949 research outputs found
Luttinger liquid behavior in multi-wall carbon nanotubes
The low-energy theory for multi-wall carbon nanotubes including the
long-ranged Coulomb interactions, internal screening effects, and
single-electron hopping between graphite shells is derived and analyzed by
bosonization methods. Characteristic Luttinger liquid power laws are found for
the tunneling density of states, with exponents approaching their Fermi liquid
value only very slowly as the number of conducting shells increases. With minor
modifications, the same conclusions apply to transport in ropes of single-wall
nanotubes.Comment: 4 pages Revte
Universality of electron correlations in conducting carbon nanotubes
Effective low-energy Hamiltonian of interacting electrons in conducting
single-wall carbon nanotubes with arbitrary chirality is derived from the
microscopic lattice model. The parameters of the Hamiltonian show very weak
dependence on the chiral angle, which makes the low energy properties of
conducting chiral nanotubes universal. The strongest Mott-like electron
instability at half filling is investigated within the self-consistent harmonic
approximation. The energy gaps occur in all modes of elementary excitations and
estimate at eV.Comment: 4 pages, 2 figure
Electronic Properties of Armchair Carbon Nanotubes : Bosonization Approach
The phase Hamiltonian of armchair carbon nanotubes at half-filling and away
from it is derived from the microscopic lattice model by taking the long range
Coulomb interaction into account. We investigate the low energy properties of
the system using the renormalization group method. At half-filling, the ground
state is a Mott insulator with spin gap, in which the bound states of electrons
at different atomic sublattices are formed. The difference from the recent
results [Phys. Rev. Lett. 79, 5082 (1997)] away half-filling is clarified.Comment: 4 pages, 1 figure, Revte
Disorder, pseudospins, and backscattering in carbon nanotubes
We address the effects of disorder on the conducting properties of metal and
semiconducting carbon nanotubes. Experimentally, the mean free path is found to
be much larger in metallic tubes than in doped semiconducting tubes. We show
that this result can be understood theoretically if the disorder potential is
long-ranged. The effects of a pseudospin index that describes the internal
sublattice structure of the states lead to a suppression of scattering in
metallic tubes, but not in semiconducting tubes. This conclusion is supported
by tight-binding calculations.Comment: four page
Exciton binding energies in carbon nanotubes from two-photon photoluminescence
One- and two-photon luminescence excitation spectroscopy showed a series of
distinct excitonic states in single-walled carbon nanotubes. The energy
splitting between one- and two-photon-active exciton states of different
wavefunction symmetry is the fingerprint of excitonic interactions in carbon
nanotubes. We determine exciton binding energies of 0.3-0.4 eV for different
nanotubes with diameters between 0.7 and 0.9 nm. Our results, which are
supported by ab-initio calculations of the linear and non-linear optical
spectra, prove that the elementary optical excitations of carbon nanotubes are
strongly Coulomb-correlated, quasi-one dimensionally confined electron-hole
pairs, stable even at room temperature. This alters our microscopic
understanding of both the electronic structure and the Coulomb interactions in
carbon nanotubes, and has direct impact on the optical and transport properties
of novel nanotube devices.Comment: 5 pages, 4 figure
Strategies for measurement of atmospheric column means of carbon dioxide from aircraft using discrete sampling
[1] Automated flask sampling aboard small charter aircraft has been proposed as a low-cost, reliable method to greatly increase the density of measurements of CO2 mixing ratios in continental regions in order to provide data for assessment of global and regional CO2 budgets. We use data from the CO2 Budget and Rectification-Airborne 2000 campaign over North America to study the feasibility of using discrete ( flask) sampling to determine column mean CO2 in the lowest 4 km of the atmosphere. To simulate flask sampling, data were selected from profiles of CO2 measured continuously with an onboard ( in situ) analyzer. We find that midday column means can be determined without bias relative to true column means measured by the in situ analyzer to within 0.15 and better than 0.10 ppm by using 10 and 20 instantaneously collected flask samples, respectively. More precise results can be obtained by using a flask sampling strategy that linearly integrates over portions of the air column. Using less than 8 - 10 flasks can lead to significant sampling bias for some common profile shapes. Sampling prior to the breakup of the nocturnal stable layer will generally lead to large sampling bias because of the inability of aircraft to probe large CO2 gradients that often exist very close to the ground at night and during the early morning
Subband population in a single-wall carbon nanotube diode
We observe current rectification in a molecular diode consisting of a
semiconducting single-wall carbon nanotube and an impurity. One half of the
nanotube has no impurity, and it has a current-voltage (I-V) charcteristic of a
typical semiconducting nanotube. The other half of the nanotube has the
impurity on it, and its I-V characteristic is that of a diode. Current in the
nanotube diode is carried by holes transported through the molecule's
one-dimensional subbands. At 77 Kelvin we observe a step-wise increase in the
current through the diode as a function of gate voltage, showing that we can
control the number of occupied one-dimensional subbands through electrostatic
doping.Comment: to appear in Physical Review Letters. 4 pages & 3 figure
Scanned Probe Microscopy of Electronic Transport in Carbon Nanotubes
We use electrostatic force microscopy and scanned gate microscopy to probe
the conducting properties of carbon nanotubes at room temperature. Multi-walled
carbon nanotubes are shown to be diffusive conductors, while metallic
single-walled carbon nanotubes are ballistic conductors over micron lengths.
Semiconducting single-walled carbon nanotubes are shown to have a series of
large barriers to conduction along their length. These measurements are also
used to probe the contact resistance and locate breaks in carbon nanotube
circuits.Comment: 4 page
Multi-wall carbon nanotubes as quantum dots
We have measured the differential conductance dI/dV of individual multi-wall
carbon nanotubes (MWNT) of different lengths. A cross-over from wire-like (long
tubes) to dot-like (short tubes) behavior is observed. dI/dV is dominated by
random conductance fluctuations (UCF) in long MWNT devices (L=2...7 ),
while Coulomb blockade and energy level quantization are observed in short ones
(L=300 nm). The electron levels of short MWNT dots are nearly four-fold
degenerate (including spin) and their evolution in magnetic field (Zeeman
splitting) agrees with a g-factor of 2. In zero magnetic field the sequential
filling of states evolves with spin S according to S=0 -> 1/2 -> 0... In
addition, a Kondo enhancement of the conductance is observed when the number of
electrons on the tube is odd.Comment: 10 pages, 4 figure
Kondo physics in carbon nanotubes
The connection of electrical leads to wire-like molecules is a logical step
in the development of molecular electronics, but also allows studies of
fundamental physics. For example, metallic carbon nanotubes are quantum wires
that have been found to act as one-dimensional quantum dots, Luttinger-liquids,
proximity-induced superconductors and ballistic and diffusive one-dimensional
metals. Here we report that electrically-contacted single-wall nanotubes can
serve as powerful probes of Kondo physics, demonstrating the universality of
the Kondo effect. Arising in the prototypical case from the interaction between
a localized impurity magnetic moment and delocalized electrons in a metallic
host, the Kondo effect has been used to explain enhanced low-temperature
scattering from magnetic impurities in metals, and also occurs in transport
through semiconductor quantum dots. The far higher tunability of dots (in our
case, nanotubes) compared with atomic impurities renders new classes of
Kondo-like effects accessible. Our nanotube devices differ from previous
systems in which Kondo effects have been observed, in that they are
one-dimensional quantum dots with three-dimensional metal (gold) reservoirs.
This allows us to observe Kondo resonances for very large electron number (N)
in the dot, and approaching the unitary limit (where the transmission reaches
its maximum possible value). Moreover, we detect a previously unobserved Kondo
effect, occurring for even values of N in a magnetic field.Comment: 7 pages, pdf onl
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