13 research outputs found

    Strong Correlations in Electron Doped Phthalocyanine Conductors Near Half Filling

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    We propose that electron doped nontransition metal-phthalocyanines (MPc) like ZnPc and MgPc, similar to those very recently reported, should constitute novel strongly correlated metals. Due to orbital degeneracy, Jahn-Teller coupling and Hund's rule exchange, and with a large on-site Coulomb repulsion, these molecular conductors should display, particularly near half filling at two electrons/molecule, very unconventional properties, including Mott insulators, strongly correlated superconductivity, and other intriguing phases.Comment: 4 pages, 1 figure, submited to PR

    Collectively Induced Quantum-Confined Stark Effect in Monolayers of Molecules Consisting of Polar Repeating Units

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    High Resolution Tips for Switching Magnetization MFM

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    Switching magnetization magnetic force microscopy (SM-MFM) is based on two-pass magnetic force microscopy with opposite orientation of tip magnetization between two scans. The sum of the scanned data with reversed tip magnetization depicts local van der Waals forces, and their difference maps the local magnetic forces. Tip magnetization can be easily reversed in external magnetic field during the scanning. The separation of the forces mapped enables scanning in close proximity of the sample (~5 nm). Therefore, extremely high spatial resolution (10 nm) is achievable by the SM-MFM. Image phase resolution of the MFM method depends on various geometric parameters of the tip, such as tip length, its apex radius and taper angle. The parameters are determined by the evaporation process, within which the standard atomic force microscopy tips are coated with magnetic layer. In this work we show that the thickness of the coated layer is important for the SM-MFM spatial resolution

    Individual vortex nucleation/annihilation in ferromagnetic nanodots with broken symmetry observed by micro-Hall magnetometry

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    We studied vortex nucleation/annihilation process and its temperature dependence in micromagnetic objects with lowered symmetry using micro-Hall magnetometry. Magnetization reversal curves were obtained for the Pacman-like nanodots placed directly on Hall probes. Lowered symmetry of the object leads to good control of its chirality. Vortex nucleation and annihilation fields strongly depend on the angle of the external in-plane magnetic field with respect on the nanodot symmetry. The micromagnetic simulations support the experimental results - the vortex nucleation fields are controlled by local magnetization configurations present in the object (C-, S-, and double S-states) for field just above vortex nucleation field. The experiments also confirm that the vortex nucleation proceeds via thermal activation over an energy barrier

    Vortex Dynamics in Ferromagnetic Nanoelements Observed by Micro-Hall Probes

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    In this work we measure the nucleation and annihilation of magnetic vortices in Pacman-like (PL) micromagnets prepared from Permalloy (Ni81Fe19Ni_{81}Fe_{19}, Py) at 77 K. Lateral dimensions of explored objects are ≤1 μm with thickness of about 40 nm. The micromagnets are located directly on the high-sensitive micro-Hall probe based on GaAs/AlGaAs heterostructure by lift-off process. Experiments show good agreement of the magnetization reversal with the micromagnetic simulation. Other shapes of micromagnets are also considered to obtain more precise picture of the vortex dynamics

    Duffing oscillation-induced reversal of magnetic vortex core by a resonant perpendicular magnetic field

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    Nonlinear dynamics of the magnetic vortex state in a circular nanodisk was studied under a perpendicular alternating magnetic field that excites the radial modes of the magnetic resonance. Here, we show that as the oscillating frequency is swept down from a frequency higher than the eigenfrequency, the amplitude of the radial mode is almost doubled to the amplitude at the fixed resonance frequency. This amplitude has a hysteresis vs. frequency sweeping direction. Our result showed that this phenomenon was due to a Duffing-type nonlinear resonance. Consequently, the amplitude enhancement reduced the vortex core-switching magnetic field to well below 10 mT. A theoretical model corresponding to the Duffing oscillator was developed from the Landau–Lifshitz–Gilbert equation to explore the physical origin of the simulation result. This work provides a new pathway for the switching of the magnetic vortex core polarity in future magnetic storage devices
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