804 research outputs found
Roles of intrinsic anisotropy and pi-band pairbreaking effects on critical currents in tilted c-axis MgB2 films probed by magneto-optical and transport measurements
Investigations of MgB2 and Fe-based superconductors in recent years have
revealed many unusual effects of multiband superconductivity but manifestations
of anisotropic multiband effects in the critical current density Jc have not
been addressed experimentally, mostly because of the difficulties to measure Jc
along the c-axis. To investigate the effect of very different intrinsic
anisotropies of sigma and pi electron bands in MgB2 on current transport, we
grew epitaxial films with tilted c-axis (THETA ~ 19.5{\deg}), which enabled us
to measure the components of Jc both along the ab-plane and the c-axis using
magneto-optical and transport techniques. These measurements were combined with
scanning and transmission electron microscopy, which revealed terraced steps on
the surface of the c-axis tilted films. The measured field and temperature
dependencies of the anisotropic Jc(H) show that Jc,L parallel to the terraced
steps is higher than Jc,T perpendicular to the terraced steps, and Jc of
thinner films (50 nm) obtained from transport experiments at 0.1 T reaches ~10%
of the depairing current density Jd in the ab plane, while magneto-optical
imaging revealed much higher Jc at lower fields. To analyze the experimental
data we developed a model of anisotropic vortex pinning which accounts for the
observed behavior of Jc in the c-axis tilted films and suggests that the
apparent anisotropy of Jc is affected by current pairbreaking effects in the
weaker {\pi} band. Our results indicate that the out-of-plane current transport
mediated by the {\pi} band could set the ultimate limit of Jc in MgB2
polycrystals.Comment: 21 pges, 13 figure
Evidence for electromagnetic granularity in polycrystalline Sm1111 iron-pnictides with enhanced phase purity
We prepared polycrystalline SmFeAsO1-xFx (Sm1111) bulk samples by sintering
and hot isostatic pressing (HIP) in order to study the effects of phase purity
and relative density on the intergranular current density. Sintered and HIPped
Sm1111 samples are denser with fewer impurity phases, such as SmOF and the
grain boundary wetting phase, FeAs. We found quite complex magnetization
behavior due to variations of both the inter and intragranular current
densities. Removing porosity and reducing second phase content enhanced the
intergranular current density, but HIPping reduced Tc and the intragranular
current density, due to loss of fluorine and reduction of Tc. We believe that
the HIPped samples are amongst the purest polycrystalline 1111 samples yet
made. However, their intergranular current densities are still small, providing
further evidence that polycrystalline pnictides, like polycrystalline cuprates,
are intrinsically granular.Comment: 14 pages, 6 figure
Search for dinucleon decay into pions at Super-Kamiokande
A search for dinucleon decay into pions with the Super-Kamiokande detector
has been performed with an exposure of 282.1 kiloton-years. Dinucleon decay is
a process that violates baryon number by two units. We present the first search
for dinucleon decay to pions in a large water Cherenkov detector. The modes
O C, O
N, and O
O are investigated. No significant excess in the
Super-Kamiokande data has been found, so a lower limit on the lifetime of the
process per oxygen nucleus is determined. These limits are:
years,
years, and
years. The lower
limits on each mode are about two orders of magnitude better than previous
limits from searches for dinucleon decay in iron.Comment: 20 pages, 17 figures. Accepted for publication in Physical Review D
on March 30, 201
Preparation of amino-substituted indenes and 1,4-dihydronaphthalenes using a one-pot multireaction approach: total synthesis of oxybenzo[c]phenanthridine alkaloids
Allylic trichloroacetimidates bearing a 2-vinyl or 2-allylaryl group have been designed as substrates for a one-pot, two-step multi-bond-forming process leading to the general preparation of aminoindenes and amino-substituted 1,4-dihydronaphthalenes. The synthetic utility of the privileged structures formed from this one-pot process was demonstrated with the total synthesis of four oxybenzo[c]phenanthridine alkaloids, oxychelerythrine, oxysanguinarine, oxynitidine, and oxyavicine. An intramolecular biaryl Heck coupling reaction, catalyzed using the Hermann–Beller palladacycle was used to effect the key step during the synthesis of the natural products
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