-group protection. Passive transfer of immune serum demonstrates the protection is mediated by stem-specific antibodies. Furthermore, antibodies indudced by these HA stems have broad HA reactivity, yet they do not have antibody-dependent enhancement activity
NMR investigations of the interaction between the azo-dye sunset yellow and Fluorophenol
The interaction of small molecules with larger noncovalent assemblies is important across a wide range of disciplines. Here, we apply two complementary NMR spectroscopic methods to investigate the interaction of various fluorophenol isomers with sunset yellow. This latter molecule is known to form noncovalent aggregates in isotropic solution, and form liquid crystals at high concentrations. We utilize the unique fluorine-19 nucleus of the fluorophenol as a reporter of the interactions via changes in both the observed chemical shift and diffusion coefficients. The data are interpreted in terms of the indefinite self-association model and simple modifications for the incorporation of a second species into an assembly. A change in association mode is tentatively assigned whereby the fluorophenol binds end-on with the sunset yellow aggregates at low concentration and inserts into the stacks at higher concentrations
The Hubbard Model at Infinite Dimensions: Thermodynamic and Transport Properties
We present results on thermodynamic quantities, resistivity and optical
conductivity for the Hubbard model on a simple hypercubic lattice in infinite
dimensions. Our results for the paramagnetic phase display the features
expected from an intuitive analysis of the one-particle spectra and
substantiate the similarity of the physics of the Hubbard model to those of
heavy fermion systems. The calculations were performed using an approximate
solution to the single-impurity Anderson model, which is the key quantity
entering the solution of the Hubbard model in this limit. To establish the
quality of this approximation we compare its results, together with those
obtained from two other widely used methods, to essentially exact quantum Monte
Carlo results.Comment: 29 pages, 16 figure
Quasi-long-range order in the random anisotropy Heisenberg model: functional renormalization group in 4-\epsilon dimensions
The large distance behaviors of the random field and random anisotropy O(N)
models are studied with the functional renormalization group in 4-\epsilon
dimensions. The random anisotropy Heisenberg (N=3) model is found to have a
phase with the infinite correlation radius at low temperatures and weak
disorder. The correlation function of the magnetization obeys a power law <
m(x) m(y) >\sim |x-y|^{-0.62\epsilon}. The magnetic susceptibility diverges at
low fields as \chi \sim H^{-1+0.15\epsilon}. In the random field O(N) model the
correlation radius is found to be finite at the arbitrarily weak disorder for
any N>3. The random field case is studied with a new simple method, based on a
rigorous inequality. This approach allows one to avoid the integration of the
functional renormalization group equations.Comment: 12 pages, RevTeX; a minor change in the list of reference
Effects of gap anisotropy upon the electronic structure around a superconducting vortex
An isolated single vortex is considered within the framework of the
quasiclassical theory. The local density of states around a vortex is
calculated in a clean type II superconductor with an anisotropy. The anisotropy
of a superconducting energy gap is crucial for bound states around a vortex. A
characteristic structure of the local density of states, observed in the
layered hexagonal superconductor 2H-NbSe2 by scanning tunneling microscopy
(STM), is well reproduced if one assumes an anisotropic s-wave gap in the
hexagonal plane. The local density of states (or the bound states) around the
vortex is interpreted in terms of quasiparticle trajectories to facilitate an
understanding of the rich electronic structure observed in STM experiments. It
is pointed out that further fine structures and extra peaks in the local
density of states should be observed by STM.Comment: 11 pages, REVTeX; 20 PostScript figures; An Animated GIFS file for
the star-shaped vortex bound states is available at
http://mp.okayama-u.ac.jp/~hayashi/vortex.htm
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