16 research outputs found
Nanoantenna-enhanced ultrafast nonlinear spectroscopy of a single gold nanoparticle
Optical nanoantennas are a novel tool to investigate previously unattainable
dimensions in the nanocosmos. Just like their radio-frequency equivalents,
nanoantennas enhance the light-matter interaction in their feed gap. Antenna
enhancement of small signals promises to open a new regime in linear and
nonlinear spectroscopy on the nanoscale. Without antennas especially the
nonlinear spectroscopy of single nanoobjects is very demanding. Here, we
present for the first time antenna-enhanced ultrafast nonlinear optical
spectroscopy. In particular, we utilize the antenna to determine the nonlinear
transient absorption signal of a single gold nanoparticle caused by mechanical
breathing oscillations. We increase the signal amplitude by an order of
magnitude which is in good agreement with our analytical and numerical models.
Our method will find applications in linear and nonlinear spectroscopy of
nanoobjects, ranging from single protein binding events via nonlinear tensor
elements to the limits of continuum mechanics
Ultrafast optical control of entanglement between two quantum dot spins
The interaction between two quantum bits enables entanglement, the
two-particle correlations that are at the heart of quantum information science.
In semiconductor quantum dots much work has focused on demonstrating single
spin qubit control using optical techniques. However, optical control of
entanglement of two spin qubits remains a major challenge for scaling from a
single qubit to a full-fledged quantum information platform. Here, we combine
advances in vertically-stacked quantum dots with ultrafast laser techniques to
achieve optical control of the entangled state of two electron spins. Each
electron is in a separate InAs quantum dot, and the spins interact through
tunneling, where the tunneling rate determines how rapidly entangling
operations can be performed. The two-qubit gate speeds achieved here are over
an order of magnitude faster than in other systems. These results demonstrate
the viability and advantages of optically controlled quantum dot spins for
multi-qubit systems.Comment: 24 pages, 5 figure
Multi-wave coherent control of a solid-state single emitter
The authors acknowledge support by the European Research Council Starting Grant 'PICSEN' contract no. 306387.Coherent control of individual two-level systems (TLSs) is at the basis of any implementation of quantum information. An impressive level of control is now achieved using nuclear, vacancies and charge spins. Manipulation of bright exciton transitions in semiconductor quantum dots (QDs) is less advanced, principally due to the sub-nanosecond dephasing. Conversely, owing to their robust coupling to light, one can apply tools of nonlinear spectroscopy to achieve all-optical command. Here, we report on the coherent manipulation of an exciton via multi-wave mixing. Specifically, we employ three resonant pulses driving a single InAs QD. The first two induce a four-wave mixing (FWM) transient, which is projected onto a six-wave mixing (SWM) depending on the delay and area of the third pulse, in agreement with analytical predictions. Such a switch enables to demonstrate the generation of SWM on a single emitter and to engineer the spectro-temporal shape of the coherent response originating from a TLS. These results pave the way toward multi-pulse manipulations of solid state qubits via implementing the NMR-like control schemes in the optical domain.PostprintPeer reviewe