357 research outputs found
Large spin-orbit splitting and weakly-anisotropic superconductivity revealed with single-crystalline noncentrosymmetric CaIrSi3
We report normal and superconducting properties of the Rashba-type
noncentrosymmetric com- pound CaIrSi3, using single crystalline samples with
nearly 100% superconducting volume fraction. The electronic density of states
revealed by the hard x-ray photoemission spectroscopy can be well explained by
the relativistic first-principle band calculation. This indicates that strong
spin-orbit interaction indeed affects the electronic states of this compound.
The obtained H - T phase diagram exhibits only approximately 10% anisotropy,
indicating that the superconducting properties are almost three dimensional.
Nevertheless, strongly anisotropic vortex pinning is observed.Comment: 8 pages, 6 figures, 1 table, accepted for publication in Phys. Rev.
Electronic correlations and Hund's coupling effects in SrMoO revealed by photoemission spectroscopy
We investigate the electronic structure of a perovskite-type Pauli paramagnet
SrMoO3 (t2g2) thin film using hard x-ray photoemission spectroscopy and compare
the results to the realistic calculations that combine the density functional
theory within the local-density approximation (LDA) with the dynamical-mean
field theory (DMFT). Despite the clear signature of electron correlations in
the electronic specific heat, the narrowing of the quasiparticle bands is not
observed in the photoemission spectrum. This is explained in terms of the
characteristic effect of Hund's rule coupling for partially-filled t2g bands,
which induces strong quasiparticle renormalization already for values of
Hubbard interaction which are smaller than the bandwidth. The interpretation is
supported by additional model DMFT calculations including Hund's rule coupling,
that show renormalization of low-energy quasiparticles without affecting the
overall bandwidth. The photoemission spectra show additional spectral weight
around -2 eV that is not present in the LDA+DMFT. We interpret this weight as a
plasmon satellite, which is supported by measured Mo, Sr and Oxygen core-hole
spectra that all show satellites at this energy.Comment: 8 pages, 7 figure
Evidence for suppressed metallicity on the surface of La2-xSrxCuO4 and Nd2-xCexCuO4
Hard X-ray Photoemission spectroscopy (PES) of copper core electronic states,
with a probing depth of 60 \AA, is used to show that the Zhang-Rice
singlet feature is present in LaCuO but is absent in NdCuO.
Hole- and electron doping in LaSrCuO (LSCO) and
NdCeCuO (NCCO) result in new well-screened features which are
missing in soft X-ray PES. Impurity Anderson model calculations establish
metallic screening as its origin, which is strongly suppressed within 15
of the surface. Complemented with X-ray absorption spectroscopy,
the small chemical-potential shift in core levels ( eV) are shown to
be consistent with modifications of valence and conduction band states spanning
the band gap ( eV) upon hole- and electron-doping in LSCO and NCCO.Comment: 4 pages, 4 figure
Investigation on MnGa/MgO interface for magnetic tunneling junctions
The MnGa Heusler compound and related alloys are the most promising
materials for the realization of spin-transfer-torque switching in magneto
tunneling junctions. Improved performance can be achieved by high quality
interfaces in these multilayered structured devices. In this context, the
interface between MnGa and MgO is of particular interest because of
its spin polarization properties in tunneling junctions. We performed a
chemical characterization of the MgO/MnGa junction by hard x-ray
photoelectron spectroscopy (HAXPES). The experiment indicated the formation of
Ga-O bonds at the interface and evidenced changes in the local environment of
Mn atoms in the proximity of the MgO film. In addition, we show that the
insertion of a metallic Mg-layer interfacing the MgO and Mn--Ga film strongly
suppresses the oxidation of gallium
Bulk screening in core level photoemission from Mott-Hubbard and Charge-Transfer systems
We report bulk-sensitive hard X-ray ( = 5.95 KeV) core level
photoemission spectroscopy (PES) of single crystal VCrO
and the high- cuprate BiSrCaCuO (Bi2212).
VCrO exhibits low binding energy "satellites" to the V
"main lines" in the metallic phase, which are suppressed in the
antiferromagnetic insulator phase. In contrast, the Cu spectra of Bi2212
do not show temperature dependent features, but a comparison with soft X-ray
PES indicates a large increase in the "satellites" or weight
in the bulk. Cluster model calculations, including full multiplet structure and
a screening channel derived from the coherent band at the Fermi energy, give
very satisfactory agreement with experiments
Recoil effects of photoelectrons in a solid
High energy resolution C 1 photoelectron spectra of graphite were measured
at the excitation energy of 340, 870, 5950 and 7940eV using synchrotron
radiation. On increasing the excitation energy, i.e., increasing kinetic energy
of the photoelectron, the bulk origin C 1 peak position shifts to higher
binding energies. This systematic shift is due to the kinetic energy loss of
the high-energy photoelectron by kicking the atom, and is clear evidence of the
recoil effect in photoelectron emission. It is also observed that the
asymmetric broadening increases for the higher energy photoelectrons. All these
recoil effects can be quantified in the same manner as the M\"ossbauer effect
for -ray emission from nuclei embedded in crystals.Comment: 4 pages, 2 figure
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