Super-quadratic behavior of luminescence decay excited by energy-transfer upconversion

For several decades, energy-transfer upconversion (ETU) in rare-earth-ion doped systems [1,2] has attracted much attention, firstly, because of the fundamental interest in the physical nature of this process and, secondly, because of very practical considerations, namely the demonstration of near-infrared pumped visible light sources and, in reverse, the detrimental influence of ETU on the efficiency of infrared emitting systems.\ud We investigate fundamentally the behavior of infrared luminescence emitted directly from a metastable level and visible luminescence emitted after ETU from this level to higher-lying levels. Although these two luminescences are connected by the same metastable level and influenced by the same ETU process, the infrared luminescence probes all ions, while the visible luminescence probes only the class of ions susceptible to ETU [3]. A simple analytical model [4] predicts that such luminescence decay curves exhibit a super-quadratic dependence of upconversion on direct luminescence decay.\ud The Nd3+ ion can serve as a model system for such investigations. It exhibits strong ETU from the metastable 4F3/2 level. When doped into oxide matrices, the 4F3/2 level is the only metastable level. The Nd3+ energy levels excited by ETU decay by fast multiphonon relaxation and, hence, the weak visible fluorescence emitted from these levels represents a quasi instantaneous reaction on the dynamics of the 4F3/2 level. Experimental results obtained after pulsed laser excitation of Nd3+-doped oxide host materials show indeed a super-quadratic behavior of upconversion versus direct luminescence decay, in accordance with the model predictions [4].\ud \ud [1] F. Auzel, Proc. IEEE 1973, 6, 758\ud [2] J.C. Wright, Top. Appl. Phys. 1976, 15, 239\ud [3] M. Pollnau, D.R. Gamelin, S.R. Lüthi, H.U. Güdel, M.P. Hehlen, Phys. Rev. B 2000, 61, 3337\ud [4] M. Pollnau, J. Alloys Compd. 2002, 341, 5

Superquadratic behavior of upconversion luminescence transients in rare-earth-ion doped laser crystals

Inhomogeneous active-ion distributions in laser materials lead to strong deviations of upconversion versus direct luminescence transients from the quadratic law of energy-transfer upconversion. Measured luminescence decay curves in LaSc3(BO3)4:Nd3+ and GdVO4:Nd3+ confirm experimentally the predicted deviations. Differences in energy migration within the metastable level of Nd3+ are identified

Dependence of upconversion on direct luminescence decay in energy-transfer upconversion

For several decades, energy-transfer upconversion (ETU) in rare-earth-ion doped systems [1,2] has attracted much attention, firstly, because of the fundamental interest in the physical nature of this process and, secondly, because of very practical considerations, namely the demonstration of near-infrared pumped visible light sources and, in reverse, the detrimental influence of ETU on the efficiency of infrared emitting systems. We investigate fundamentally the behavior of and interaction between infrared luminescence emitted directly from a metastable level and visible luminescence emitted after ETU from this metastable level to higher-lying levels. Although these two luminescences are connected by the same metastable level and influenced by the same ETU process, they probe different classes of ions. Whereas the infrared luminescence probes all ions, the visible luminescence probes only the class of ions susceptible to ETU [3]. A simple analytical model [4] predicts that such luminescence decay curves exhibit a super-quadratic dependence of upconversion on direct luminescence decay. The fraction of ions susceptible to ETU can be derived from this model. The Nd3+ ion can serve as a model system for such investigations. It exhibits strong ETU from the metastable 4F3/2 level. When doped into oxide matrices, the 4F3/2 level is the only metastable level within the 4f subshell. The Nd3+ energy levels excited by ETU decay by fast multiphonon relaxation and, hence, the weak visible fluorescence emitted from these levels represents a quasi instantaneous reaction on the dynamics of the 4F3/2 metastable level. Experimental results obtained after pulsed laser excitation of Nd3+-doped oxide host materials show indeed a super-quadratic behavior of upconversion versus direct luminescence decay, in accordance with the model predictions [4]. [1] F. Auzel, Proc. IEEE 6, 758 (1973) [2] J.C. Wright, Top. Appl. Phys. 15, 239 (1976) [3] M. Pollnau, D.R. Gamelin, S.R. Lüthi, H.U. Güdel, M.P. Hehlen, Phys. Rev. B 61, 3337 (2000) [4] M. Pollnau, J. Alloys Compd. 341, 51 (2002

Dynamical response of the "GGG" rotor to test the Equivalence Principle: theory, simulation and experiment. Part I: the normal modes

Recent theoretical work suggests that violation of the Equivalence Principle might be revealed in a measurement of the fractional differential acceleration $\eta$ between two test bodies -of different composition, falling in the gravitational field of a source mass- if the measurement is made to the level of $\eta\simeq 10^{-13}$ or better. This being within the reach of ground based experiments, gives them a new impetus. However, while slowly rotating torsion balances in ground laboratories are close to reaching this level, only an experiment performed in low orbit around the Earth is likely to provide a much better accuracy. We report on the progress made with the "Galileo Galilei on the Ground" (GGG) experiment, which aims to compete with torsion balances using an instrument design also capable of being converted into a much higher sensitivity space test. In the present and following paper (Part I and Part II), we demonstrate that the dynamical response of the GGG differential accelerometer set into supercritical rotation -in particular its normal modes (Part I) and rejection of common mode effects (Part II)- can be predicted by means of a simple but effective model that embodies all the relevant physics. Analytical solutions are obtained under special limits, which provide the theoretical understanding. A simulation environment is set up, obtaining quantitative agreement with the available experimental data on the frequencies of the normal modes, and on the whirling behavior. This is a needed and reliable tool for controlling and separating perturbative effects from the expected signal, as well as for planning the optimization of the apparatus.Comment: Accepted for publication by "Review of Scientific Instruments" on Jan 16, 2006. 16 2-column pages, 9 figure

Thermal noise reduction for present and future gravitational wave detectors

Thermal noise in mirror suspension is and will be the most severe fundamental limit to the low-frequency sensitivity of interferometric gravitational wave detectors currently under construction. The technical solutions, adopted in the Virgo detector, optimize the current suspension scheme, but new materials and new designs are needed to further reduce the suspension thermal noise. Silicon fibers are promising candidates both for room temperature advanced detectors and for future cryogenic interferometric detectors