29 research outputs found
Coupling molecular spin states by photon-assisted tunneling
Artificial molecules containing just one or two electrons provide a powerful
platform for studies of orbital and spin quantum dynamics in nanoscale devices.
A well-known example of these dynamics is tunneling of electrons between two
coupled quantum dots triggered by microwave irradiation. So far, these
tunneling processes have been treated as electric dipole-allowed
spin-conserving events. Here we report that microwaves can also excite
tunneling transitions between states with different spin. In this work, the
dominant mechanism responsible for violation of spin conservation is the
spin-orbit interaction. These transitions make it possible to perform detailed
microwave spectroscopy of the molecular spin states of an artificial hydrogen
molecule and open up the possibility of realizing full quantum control of a two
spin system via microwave excitation.Comment: 13 pages, 9 figure
Universal quantum control of two-electron spin quantum bits using dynamic nuclear polarization
One fundamental requirement for quantum computation is to perform universal
manipulations of quantum bits at rates much faster than the qubit's rate of
decoherence. Recently, fast gate operations have been demonstrated in logical
spin qubits composed of two electron spins where the rapid exchange of the two
electrons permits electrically controllable rotations around one axis of the
qubit. However, universal control of the qubit requires arbitrary rotations
around at least two axes. Here we show that by subjecting each electron spin to
a magnetic field of different magnitude we achieve full quantum control of the
two-electron logical spin qubit with nanosecond operation times. Using a single
device, a magnetic field gradient of several hundred milliTesla is generated
and sustained using dynamic nuclear polarization of the underlying Ga and As
nuclei. Universal control of the two-electron qubit is then demonstrated using
quantum state tomography. The presented technique provides the basis for single
and potentially multiple qubit operations with gate times that approach the
threshold required for quantum error correction.Comment: 11 pages, 4 figures. Supplementary Material included as ancillary
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Observation of anomalous decoherence effect in a quantum bath at room temperature
Decoherence of quantum objects is critical to modern quantum sciences and
technologies. It is generally believed that stronger noises cause faster
decoherence. Strikingly, recent theoretical research discovers the opposite
case for spins in quantum baths. Here we report experimental observation of the
anomalous decoherence effect for the electron spin-1 of a nitrogen-vacancy
centre in high-purity diamond at room temperature. We demonstrate that under
dynamical decoupling, the double-transition can have longer coherence time than
the single-transition, even though the former couples to the nuclear spin bath
as twice strongly as the latter does. The excellent agreement between the
experimental and the theoretical results confirms the controllability of the
weakly coupled nuclear spins in the bath, which is useful in quantum
information processing and quantum metrology.Comment: 22 pages, related paper at http://arxiv.org/abs/1102.557
Circuit Quantum Electrodynamics with a Spin Qubit
Circuit quantum electrodynamics allows spatially separated superconducting
qubits to interact via a "quantum bus", enabling two-qubit entanglement and the
implementation of simple quantum algorithms. We combine the circuit quantum
electrodynamics architecture with spin qubits by coupling an InAs nanowire
double quantum dot to a superconducting cavity. We drive single spin rotations
using electric dipole spin resonance and demonstrate that photons trapped in
the cavity are sensitive to single spin dynamics. The hybrid quantum system
allows measurements of the spin lifetime and the observation of coherent spin
rotations. Our results demonstrate that a spin-cavity coupling strength of 1
MHz is feasible.Comment: Related papers at http://pettagroup.princeton.edu
Confluence of resonant laser excitation and bi-directional quantum dot nuclear spin polarization
Resonant laser scattering along with photon correlation measurements have
established the atom-like character of quantum dots. Here, we present
measurements which challenge this identification for a wide range of
experimental parameters: the absorption lineshapes that we measure at magnetic
fields exceeding 1 Tesla indicate that the nuclear spins polarize by an amount
that ensures locking of the quantum dot resonances to the incident laser
frequency. In contrast to earlier experiments, this nuclear spin polarization
is bi-directional, allowing the electron+nuclear spin system to track the
changes in laser frequency dynamically on both sides of the quantum dot
resonance. Our measurements reveal that the confluence of the laser excitation
and nuclear spin polarization suppresses the fluctuations in the resonant
absorption signal. A master equation analysis shows narrowing of the nuclear
Overhauser field variance, pointing to potential applications in quantum
information processing
Coherent control of three-spin states in a triple quantum dot
Spin qubits involving individual spins in single quantum dots or coupled
spins in double quantum dots have emerged as potential building blocks for
quantum information processing applications. It has been suggested that triple
quantum dots may provide additional tools and functionalities. These include
the encoding of information to either obtain protection from decoherence or to
permit all-electrical operation, efficient spin busing across a quantum
circuit, and to enable quantum error correction utilizing the three-spin
Greenberger-Horn-Zeilinger quantum state. Towards these goals we demonstrate
for the first time coherent manipulation between two interacting three-spin
states. We employ the Landau-Zener-St\"uckelberg approach for creating and
manipulating coherent superpositions of quantum states. We confirm that we are
able to maintain coherence when decreasing the exchange coupling of one spin
with another while simultaneously increasing its coupling with the third. Such
control of pairwise exchange is a requirement of most spin qubit architectures
but has not been previously demonstrated.Comment: 12 pages, 13 figures, and 2 table