234 research outputs found
Femtosecond x-ray absorption spectroscopy of spin and orbital angular momentum in photoexcited Ni films during ultrafast demagnetization
We follow for the first time the evolution of the spin and orbital angular
momentum of a thin Ni film during ultrafast demagnetization, by means of x-ray
magnetic circular dichroism. Both components decrease with a 130 +/- 40 fs time
constant upon excitation with a femtosecond laser pulse. Additional x-ray
absorption measurements reveal an increase in the spin-orbit interaction by 6
+/- 2 % during this process. This is the experimental demonstration quantifying
the importance of spin-orbit mediated processes during the demagnetization
A soft X ray plane grating monochromator optimized for elliptical dipole radiation from modern sources
Abstract We describe a new but yet well proven way of making elliptically polarized dipole radiation from the BESSY II storage ring applicable to the SX700 type collimated plane grating monochromator PM3. We show that due to the limited vertical acceptance of the grating a simple use of vertical apertures is not possible in this case. Rather, deflecting the beam up or downwards by rotating the vertically collimating toroidal mirror M1 around the light axis leads to an excellent performance. The resulting detune of the photon energy can be taken into account by a readjustment of the monochromator internal plane mirror M2. The energy resolution of the beamline is not affected by the non zero roll of the collimating mirro
Laser pump X ray probe experiments with electrons ejected from a Cu 111 target space charge acceleration
A comprehensive investigation of the emission characteristics for electrons induced by X rays of a few hundred eV at grazing incidence angles on an atomically clean Cu 111 sample during laser excitation is presented. Electron energy spectra due to intense infrared laser irradiation are investigated at the BESSY II slicing facility. Furthermore, the influence of the corresponding high degree of target excitation high peak current of photoemission on the properties of Auger and photoelectrons liberated by a probe X ray beam is investigated in time resolved pump and probe measurements. Strong electron energy shifts have been found and assigned to space charge acceleration. The variation of the shift with laser power and electron energy is investigated and discussed on the basis of experimental as well as new theoretical result
Electronic tuneability of a structurally rigid surface intermetallic and Kondo lattice: CePt / Pt(111)
We present an extensive study of structure, composition, electronic and
magnetic properties of Ce--Pt surface intermetallic phases on Pt(111) as a
function of their thickness. The sequence of structural phases appearing in low
energy electron diffraction (LEED) may invariably be attributed to a single
underlying intermetallic atomic lattice. Findings from both microscopic and
spectroscopic methods, respectively, prove compatible with CePt formation
when their characteristic probing depth is adequately taken into account. The
intermetallic film thickness serves as an effective tuning parameter which
brings about characteristic variations of the Cerium valence and related
properties. Soft x-ray absorption (XAS) and magnetic circular dichroism (XMCD)
prove well suited to trace the changing Ce valence and to assess relevant
aspects of Kondo physics in the CePt surface intermetallic. We find
characteristic Kondo scales of the order of 10 K and evidence for
considerable magnetic Kondo screening of the local Ce moments.
CePt/Pt(111) and related systems therefore appear to be promising
candidates for further studies of low-dimensional Kondo lattices at surfaces.Comment: 14 pages, 11 figure
Configuration development study of the X-24C hypersonic research airplane
Bottom line results were made of a three-phase study to determine the feasibility of designing, building, and operating, and maintaining an air-launched high performance aircraft capable of cruising at speeds up to Mach 8 for short durations. The results show that Lockalloy heat-sink structure affords the capability for a 'work-horse' vehicle which can serve as an excellent platform for this research. It was further concluded that the performance of a blended wing body configuration surpassed that of a lifting body design for typical X-24C missions. The cost of a two vehicle program, less engines, B-52 modification and contractor support after delivery, can be kept within $70M (in Jan. 1976 dollars)
Study of the depletion depth in a frontside biased CMOS pixel sensors
Depletion of the sensitive volume for semiconductor based detectors is a key to achieve high performance. It is for instance required for charged particle detection in highly radiative environment and for X-ray spectroscopy.
PIPPER-2 is a CMOS pixel sensor featuring an architecture that allows the application of the reverse bias of the pn junction from the frontside (cathode), on the electronic side, without process modification. Biasing voltages up to 45 V have been applied to sensor prototypes fabricated on two different high resistivity substrates: a thin epitaxial layer (1 kΩ cm) and a 40 μm thick bulk substrate (600 Ω cm).
Calculations from a simplified analytical model and 3D-TCAD simulations were conducted to predict the evolution of the depletion depth with the bias voltage. These expectations were compared to measurements of PIPPER-2 illuminated with two X-ray energies.
We conclude that the frontside biasing method allows the full-depletion of the thin epitaxial layer. In contrast, depletion of the bulk substrate reaches about half-depth but X-rays are still detected over the full depth
On-site correlation in valence and core states of ferromagnetic nickel
We present a method which allows to include narrow-band correlation effects
into the description of both valence and core states and we apply it to the
prototypical case of nickel. The results of an ab-initio band calculation are
used as input mean-field eigenstates for the calculation of self-energy
corrections and spectral functions according to a three-body scattering
solution of a multi-orbital Hubbard hamiltonian. The calculated quasi-particle
spectra show a remarkable agreement with photoemission data in terms of band
width, exchange splitting, satellite energy position of valence states, spin
polarization of both the main line and the satellite of the 3p core level.Comment: 14 pages, 10 PostScript figures, RevTeX, submitted to PR
Angular Momentum Flow During Ultrafast Demagnetization of a Ferrimagnet
One of the key processes setting the speed of the ultrafast magnetization phenomena is the angular momentum transfer from and into the spin system. However, the way the angular momentum flows during ultrafast demagnetization and magnetization switching phenomena remains elusive so far. We report on time resolved soft x ray magnetic circular dichroism measurements of the ferrimagnetic GdFeCo alloy allowing us to record the dynamics of elemental spin and orbital moments at the Fe and Gd sites during femtosecond laser induced demagnetization. We observe a complete transfer of spin and orbital angular momentum to the lattice during the first hundreds of femtoseconds of the demagnetization proces
On the electronic structure of electron doped LaOFeAs as seen by X-ray absorption spectroscopy
We investigated the recently found superconductor LaO_{1-x}F_xFeAs by X-ray
absorption spectroscopy (XAS). From a comparison of the O K-edge with LDA
calculations we find good agreement and are able to explain the structure and
changes of the spectra with electron doping. An important result from this edge
is a limitation of the Hubbard U to values not significantly larger than 1 eV.
From experimental Fe L_2,3-edge spectra and charge transfer multiplet
calculations we gain further information on important physical values such as
hopping parameters, the charge transfer energy Delta, and the on-site Hubbard
U. Furthermore we find the system to be very covalent with a large amount of
ligand holes. A shift in the chemical potential is visible in the O K- and Fe
L_2,3-edge spectra which emphasizes the importance of band effects in these
compounds.Comment: 4 pages, 2 figure
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