372 research outputs found
Exciton-phonon effects in carbon nanotube optical absorption
We find that the optical properties of carbon nanotubes reflect remarkably
strong effects of exciton-phonon coupling. Tight-binding calculations show that
a significant fraction of the spectral weight of the absorption peak is
transferred to a distinct exciton+phonon sideband, which is peaked at around
200 meV above the main absorption peak. This sideband provides a distinctive
signature of the excitonic character of the optical transition. The
exciton-phonon coupling is reflected in a dynamical structural distortion,
which contributes a binding energy of up to 100 meV. The distortion is
surprisingly long-ranged, and is strongly dependent on chirality.Comment: 5 pages, 3 figure
Optical Absorption Study by Ab initio Downfolding Approach: Application to GaAs
We examine whether essence and quantitative aspects of electronic excitation
spectra are correctly captured by an effective low-energy model constructed
from an {\em ab initio} downfolding scheme. A global electronic structure is
first calculated by {\em ab initio} density-functional calculations with the
generalized gradient approximation. With the help of constrained density
functional theory, the low-energy effective Hamiltonian for bands near the
Fermi level is constructed by the downfolding procedure in the basis of
maximally localized Wannier functions. The excited states of this low-energy
effective Hamiltonian ascribed to an extended Hubbard model are calculated by
using a low-energy solver. As the solver, we employ the Hartree-Fock
approximation supplemented by the single-excitation configuration-interaction
method considering electron-hole interactions. The present three-stage method
is applied to GaAs, where eight bands are retained in the effective model after
the downfolding. The resulting spectra well reproduce the experimental results,
indicating that our downfolding scheme offers a satisfactory framework of the
electronic structure calculation, particularly for the excitations and dynamics
as well as for the ground state.Comment: 14 pages, 6 figures, and 1 tabl
Intersublevel Polaron Dephasing in Self-Assembled Quantum Dots
Polaron dephasing processes are investigated in InAs/GaAs dots using
far-infrared transient four wave mixing (FWM) spectroscopy. We observe an
oscillatory behaviour in the FWM signal shortly (< 5 ps) after resonant
excitation of the lowest energy conduction band transition due to coherent
acoustic phonon generation. The subsequent single exponential decay yields long
intraband dephasing times of 90 ps. We find excellent agreement between our
measured and calculated FWM dynamics, and show that both real and virtual
acoustic phonon processes are necessary to explain the temperature dependence
of the polarization decay.Comment: 10 pages, 4 figures, submitted to Phys Rev Let
Electron-Phonon Interacation in Quantum Dots: A Solvable Model
The relaxation of electrons in quantum dots via phonon emission is hindered
by the discrete nature of the dot levels (phonon bottleneck). In order to
clarify the issue theoretically we consider a system of discrete fermionic
states (dot levels) coupled to an unlimited number of bosonic modes with the
same energy (dispersionless phonons). In analogy to the Gram-Schmidt
orthogonalization procedure, we perform a unitary transformation into new
bosonic modes. Since only of them couple to the fermions, a
numerically exact treatment is possible. The formalism is applied to a GaAs
quantum dot with only two electronic levels. If close to resonance with the
phonon energy, the electronic transition shows a splitting due to quantum
mechanical level repulsion. This is driven mainly by one bosonic mode, whereas
the other two provide further polaronic renormalizations. The numerically exact
results for the electron spectral function compare favourably with an analytic
solution based on degenerate perturbation theory in the basis of shifted
oscillator states. In contrast, the widely used selfconsistent first-order Born
approximation proves insufficient in describing the rich spectral features.Comment: 8 pages, 4 figure
Theory of optical spectra of polar quantum wells: Temperature effects
Theoretical and numerical calculations of the optical absorption spectra of
excitons interacting with longitudinal-optical phonons in quasi-2D polar
semiconductors are presented. In II-VI semiconductor quantum wells, exciton
binding energy can be tuned on- and off-resonance with the longitudinal-optical
phonon energy by varying the quantum well width. A comprehensive picture of
this tunning effect on the temperature-dependent exciton absorption spectrum is
derived, using the exciton Green's function formalism at finite temperature.
The effective exciton-phonon interaction is included in the Bethe-Salpeter
equation. Numerical results are illustrated for ZnSe-based quantum wells. At
low temperatures, both a single exciton peak as well as a continuum resonance
state are found in the optical absorption spectra. By contrast, at high enough
temperatures, a splitting of the exciton line due to the real phonon absorption
processes is predicted. Possible previous experimental observations of this
splitting are discussed.Comment: 10 pages, 9 figures, to appear in Phys. Rev. B. Permanent address:
[email protected]
Ultrahigh Bandwidth Spin Noise Spectroscopy: Detection of Large g-Factor Fluctuations in Highly n-Doped GaAs
We advance all optical spin noise spectroscopy (SNS) in semiconductors to
detection bandwidths of several hundred gigahertz by employing an ingenious
scheme of pulse trains from ultrafast laser oscillators as an optical probe.
The ultrafast SNS technique avoids the need for optical pumping and enables
nearly perturbation free measurements of extremely short spin dephasing times.
We employ the technique to highly n-doped bulk GaAs where magnetic field
dependent measurements show unexpected large g-factor fluctuations.
Calculations suggest that such large g-factor fluctuations do not necessarily
result from extrinsic sample variations but are intrinsically present in every
doped semiconductor due to the stochastic nature of the dopant distribution.Comment: 5 pages, 3 figure
Ab initio Green's function formalism for band structures
Using the Green's function formalism, an ab initio theory for band structures
of crystals is derived starting from the Hartree-Fock approximation. It is
based on the algebraic diagrammatic construction scheme for the self-energy
which is formulated for crystal orbitals (CO-ADC). In this approach, the poles
of the Green's function are determined by solving a suitable Hermitian
eigenvalue problem. The method is not only applicable to the outer valence and
conduction bands, it is also stable for inner valence bands where strong
electron correlations are effective. The key to the proposed scheme is to
evaluate the self-energy in terms of Wannier orbitals before transforming it to
a crystal momentum representation. Exploiting the fact that electron
correlations are mainly local, one can truncate the lattice summations by an
appropriate configuration selection scheme. This yields a flat configuration
space; i.e., its size scales only linearly with the number of atoms per unit
cell for large systems and, under certain conditions, the computational effort
to determine band structures also scales linearly. As a first application of
the new formalism, a lithium fluoride crystal has been chosen. A minimal basis
set description is studied, and a satisfactory agreement with previous
theoretical and experimental results for the fundamental band gap and the width
of the F 2p valence band complex is obtained.Comment: 20 pages, 3 figures, 1 table, RevTeX4, new section on lithium
fluorid
The Yellow Excitonic Series of Cu2O Revisited by Lyman Spectroscopy
We report on the observation of the yellow exciton Lyman series up to the
fourth term in Cu2O by time-resolved mid-infrared spectroscopy. The dependence
of the oscillator strength on the principal quantum number n can be well
reproduced using the hydrogenic model including an AC dielectric constant, and
precise information on the electronic structure of the 1s exciton state can be
obtained. A Bohr radius a_{1s}=7.9 A and a 1s-2p transition dipole moment
\mu_{1s-2p}= 4.2 eA were found
Synchronized pulse control of decoherence
We present a new strategy for multipulse control over decoherence. When a
two-level system interacts with a reservoir characterized by a specific
frequency, we find that the decoherence is effectively suppressed by
synchronizing the pulse-train application with the dynamical motion of the
reservoir.Comment: 14 pages, 8 figure
A Study Of A New Class Of Discrete Nonlinear Schroedinger Equations
A new class of 1D discrete nonlinear Schrdinger Hamiltonians
with tunable nonlinerities is introduced, which includes the integrable
Ablowitz-Ladik system as a limit. A new subset of equations, which are derived
from these Hamiltonians using a generalized definition of Poisson brackets, and
collectively refered to as the N-AL equation, is studied. The symmetry
properties of the equation are discussed. These equations are shown to possess
propagating localized solutions, having the continuous translational symmetry
of the one-soliton solution of the Ablowitz-Ladik nonlinear
Schrdinger equation. The N-AL systems are shown to be suitable
to study the combined effect of the dynamical imbalance of nonlinearity and
dispersion and the Peierls-Nabarro potential, arising from the lattice
discreteness, on the propagating solitary wave like profiles. A perturbative
analysis shows that the N-AL systems can have discrete breather solutions, due
to the presence of saddle center bifurcations in phase portraits. The
unstaggered localized states are shown to have positive effective mass. On the
other hand, large width but small amplitude staggered localized states have
negative effective mass. The collison dynamics of two colliding solitary wave
profiles are studied numerically. Notwithstanding colliding solitary wave
profiles are seen to exhibit nontrivial nonsolitonic interactions, certain
universal features are observed in the collison dynamics. Future scopes of this
work and possible applications of the N-AL systems are discussed.Comment: 17 pages, 15 figures, revtex4, xmgr, gn
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