15 research outputs found

    Advancing mid-infrared spectroscopy for biomedical applications

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    Direct Generation of an Ultrabroad Spectrum from YtterbiumDoped Thin-Disk Lasers

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    Broadband interferometric subtraction of optical fields

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    We present a Mach-Zehnder-like interferometer capable of simultaneous super-octave (950 – 2100 nm) destructive interference with an intensity extinction of 4 × 10−4. Achromatic nulling is achieved by unbalancing the number of Fresnel reflections off optically denser media in the two interferometer arms. With a methane gas sample in one interferometer arm, we isolate the coherent molecular vibrational emission from the broadband, impulsive excitation and quantitatively examine the potential improvement in detectable concentration, compared to direct transmission geometry. The novel concept will benefit sensing applications requiring high detection sensitivity and dynamic range, including time-domain and frequency-domain spectroscopy.publishe

    Self-compressed, spectral broadening of a Yb:YAG thin-disk amplifier

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    We demonstrate pulse shortening of 1-ps Yb:YAG thin-disk regenerative amplifier to 500 fs by cross-polarized wave generation (XPW) in a 6 mm BaF2 crystal. The process is self-compressed and has 8.5% conversion efficiency corresponding to 18 µJ energy. Our theoretical and experimental investigation shows that the factor of 3−−√ spectral broadening and pulse shortening in ps-XPW-generation only happens in unsaturated regime. We demonstrate that the initial spectral chirp affects the spectral broadening and pulse shortening of XPW pulses

    Sub-Optical-Cycle Light-Matter Energy Transfer Dynamics in Molecular Vibrational Spectroscopy

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    High-power, 1-ps, all-Yb:YAG thin-disk regenerative amplifier

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    We report a 100 W, 20 mJ, 1-ps, all-Yb:YAG thin-disk regenerative amplifier seeded by a microjoule-level Yb:YAG thin-disk Kerr-lens mode-locked oscillator. The regenerative amplifier is implemented in a chirped pulse amplification system and operates at an ambient temperature in air, delivering ultrastable output pulses at a 5 kHz repetition rate and with a root mean square power noise value of less than 0.5%. Second harmonic generation of the amplifier’s output in a 1.5 mm-thick BBO crystal results in more than 70 W at 515 nm, making the system an attractive source for pumping optical parametric chirped pulse amplifiers in the visible and near-infrared spectral ranges
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