549 research outputs found

    Contiguous 3d and 4f magnetism: towards strongly correlated 3d electrons in YbFe2Al10

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    We present magnetization, specific heat, and 27Al NMR investigations on YbFe2Al10 over a wide range in temperature and magnetic field. The magnetic susceptibility at low temperatures is strongly enhanced at weak magnetic fields, accompanied by a ln(T0/T) divergence of the low-T specific heat coefficient in zero field, which indicates a ground state of correlated electrons. From our hard X-ray photo emission spectroscopy (HAXPES) study, the Yb valence at 50 K is evaluated to be 2.38. The system displays valence fluctuating behavior in the low to intermediate temperature range, whereas above 400 K, Yb3+ carries a full and stable moment, and Fe carries a moment of about 3.1 mB. The enhanced value of the Sommerfeld Wilson ratio and the dynamic scaling of spin-lattice relaxation rate divided by T [27(1/T1T)] with static susceptibility suggests admixed ferromagnetic correlations. 27(1/T1T) simultaneously tracks the valence fluctuations from the 4f -Yb ions in the high temperature range and field dependent antiferromagnetic correlations among partially Kondo screened Fe 3d moments at low temperature, the latter evolve out of an Yb 4f admixed conduction band.Comment: To appear in Phys. Rev. Let

    Repulsion and attraction in high Tc superconductors

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    The influence of repulsion and attraction in high-Tc superconductors to the gap functions is studied. A systematic method is proposed to compute the gap functions using the irreducible representations of the point group. It is found that a pure s-wave superconductivity exists only at very low temperatures, and attractive potentials on the near shells significantly expand the gap functions and increase significantly the critical temperature of superconductivity. A strong on-site repulsion drives the A1gA_{1g} gap into a B1gB_{1g} gap. It is expected that superconductivity with the A1gA_{1g} symmetry reaches a high critical temperature due to the cooperation of the on-site and the next-nearest neighbor attractions.Comment: 4 pages, 5figure

    Quantitative study of valence and configuration interaction parameters of the Kondo semiconductors CeM2Al10 (M = Ru, Os and Fe) by means of bulk-sensitive hard x-ray photoelectron spectroscopy

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    The occupancy of the 4f^n contributions in the Kondo semiconductors CeM2Al10(M = Ru, Os and Fe) has been quantitatively determined by means of bulk-sensitive hard x-ray photoelectron spectroscopy (HAXPES) on the Ce 3d core levels. Combining a configuration interaction scheme with full multiplet calculations allowed to accurately describe the HAXPES data despite the presence of strong plasmon excitations in the spectra. The configuration interaction parameters obtained from this analysis -- in particular the hybridization strength V_eff and the effective f binding energy Delta_f -- indicate a slightly stronger exchange interaction in CeOs2Al10 compared to CeRu2Al10, and a significant increase in CeFe2Al10. This verifies the coexistence of a substantial amount of Kondo screening with magnetic order and places the entire CeM2Al10 family in the region of strong exchange interactions.Comment: 9 pages, 4 figures, submitted to Physical Review

    Core-Level Photoemission and Work-Function Investigation of Na on Cu(110)

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    Core-level photoemission, low-energy electron diffraction (LEED), and work-function change measurements have been carried out to study the coverage dependence of Na/Cu(110) at room temperature. The results of LEED and work-function measurements are qualitatively similar to most other investigations of alkali-metal adsorption on fcc(110) metal surfaces. With LEED, we observed an alkali-metal-induced (1×2) reconstruction at intermediate coverage. We have performed a simple calculation to account for the work-function differences between Na/fcc(110) and Na/fcc(111) metal surfaces. The comparison of coverage-dependent core-level binding-energy shifts between Na/Cu(110) and Na/Cu(111) reveals that a low-coverage plateau in the curve of binding energy vs Na coverage for Na/Cu(110) is associated with the Na-induced reconstruction, and can be accounted for within a localized picture of the reconstruction

    Threshold electric field in unconventional density waves

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    As it is well known most of charge density wave (CDW) and spin density wave (SDW) exhibit the nonlinear transport with well defined threshold electric field E_T. Here we study theoretically the threshold electric field of unconventional density waves. We find that the threshold field increases monotonically with temperature without divergent behaviour at T_c, unlike the one in conventional CDW. The present result in the 3D weak pinning limit appears to describe rather well the threshold electric field observed recently in the low-temperature phase (LTP) of alpha-(BEDT-TTF)_2KHg(SCN)_4.Comment: 4 pages, 2 figure

    Phase-Sensitive Tetracrystal Pairing-Symmetry Measurements and Broken Time-Reversal Symmetry States of High Tc Superconductors

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    A detailed analysis of the symmetric tetracrystal geometry used in phase-sensitive pairing symmetry experiments on high Tc superconductors is carried out for both bulk and surface time-reversal symmetry-breaking states, such as the d+id' and d+is states. The results depend critically on the substrate geometry. In the general case, for the bulk d+id' (or d+is) state, the measured flux quantization should in general not be too different from that obtained in the pure d-wave case, provided |d'| << |d| (or |s| << |d|). However, in one particular high symmetry geometry, the d+id' state gives results that allow it to be distinguished from the pure d and the d + is states. Results are also given for the cases where surface d+is or d+id' states occur at a [110] surface of a bulk d-wave superconductor. Remarkably, in the highest symmetry geometry, a number of the broken time-reversal symmetry states discussed above give flux quantization conditions usually associated with states not having broken time- reversal symmetry.Comment: 6 page

    Bulk and surface electronic properties of SmB6: a hard x-ray photoelectron spectroscopy study

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    We have carried out bulk-sensitive hard x-ray photoelectron spectroscopy (HAXPES) measurements on in-situ cleaved and ex-situ polished SmB6 single crystals. Using the multiplet-structure in the Sm 3d core level spectra, we determined reliably that the valence of Sm in bulk SmB6 is close to 2.55 at ~5 K. Temperature dependent measurements revealed that the Sm valence gradually increases to 2.64 at 300 K. From a detailed line shape analysis we can clearly observe that not only the J=0 but also the J=1 state of the Sm 4f 6 configuration becomes occupied at elevated temperatures. Making use of the polarization dependence, we were able to identify and extract the Sm 4f spectral weight of the bulk material. Finally, we revealed that the oxidized or chemically damaged surface region of the ex-situ polished SmB6 single crystal is surprisingly thin, about 1 nm only.Comment: 11 pages, 8 figure

    Simple theory of extremely overdoped HTS

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    We demonstrate the existence of a simple physical picture of superconductivity for extremely overdoped CuO2 planes. It possesses all characteristic features of HTS, such as a high superconducting transition temperature, the dx2y2d_{x^2 - y^2} symmetry of order parameter, and the coexistence of a single electron Fermi surface and a pseudogap in the normal state. Values of pseudogap are calculated for different doping levels. An orbital paramagnetism of preformed pairs is predicted.Comment: 7 pages, 1 figur
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