Effect of Coulomb correlation on electron transport through concentric quantum ring-quantum dot structure

We theoretically study the single electron transfer through two-terminal quantum ring capacitively coupled to charged dot placed in its center. For this purpose we solve time-dependent Schrodinger equation for fully correlated two-particle system constituted by the transferred electron and the second particle confined in the dot. Analysis of transmission probability dependence on magnetic field in Ahronov-Bohm effect indicates that the maxima of transmission probability may be enhanced as well as reduced for attractive or repulsive Coulomb interaction respectively. The existence of Coulomb correlation in the system may also lead to inelastic scattering of the transferred electron. In such case, transmission of electron thorugh the ring is not completely blocked for (n+1/2) magnetic flux quanta

Few-electron artificial molecules formed by laterally coupled quantum rings

We study the artificial molecular states formed in laterally coupled double semiconductor nanorings by systems containing one, two and three electrons. An interplay of the interring tunneling and the electron-electron interaction is described and its consequences for the magnetization and charging properties of the system are determined. It is shown that both the magnetic dipole moment generated by the double ring structure and the chemical potential of the system as function of the external magnetic field strongly depend on the number of electrons and the interring barrier thickness. Both the magnetization and chemical potentials exhibit cusps at the magnetic fields inducing ground-state parity and / or spin transformations. The symmetry transformations are discussed for various tunnel coupling strengths: from rings coupled only electrostatically to the limit of coalesced rings. We find that in the ground-states for rings of different radii the magnetic field transfers the electron charge from one ring to the other. The calculations are performed with the configuration interaction method based on an approach of Gaussian functions centered on a rectangular array of points covering the studied structure. Electron-electron correlation is also discussed

Stability of negative and positive trions in quantum wires

Binding energies of negative ($X^-$) and positive trions ($X^+$) in quantum wires are studied for strong quantum confinement of carriers which results in a numerical exactly solvable model. The relative electron and hole localization has a strong effect on the stability of trions. For equal hole and electron confinement, $X^+$ is more stable but a small imbalance of the particle localization towards a stronger hole localization e.g. due to its larger effective mass, leads to the interchange of $X^-$ and $X^+$ recombination lines in the photoluminescent spectrum as was recently observed experimentally. In case of larger $X^-$ stability, a magnetic field oriented parallel to the wire axis leads to a stronger increase of the $X^+$ binding energy resulting in a crossing of the $X^+$ and $X^-$ lines

Exciton and negative trion dissociation by an external electric field in vertically coupled quantum dots

We study the Stark effect for an exciton confined in a pair of vertically coupled quantum dots. A single-band approximation for the hole and a parabolic lateral confinement potential are adopted which allows for the separation of the lateral center-of-mass motion and consequently for an exact numerical solution of the Schr\"odinger equation. We show that for intermediate tunnel coupling the external electric field leads to the dissociation of the exciton via an avoided crossing of bright and dark exciton energy levels which results in an atypical form of the Stark shift. The electric-field-induced dissociation of the negative trion is studied using the approximation of frozen lateral degrees of freedom. It is shown that in a symmetric system of coupled dots the trion is more stable against dissociation than the exciton. For an asymmetric system of coupled dots the trion dissociation is accompanied by a positive curvature of the recombination energy line as a function of the electric field.Comment: PRB - in prin

In situ biospectroscopic investigation of rapid ischemic and postmortem induced biochemical alterations in the rat brain

© 2014 American Chemical Society. Rapid advances in imaging technologies have pushed novel spectroscopic modalities such as Fourier transform infrared spectroscopy (FTIR) and X-ray absorption spectroscopy (XAS) at the sulfur K-edge to the forefront of direct in situ investigation of brain biochemistry. However, few studies have examined the extent to which sample preparation artifacts confound results. Previous investigations using traditional analyses, such as tissue dissection, homogenization, and biochemical assay, conducted extensive research to identify biochemical alterations that occur ex vivo during sample preparation. In particular, altered metabolism and oxidative stress may be caused by animal death. These processes were a concern for studies using biochemical assays, and protocols were developed to minimize their occurrence. In this investigation, a similar approach was taken to identify the biochemical alterations that are detectable by two in situ spectroscopic methods (FTIR, XAS) that occur as a consequence of ischemic conditions created during humane animal killing. FTIR and XAS are well suited to study markers of altered metabolism such as lactate and creatine (FTIR) and markers of oxidative stress such as aggregated proteins (FTIR) and altered thiol redox (XAS). The results are in accordance with previous investigations using biochemical assays and demonstrate that the time between animal death and tissue dissection results in ischemic conditions that alter brain metabolism and initiate oxidative stress. Therefore, future in situ biospectroscopic investigations utilizing FTIR and XAS must take into consideration that brain tissue dissected from a healthy animal does not truly reflect the in vivo condition, but rather reflects a state of mild ischemia. If studies require the levels of metabolites (lactate, creatine) and markers of oxidative stress (thiol redox) to be preserved as close as possible to the in vivo condition, then rapid freezing of brain tissue via decapitation into liquid nitrogen, followed by chiseling the brain out at dry ice temperatures is required

Synchrotron Radiation X-Ray Microfluorescence Reveals Polarized Distribution of Atomic Elements during Differentiation of Pluripotent Stem Cells

The mechanisms underlying pluripotency and differentiation in embryonic and reprogrammed stem cells are unclear. In this work, we characterized the pluripotent state towards neural differentiated state through analysis of trace elements distribution using the Synchrotron Radiation X-ray Fluorescence Spectroscopy. Naive and neural-stimulated embryoid bodies (EB) derived from embryonic and induced pluripotent stem (ES and iPS) cells were irradiated with a spatial resolution of 20 µm to make elemental maps and qualitative chemical analyses. Results show that these embryo-like aggregates exhibit self-organization at the atomic level. Metallic elements content rises and consistent elemental polarization pattern of P and S in both mouse and human pluripotent stem cells were observed, indicating that neural differentiation and elemental polarization are strongly correlated