59 research outputs found
Time-domain Brillouin Scattering as a Local Temperature Probe in Liquids
We present results of time-domain Brillouin scattering (TDBS) to determine
the local temperature of liquids in contact to an optical transducer. TDBS is
based on an ultrafast pump-probe technique to determine the light scattering
frequency shift caused by the propagation of coherent acoustic waves in a
sample. Since the temperature influences the Brillouin scattering frequency
shift, the TDBS signal probes the local temperature of the liquid. Results for
the extracted Brillouin scattering frequencies recorded at different liquid
temperatures and at different laser powers - i.e. different steady state
background temperatures- are shown to demonstrate the usefulness of TDBS as a
temperature probe. This TDBS experimental scheme is a first step towards the
investigation of ultrathin liquids measured by GHz ultrasonic probing.Comment: arXiv admin note: substantial text overlap with arXiv:1702.0107
Ultrafast Acousto-Plasmonics in Gold Nanoparticles Superlattice
We report the investigation of the generation and detection of GHz coherent
acoustic phonons in plasmonic gold nanoparticles superlattices (NPS). The
experiments have been performed from an optical femtosecond pump-probe scheme
across the optical plasmon resonance of the superlattice. Our experiments allow
to estimate the collective elastic response (sound velocity) of the NPS as well
as an estimate of the nano-contact elastic stiffness. It appears that the
light-induced coherent acoustic phonon pulse has a typical in-depth spatial
extension of about 45 nm which is roughly 4 times the optical skin depth in
gold. The modeling of the transient optical reflectivity indicates that the
mechanism of phonon generation is achieved through ultrafast heating of the NPS
assisted by light excitation of the volume plasmon. These results demonstrate
how it is possible to map the photon-electron-phonon interaction in
subwavelength nanostructures
Single-bubble and multi-bubble cavitation in water triggered by laser-driven focusing shock waves
In this study a single laser pulse spatially shaped into a ring is focused
into a thin water layer, creating an annular cavitation bubble and cylindrical
shock waves: an outer shock that diverges away from the excitation laser ring
and an inner shock that focuses towards the center. A few nanoseconds after the
converging shock reaches the focus and diverges away from the center, a single
bubble nucleates at the center. The inner diverging shock then reaches the
surface of the annular laser-induced bubble and reflects at the boundary,
initiating nucleation of a tertiary bubble cloud. In the present experiments,
we have performed time-resolved imaging of shock propagation and bubble wall
motion. Our experimental observations of single-bubble cavitation and collapse
and appearance of ring-shaped bubble clouds are consistent with our numerical
simulations that solve a one dimensional Euler equation in cylindrical
coordinates. The numerical results agree qualitatively with the experimental
observations of the appearance and growth of bubble clouds at the smallest
laser excitation rings. Our technique of shock-driven bubble cavitation opens
novel perspectives for the investigation of shock-induced single-bubble or
multi-bubble cavitation phenomena in thin liquids
Direct Visualization of Laser-Driven Focusing Shock Waves
Cylindrically or spherically focusing shock waves have been of keen interest
for the past several decades. In addition to fundamental study of materials
under extreme conditions, cavitation, and sonoluminescence, focusing shock
waves enable myriad applications including hypervelocity launchers, synthesis
of new materials, production of high-temperature and high-density plasma
fields, and a variety of medical therapies. Applications in controlled
thermonuclear fusion and in the study of the conditions reached in laser fusion
are also of current interest. Here we report on a method for direct real-time
visualization and measurement of laser-driven shock generation, propagation,
and 2D focusing in a sample. The 2D focusing of the shock front is the
consequence of spatial shaping of the laser shock generation pulse into a ring
pattern. A substantial increase of the pressure at the convergence of the
acoustic shock front is observed experimentally and simulated numerically.
Single-shot acquisitions using a streak camera reveal that at the convergence
of the shock wave in liquid water the supersonic speed reaches Mach 6,
corresponding to the multiple gigapascal pressure range 30 GPa
Transient Grating Spectroscopy in Magnetic Thin Films:Simultaneous Detection of Elastic and Magnetic Dynamics
Surface magnetoelastic waves are coupled elastic and magnetic excitations that propagate along the surface of a magnetic material. Ultrafast optical techniques allow for a non-contact excitation and detection scheme while providing the ability to measure both elastic and magnetic components individually. Here we describe a simple setup suitable for excitation and time resolved measurements of high frequency magnetoelastic waves, which is based on the transient grating technique. The elastic dynamics are measured by diffracting a probe laser pulse from the long-wavelength spatially periodic structural deformation. Simultaneously, a magnetooptical measurement, either Faraday or Kerr effect, is sensitive to the out-of-plane magnetization component. The correspondence in the response of the two channels probes the resonant interaction between the two degrees of freedom and reveals their intimate coupling. Unraveling the observed dynamics requires a detailed understanding of the spatio-temporal evolution of temperature, magnetization and thermo-elastic strain in the ferromagnet. Numerical solution of thermal diffusion in two dimensions provides the basis on which to understand the sensitivity in the magnetooptic detection
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