Photo-excitation band-structure engineering of 2H-NbSe2_2 probed by time- and angle-resolved photoemission spectroscopy

We investigated the nonequilibrium electronic structure of 2H-NbSe$_2$ by time- and angle-resolved photoemission spectroscopy. We find that the band structure is distinctively modulated by strong photo-excitation, as indicated by the unusual increase in the photoelectron intensities around E$_F$. In order to gain insight into the observed photo-induced electronic state, we performed DFT calculations with modulated lattice structures, and found that the variation of the Se height from the Nb layer results in a significant change in the effective mass and band gap energy. We further study the momentum-dependent carrier dynamics. The results suggest that the relaxation is faster at the K-centered Fermi surface than at the $\Gamma$-centered Fermi surface, which can be attributed to the stronger electron-lattice coupling at the K-centered Fermi surface. Our demonstration of band structure engineering suggests a new role for light as a tool for controlling the functionalities of solid-state materials.Comment: 7 pages, 5 figure

Generation of sub-two-cycle CEP-stable optical pulses at 3.5 μm by multiple-plate pulse compression for high-harmonic generation in crystals

Multiple-plate pulse compression of femtosecond mid-infrared pulses is demonstrated using YAG and Si windows. With this robust compression scheme, we produce sub-two-cycle, CEP-stable optical pulses and observe CEP-dependent high harmonic generation in crystals

Generation of sub-two-cycle CEP-stable optical pulses at 3.5 μm by multiple-plate pulse compression for high-harmonic generation in crystals

Multiple-plate pulse compression of femtosecond mid-infrared pulses is demonstrated using YAG and Si windows. With this robust compression scheme, we produce sub-two-cycle, CEP-stable optical pulses and observe CEP-dependent high harmonic generation in crystals

Resonant-Like Field Enhancement by Nanoscale Grating-Coupled Propagating Surface Plasmons and Localized Surface Plasmons in the Mid-Infrared Range: Implications for Ultrafast Plasmonic Electron Sources

We investigated electron emission induced by an intense mid-infrared (MIR) field from a nanoscale aluminum-coated grating. The total photoelectron yields clearly show a resonant-like behavior when frustrated diffraction occurs near the Wood anomaly. This result indicates that a strong near field, which is formed by the localized surface plasmons (LSPs) at the ridge of the grating, can be enhanced by resonantly produced propagating surface plasmons (PSPs) owing to the phase matching between the diffracted light and PSPs. The observed photoelectron spectra can be reproduced well by a simple one-dimensional (1D) model of a near field that contains two parameters: the field enhancement factor, α, and the ridge radius, r0. In addition, we show that the resonant-like photoemission was attributed to the interference of the near fields produced by the LSPs and PSPs in the nanoscale grating structure. These results demonstrate that the nanoscale structure is useful for ultrafast plasmonic electron sources